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Improvement of quality in the evaluation of radium isotopes 224,226,228Ra in oil scale samples

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Abstract

Elevated concentrations of the radium isotopes 224,226,228Ra exist in the scale and produced water in oil exploration. The activity concentration of 226Ra was calculated from 186.2 keV peak with no usual spectral interference of 185.7 from 235U. The activity concentration of 228Ra was calculated from its first daughter product 228Ac using the 911.2 keV gamma rays since it is a pure beta emitter. The activity concentration of 224Ra was calculated from 212Pb using the 238.6 keV gamma-ray and the secular equilibrium equation with 228Ra. The IAEA 448 (oil contaminated field soil) reference material was used as a quality control for 226,228Ra and but was unreliable for 224Ra using 212Pb.

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References

  1. Burton EF (1904) University of Toronto, Physical Science Series, p 35

  2. McLennan JC (1906) On the radioactivity of mineral oils and natural gases. https://archive.org/stream/transactionsint06conggoog#page/n406/mode/2up/search/McLennan. Accessed July 2019

  3. Raloff J (1991) NORM-the new hot wastes. Sci News 140:264–267

    Article  Google Scholar 

  4. Wilson AJ, Scott LM (1992) Characterization of radioactive petroleum piping scale with an evaluation of subsequent land contamination. Health Phys 63:681–685

    Article  CAS  Google Scholar 

  5. Al-Saleh FS, Al-Harshan GA (2008) Measurements of radiation level in petroleum products and wastes in Riyadh City refinery. J Environ Radioact 99:1026–1031

    Article  CAS  Google Scholar 

  6. Gazineu MHP, Hazin CA (2008) Radium and potassium-40 in solid wastes from the oil industry. Appl Radiat Isot 66:90–94

    Article  CAS  Google Scholar 

  7. Jodlowski P, Macuda J, Nowak J et al (2017) Radioactivity in wastes generated from shale gas exploration and production—North-Eastern Poland. J Environ Radioact 175–176:34–38

    Article  Google Scholar 

  8. Hilal MA, Attallahm MF, Mohamed GY, Fayez-Hassan M (2014) Evaluation of radiation hazard potential of TENORM waste from oil and natural gas production. J Environ Radioact 136:121–126

    Article  CAS  Google Scholar 

  9. Abdullah J, Al-Masri M, Amin Y et al (2017) An innovative procedure for NORM scales treatment and radionuclides separation. Appl Radiat Isotop 125:139–143

    Article  CAS  Google Scholar 

  10. Babatunde B, Sikoki F, Avwiri F et al (2019) Review of the status of radioactivity profile in the oil and gas producing areas of the Niger delta region of Nigeria. J Environ Radioact 202:66–73

    Article  CAS  Google Scholar 

  11. Torres L, Yadav O, Khan E (2018) Risk assessment of human exposure to Ra-226 in oil produced water from the Bakken Shale. Sci Total Environ 626:867–874

    Article  CAS  Google Scholar 

  12. Shawky S, Amer H, Nada AA, Abd El-Maksoud TM, Ibrahiem NM (2001) Characteristic of NORM in the oil industry from eastern and western deserts of Egypt. Appl Radiat Isot 55:135–139

    Article  CAS  Google Scholar 

  13. Landsberger S, Tamalis D, Leblanc C, Yoho MD (2017) Disequilibrium in the uranium and actinium series in oil scale samples. J Environ Radioact 166:126–129

    Article  CAS  Google Scholar 

  14. Millsap DW, Landsberger S (2015) Self-attenuation as a function of gamma-ray energy in naturally occurring radioactive material from oil exploration. Appl Radiat Isot 97:21–23

    Article  CAS  Google Scholar 

  15. Landsberger S, Morton J, Yoho MD (2016) Quality control in the analysis of radioactivity from the oil exploration sector. J Radioanal Nucl Chem 307:2539–2542

    Article  CAS  Google Scholar 

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Correspondence to Sheldon Landsberger.

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Okyay, S., Ozden, B., Asper, N. et al. Improvement of quality in the evaluation of radium isotopes 224,226,228Ra in oil scale samples. J Radioanal Nucl Chem 322, 1305–1309 (2019). https://doi.org/10.1007/s10967-019-06872-4

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  • DOI: https://doi.org/10.1007/s10967-019-06872-4

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