Skip to main content

Advertisement

Log in

Production of pure hydrogen from methane by low temperature plasma processing

  • Materials (Organic, Inorganic, Electronic, Thin Films)
  • Published:
Korean Journal of Chemical Engineering Aims and scope Submit manuscript

Abstract

Production of pure hydrogen from methane by a low temperature plasma process coupled with catalytic reaction was investigated. In low temperature plasma, methane molecules were converted to thin solid films and hydrogen. The conversion of methane and the hydrogen yield depended on the flow rate of methane and the discharge power for the low temperature plasma process. They increased as the flow rate decreased and the discharge power increased. A conversion as high as 87.4% and hydrogen yield as high as 67% could be obtained, but the purity of the hydrogen was less than 90%. The purity could be increased to 100% by coupling the low temperature plasma process with a catalytic reaction using a plasma-catalyst hybrid system.

This is a preview of subscription content, log in via an institution to check access.

Access this article

Price excludes VAT (USA)
Tax calculation will be finalised during checkout.

Instant access to the full article PDF.

Similar content being viewed by others

References

  1. P. Beckhaus, A. Heinzel, J. Mathiak and J. Roes, J. Power Sources, 127,294(2004).

    Article  CAS  Google Scholar 

  2. S.C. Tsang, J. B. Claridge and M.L.H. Green, Catal. Today, 23,3(1995).

    Article  CAS  Google Scholar 

  3. A. Demirbas, Energy Convers. Manage., 43,897(2002).

    Article  CAS  Google Scholar 

  4. S. G. Wang, Y.W. Li, J. X. Lu, M.Y. He and H. Jiao, J. Mol. Struct., 673,181(2004).

    Article  CAS  Google Scholar 

  5. K. Murata, M. Saito, M. Inaba and I. Takahara, Appl. Catal. B: Environmental, 70,509(2007).

    Article  CAS  Google Scholar 

  6. H. Ahmad, S. K. Kamarudin, L. J. Minggu and M. Kassim, Renw. Sust. Energy Rev., 43,599(2015).

    Article  CAS  Google Scholar 

  7. N. Majidian, N. Habibi and M. Rezaei, Korean J. Chem. Eng., 31,1162(2014).

    Article  CAS  Google Scholar 

  8. K. Srilatha, D. Srinivasulu, S.U.B. Ramakrishna and V. Himabindu, Int. J. Innovation and Studies, 9,490(2014).

    CAS  Google Scholar 

  9. M. Seong, M. Shin, J.-H. Cho, Y.-C. Lee, Y.-K. Park and J.-K. Jeon, Korean J. Chem. Eng., 31,412(2014).

    Article  CAS  Google Scholar 

  10. G. Heinz, Hydrocarbon Process. Petrol. Refiner, 41,159(1962).

    Google Scholar 

  11. A. I. Pushkarev, A.-M. Zhu, X.-S. Li and R.V. Sazonov, High Energy Chem., 43,156(2009).

    Article  CAS  Google Scholar 

  12. S. C. Kim, M. S. Lim and Y. N. Chun, Trans. Korean Hydrogen New Energy S., 17,362(2006).

    Google Scholar 

  13. L. Bromberg, D. R. Cohn and A. Rabinovich, Energy Fuels, 12,11(1998).

    Article  CAS  Google Scholar 

  14. D. H. Lee and T. Kim, Int. J. Hydrogen Energy, 38,6039(2013).

    Article  CAS  Google Scholar 

  15. W. J. Cho, J. Ind. Eng. Chem., 16,20(2010).

    Article  CAS  Google Scholar 

  16. N. Rahemi, M. Haghighi, A.A. Babaluo, M.F. Jafari and S. Allahyari, Korean J. Chem. Eng., 31,1553(2014).

    Article  CAS  Google Scholar 

  17. D.B. Nguyen and W.G. Lee, Korean J. Chem. Eng., 32,62(2015).

    Article  CAS  Google Scholar 

  18. D. L. Cho, D.C. Chung and G.-S. Kim, J. Ind. Eng. Chem., 13,287(2007).

    CAS  Google Scholar 

  19. H. Yasuda, Plasma Polymerization, Academic Press, New York (1985).

    Google Scholar 

Download references

Author information

Authors and Affiliations

Authors

Corresponding author

Correspondence to Dong Lyun Cho.

Rights and permissions

Reprints and permissions

About this article

Check for updates. Verify currency and authenticity via CrossMark

Cite this article

Cho, D.L., Kim, HN., Lee, M. et al. Production of pure hydrogen from methane by low temperature plasma processing. Korean J. Chem. Eng. 32, 2519–2523 (2015). https://doi.org/10.1007/s11814-015-0107-x

Download citation

  • Received:

  • Accepted:

  • Published:

  • Issue Date:

  • DOI: https://doi.org/10.1007/s11814-015-0107-x

Keywords

Navigation