Skip to main content
SpringerLink
Log in

Impedance analysis, modulus behavior, and dielectric properties of La0.6Bi0.1Sr0.15Ca0.15Mn0.9Cu0.1O3 ceramic prepared by sol–gel reaction

  • Published:
Journal of Materials Science: Materials in Electronics Aims and scope Submit manuscript

Abstract

In this paper, we have reported the structural, morphological, complex impedance, complex modulus, and dielectric analyzes of La0.6Bi0.1Sr0.15Ca0.15Mn0.9Cu0.1O3 polycrystalline synthesized by sol–gel process. X-ray diffraction refinement reveals that our material is characterized by phase mixtures of rhombohedral and tetragonal structures with \(R\overline{3 }c\) and I4/mcm space groups, respectively. As for the electric measurements, the dependence on the frequency of the complex impedance was studied at room temperature. The existence of electrical relaxation behavior is revealed, indicating the semi-conductor character of the compound. A comparative study of impedance and modulus responses versus frequency suggests the presence of short-range charge carrier motion. The dielectric analysis indicates a hopping conductivity mechanism in the perovskite material.

This is a preview of subscription content, log in via an institution to check access.

Access this article

Log in via an institution

Price excludes VAT (USA)
Tax calculation will be finalised during checkout.

Instant access to the full article PDF.

Institutional subscriptions

Fig. 1
Fig. 2
Fig. 3
Fig. 4
Fig. 5
Fig. 6
Fig. 7

Similar content being viewed by others

Data availability

Derived data supporting the findings of this study are available from the corresponding author upon request.

References

  1. J.C. Debnath, R. Zeng, J.H. Kim, S.X. Dou, J. Alloy Compd. 509, 3699 (2011)

    Article  CAS  Google Scholar 

  2. P. Nisha, S.S. Pillai, A. Darbandi, A. Misra, K.G. Suresh, M.R. Varma, H. Hahn, J. Phys. D: Appl. Phys. 43, 135001 (2010)

    Article  Google Scholar 

  3. K. McBride, J. Cook, S. Gray, S. Felton, L. Stella, D. Poulidi, CrystEngComm 18, 407–416 (2016)

    Article  CAS  Google Scholar 

  4. L.E. Cross, Ferroelectrics 76, 241 (1987)

    Article  CAS  Google Scholar 

  5. S. Nomura, K. Uchino, Ferroelectrics 50, 197 (1983)

    Article  Google Scholar 

  6. W. Jo, R. Dittmer, M. Acosta, J. Zang, C. Groh, E. Sapper, Ke. Wang, J. Rodel, J. Electroceram. 29, 71 (2012)

    Article  CAS  Google Scholar 

  7. S. Siragam, R.S. Dubey, L. Pappula, G. Satheesh Babu, Sci. Reports 12, 3929 (2022)

    CAS  Google Scholar 

  8. X. Zhang, Z.X. Fang, H.Y. Yang, P. Zhao, X. Zhang, Y.P. Li, Z. Xiong, H.C. Yang, S.R. Zhang, B. Tang, Acta Mater. 206, 116636 (2021)

    Article  CAS  Google Scholar 

  9. W.B. Hong, L. Li, H. Yan, X.M. Chen, J. Am. Ceram. Soc. 102, 5934–5940 (2019)

    Article  CAS  Google Scholar 

  10. J.L. Alonso, L.A. Fernandez, F. Guinia, V. Laliena, V. Martin-Mayor, Phys. Rev. B 66, 104430 (2002)

    Article  Google Scholar 

  11. S.M. Yusuf, M. Sahana, K. Dorr, U.K. Robler, K.H. Muller, Phys. Rev. B 66, 064414 (2002)

    Article  Google Scholar 

  12. R.W. Li, Z.H. Wang, X. Chen, J.R. Sun, B.G. Shen, C.H. Yau, J. Appl. Phys. 87, 5597 (2000)

    Article  CAS  Google Scholar 

  13. J.L. Cohn, M. Peterca, J.J. Neumeier, Phys. Rev. B 70, 214433 (2004)

    Article  Google Scholar 

  14. A. Pimenov, Ch. Hartinger, A. Loidl, A.A. Mukhin, VYu. Ivanov, A.M. Balbashov, Phys. Rev. B 59, 12419 (1999)

    Article  CAS  Google Scholar 

  15. J.R. Sun, G.H. Rao, B.G. Shen, H. Wong, Appl. Phys. Lett. 73, 2998 (1998)

    Article  CAS  Google Scholar 

  16. W. Tong, B. Zhang, S. Tan, Y. Zhang, Phys. Rev. B 70, 403 (1951)

    Google Scholar 

  17. G.M. Keith, C.A. Kirk, K. Sarma, N.M. Alford, E.J. Cussen, M.J. Rosseinsky, D.C. Sinclair, Chem. Mater. 16, 2007 (2004)

