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Boron network ion modulation and composite alumina densification sintering study of MABS glass for LTCC

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Abstract

In this paper, we investigated the effect of B2O3 content in borosilicate glass on the glass properties and the effect of particle-size gradation on the low-temperature co-fired ceramic composites of MABS (MO–Al2O3–B2O3–SiO2) (M = Ca, Mg) glass composite with alumina after optimization of boron content. We prepared a series of MO–Al2O3–B2O3–SiO2 glasses with different B2O3 contents and MABS glass/Al2O3 composites with different particle-size gradation pairings. The results showed that the appropriate amount of B2O3 content not only enhanced the glass network structure but also inhibited the precipitation of harmful crystalline phases. The optimized particle-size gradation promoted the sintering densification and improved the green tape stacking density, dielectric, and mechanical properties. The composites prepared by sintering the MABS glass with a B2O3 content of 9.5 wt% and a particle size of 3.0 μm with 7.71 μm Al2O3 at 830 °C exhibited good performance with a green tape density of 2.01 g/cm3, a sintered density of 3.12 g/cm3, a z-axis shrinkage of 17.10%, a dielectric constant of 8.26, a dielectric loss of 0.6 \(\times\)10–3 (at 7 GHz), coefficient of thermal expansion 6.75 ppm/°C, and flexural strength 299 MPa, demonstrating broad application potential.

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Acknowledgements

This work was financed by Priority Academic Program Development of Jiangsu Higher Education Institutions (PAPD), Key Research and Development Program of Zhejiang Province (Grant Nos. 2020C0112, 2021C01092)

Funding

This work was financed by Priority Academic Program Development of Jiangsu Higher Education Institutions (PAPD), Key Research and Development Program of Zhejiang Province (Grant Nos. 2020C0112, 2021C01092).

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Authors and Affiliations

  1. College of Materials Science and Engineering, Nanjing Tech University, Nanjing, 210009, China

    Qiang Wang, Yang Lu, Yiting Shan, Shengmin Luo, Tao Que, Xiao Wang & Hongqing Zhou

  2. Jiangsu Collaborative Innovation Center for Advanced Inorganic Function Composites, Nanjing, 210009, China

    Qiang Wang, Yang Lu, Yiting Shan, Shengmin Luo, Tao Que, Xiao Wang & Hongqing Zhou

Authors
  1. Qiang Wang
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  2. Yang Lu
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  3. Yiting Shan
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  4. Shengmin Luo
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  5. Tao Que
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  6. Xiao Wang
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  7. Hongqing Zhou
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Contributions

All authors contributed to the study's conception and design. QW and YL contributed to the conception of this study, performed the experiment, analyzed the data, and wrote the manuscript. YS, SL, TQ, XW, and HZ helped to perform the analysis with constructive discussions. All authors read and approved the final manuscript.

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Correspondence to Hongqing Zhou.

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Wang, Q., Lu, Y., Shan, Y. et al. Boron network ion modulation and composite alumina densification sintering study of MABS glass for LTCC. J Mater Sci: Mater Electron 34, 2086 (2023). https://doi.org/10.1007/s10854-023-11450-2

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