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Magnetic Ordering in BaFe\(_{11.9}\)In\(_{0.1}\)O\(_{19}\) Hexaferrite

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Abstract

The crystal and magnetic structure by powder neutron diffractometry as well as the magnetic properties by vibration sample magnetometry for the BaFe\(_{11.9}\)In\(_{0.1}\)O\(_{19}\) polycrystalline sample have been performed in a wide temperature range from 10 up to 730 K and in magnetic field up to 14 T. The atomic coordinates and lattice parameters have been Rietveld refined. The Invar effect has been observed in the low-temperature range below 150 K. It was explained by the thermal oscillation anharmonicity of atoms. The increase of the microstress value with decreasing temperature has been defined from Rietveld refinement. It is established that the ferrimagnet–paramagnet phase transition is a standard second-order one. From the macroscopic magnetization measurement, the Curie temperature and ordered magnetic moment per nominal iron ion are obtained. From the microscopic diffraction measurement, the magnetic moments at different atomic position and total magnetic moment per iron ion have been defined at different temperatures. The most likely reasons and the mechanism of magnetic ordering are discussed.

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Acknowledgments

This work was carried out with the financial support in part from the Ministry of Education and Science of the Russian Federation in the framework of Increase Competitiveness Program of NITU “MISIS” among the leading world scientific and educational centers (Nos. K4-2015-040, K3-2016-019), with support and within the state order of the Russian Federation on the organization of scientific work and by the Belarusian Republican Foundation for Basic Research (No. F15D-003), and Joint Institute for Nuclear Research (No. 04-4-1121-2015/2017).

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Authors and Affiliations

  1. SSPA “Scientific and practical materials research centre of NAS of Belarus”, P.Brovki str .19, 220072, Minsk, Belarus

    S. V. Trukhanov, A. V. Trukhanov & I. S. Kazakevich

  2. National University of Science and Technology MISiS, Leninsky Prospekt 4, 119049, Moscow, Russia

    S. V. Trukhanov, A. V. Trukhanov, V. G. Kostishin & L. V. Panina

  3. Joint Institute for Nuclear Research, Joliot-Curie str 6, 141980, Dubna, Russia

    V. O. Turchenko & A. M. Balagurov

  4. Donetsk Institute of Physics and Technology named after A.A.Galkin of the NAS of Ukraine, 72 R.Luxemburg Str, 83114, Donetsk, Ukraine

    V. O. Turchenko

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  1. S. V. Trukhanov
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Trukhanov, S.V., Trukhanov, A.V., Turchenko, V.O. et al. Magnetic Ordering in BaFe\(_{11.9}\)In\(_{0.1}\)O\(_{19}\) Hexaferrite. J Low Temp Phys 186, 44–62 (2017). https://doi.org/10.1007/s10909-016-1646-1

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