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Growth and property evaluation of nickel–graphite core–shell nanoparticles based on temperature parameters for utilization in silver paste

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Abstract

Herein, the change in the growth characteristics of nickel (Ni)–graphite core–shell nanoparticles (CSNP) based on growth time using thermal chemical vapor deposition method and its utilization in silver (Ag) paste is presented. The characteristics of the graphite shell formed on the surface of Ni–graphite CSNPs exhibited changes in structure, crystallinity, and thickness depending on the growth time. Changes in the characteristics of the graphite shell caused changes in the electrical characteristics of Ni–graphite CSNPs. Ni–graphite CSNPs synthesized based on growth time were able to present synthesis conditions with the most similar characteristics to Ag powder through electrical characteristic evaluation. In addition, through the commercialized Ag paste process, it was suggested that some of the Ag powder could be replaced with Ni–graphite CSNPs and utilized. Through this approach, a plan to improve the price competitiveness of expensive Ag paste was proposed.

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All data generated or analyzed during this study are included in this article.

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Acknowledgements

This work was supported by Materials/Parts Technology Development Program (20007170, Development of carbon materials for fuel cell electrode of FCEV), Technology Innovation Program (20006820, Development of automated system for electrochemical exfoliation of synthetic graphite production residue and multifunctional composite) funded by Ministry of Trade, Industry & Energy (MOTIE, Korea). A portion of this work was supported by Basic Science Research Program through the National Research Foundation of Korea (NRK) funded by the Ministry Education (Grant Number—NRF-2022R1I1A1A01071414). The authors extend their sincere appreciation to the Researchers Supporting Project number (RSP2023R370), King Saud University, Riyadh, Saudi Arabia for the financial support.

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The authors have not disclosed any funding.

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Authors and Affiliations

  1. Research and Development Center, Korea Carbon Industry Promotion Agency, 110-11, Banryong-Ro, Deokjin-Gu, Jeonju-Si, Jeollabuk-Do, 54853, Republic of Korea

    Seung Beom Kang & Kyeong Seok Lee

  2. Carbon Fiber Convergence Technology Research Center, Jeonbuk National University, 567 Baekje-daero, Deokjin-gu, Jeonju-Si, Jeollabuk-Do, 54896, Republic of Korea

    Dong Chul Chung

  3. Department of Physics, Kyungpook National University, 80 Daehakro, Bukgu, Daegu, 41566, Republic of Korea

    Younjung Jo & Chang-Duk Kim

  4. School of Chemical Engineering, Yeungnam University, 280 Daehak-ro, Gyeongsan, Gyeongbuk, 38541, South Korea

    Nguyen Hoang Lam, Jae-hak Jung & Nguyen Tam Nguyen Truong

  5. Department of Chemistry, College of Science, King Saud University, P.O. Box 2455, Riyadh, 11451, Saudi Arabia

    Shoyebmohamad F. Shaikh

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  1. Seung Beom Kang
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  2. Kyeong Seok Lee
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  9. Chang-Duk Kim
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Contributions

Writing—original draft preparation, conceptualization, data interpretation, writing—review and editing, SBK, KSL, DCC, and JJ; data curation validation, resources, NHL and SFS; visualization, formal analysis, supervision, JHJ; project administration, funding acquisition, NTNT and CDK. All authors have read and agreed to the published version of the manuscript.

Corresponding authors

Correspondence to Jae-hak Jung, Nguyen Tam Nguyen Truong or Chang-Duk Kim.

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Kang, S.B., Lee, K.S., Chung, D.C. et al. Growth and property evaluation of nickel–graphite core–shell nanoparticles based on temperature parameters for utilization in silver paste. J Mater Sci: Mater Electron 34, 1912 (2023). https://doi.org/10.1007/s10854-023-11371-0

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