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Enhanced Shear Thickening of Silica Colloidal Suspension Using Polystyrene-Polyacrylamide Particles

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Abstract

Shear thickening (ST) refers to a non-Newtonian behavior of concentrated colloidal suspensions, which exhibits significant viscosity increments at high shear stress or high shear rate. A shear thickening fluid (STF) consists of well-dispersed solid particles in a liquid medium. Silica particles are often used as components of STFs due to the abundance of hydroxyl groups on their surfaces. Polystyrene core-polyacrylamide shell particles (PS-PAAm particles) were prepared to enhance the ST of silica particle-based colloidal suspensions. Addition of PS-PAAm particles to various particle weight fractions of silica particle-based STFs resulted in amplification of ST in all instances. These results suggest that PS-PAAm particles enhance inter-particle interactions due to the abundance of hydrogen-bonding donor groups in polyacrylamide.

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Author notes

  1. Hoon Soo Son and Kyoung Ho Kim are co-first authors and contributed equally.

Authors and Affiliations

  1. Department of Polymer Science and Engineering, Pusan National University, Busan, 46241, Korea

    Hoon Soo Son, Kyoung Ho Kim, Eun Ho Lee, Joo Hyun Song & Hyun-jong Paik

  2. Advanced Industrial Chemistry Research Center, Korea Research Institute of Chemical Technology, Ulsan, 44412, Korea

    Joo Hyun Song, Wonjoo Lee & Bongkuk Seo

  3. Department of Chemical Engineering, Kumoh National Institute of Technology, Gumi, 39177, Korea

    Jun Hyeong Kim & Kwan Han Yoon

  4. Industry-Academic Cooperation, Kumoh National Institute of Technology, Gumi, 39177, Korea

    Young Sil Lee

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  1. Hoon Soo Son
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  2. Kyoung Ho Kim
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  3. Eun Ho Lee
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  4. Joo Hyun Song
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  7. Jun Hyeong Kim
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  9. Young Sil Lee
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  10. Hyun-jong Paik
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Correspondence to Young Sil Lee or Hyun-jong Paik.

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Acknowledgments: This work was supported by the Industrial Strategic Technology Development Program (No. 10063082/10070127) funded by the Ministry of Trade, Industry and Energy of Korea. This is also supported by the Agency for Defense Development of Korea (No. ADD-15-210-502-026). Research has been performed as a cooperation project of “The development of Sustainable materials technology for Eco-Automobile” supported by the Korea Research Institute of Chemical Technology. Assistance in XPS analysis from Korea Basic Science Institute Busan Center is acknowledged.

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Son, H.S., Kim, K.H., Lee, E.H. et al. Enhanced Shear Thickening of Silica Colloidal Suspension Using Polystyrene-Polyacrylamide Particles. Macromol. Res. 28, 523–529 (2020). https://doi.org/10.1007/s13233-020-8069-1

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  • DOI: https://doi.org/10.1007/s13233-020-8069-1

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