    Article  CAS  Google Scholar 

  18. A.M. Smith, H. Duan, A.M. Mohs, S. Nie, Adv. Drug Deliv. Rev. 60, 1226 (2008)

    Article  CAS  Google Scholar 

  19. A. Hadicke, W. Krech, Phys. Rev. B 52, 13526 (1995)

    Article  CAS  Google Scholar 

  20. R. Waser, Solid State Ion 75, 89 (1995)

    Article  CAS  Google Scholar 

  21. S.K. Roy, M.E. Orazem, J. Power Source 184, 212 (2008)

    Article  CAS  Google Scholar 

  22. S. Lanfredi, A.C.M. Rodrigues, J. Appl. Phys. 86, 2215 (1999)

    Article  CAS  Google Scholar 

  23. S. Paul, Manokamna, A. Kumar, A. Kumar, IOP Conf. Series Mater. Sci. Eng. 1225, 012054 (2022)

    Article  CAS  Google Scholar 

  24. G.-T. Pan, S. Chong, T.C.-K. Yang, P. Shukla, W.S. Chiu, J.C. Juan, Results Phys. 7, 2118–2123 (2017)

    Article  Google Scholar 

  25. F. Belkhiria, F.I.H. Rhouma, S. Hcini, M. Daoudi, H. Gammoudi, M. Amlouk, R. Chtourou, J. Lumin. 181, 1–7 (2017)

    Article  CAS  Google Scholar 

  26. E. Bouzaiene, A.H. Dhahri, J. Dhahri, E.K. Hlil, K. Taibi, Appl. Phys. A 12, 126 (2020)

    Google Scholar 

  27. E. Bouzaiene, A.H. Dhahri, J. Dhahri, E.K. Hlil, Inorg. Chem. Commun. 132, 108824 (2021)

    Article  CAS  Google Scholar 

  28. C.V. Vazquez, M.C. Blanco, M.A.L. Quintela, R.D. Sanchez, J. Rivas, S.B. Oseroff, J. Mater. Chem. 8, 991–1000 (1998)

    Article  Google Scholar 

  29. B. Garbarz-Glos, W. Bąk, M. Antonova, M. Pawlik, Mater. Sci. Eng. 49, 012031 (2013)

    CAS  Google Scholar 

  30. S. Selvasekarapandian, M. Vijaykumar, J. Mater. Chem. Phys. 80, 29–33 (2003)

    Article  CAS  Google Scholar 

  31. H. Rahmouni, A. Selmi, K. Khirouni, N. Kallel, J. Alloys Compd. 533, 93 (2012)

    Article  CAS  Google Scholar 

  32. J. Suchanicz, Mater. Sci. Eng. 55, 114 (1998)

    Article  Google Scholar 

  33. H. Baaziz, N.K. Maaloul, A. Tozri, H. Rahmouni, S. Mizouri, K. Khirouni, E. Dhahri, Chem. Phys. Lett. 640, 77–81 (2015)

    Article  CAS  Google Scholar 

  34. J.R. Macdonald, W.B. Johnson, Fundamentals of impedance spectroscopy. in Impedance Spectroscopy: Theory, Experiment, and Applications, 2nd edn. (Wiley, Newark, 2005), pp. 1–26

  35. F.I.H. Rhouma, A. Dhahri, J. Dhahri, H. Belmabrouk, M.A. Valente, Solid State Commun. 152, 1874–1879 (2012)

    Article  CAS  Google Scholar 

  36. H. Rahmouni, M. Smari, B. Cherif, E. Dhahri, K. Khirouni, Dalton Trans. 44, 10457 (2015)

    Article  CAS  Google Scholar 

  37. G. Jayakumar, D.S. Poomagal, A. Albert Irudayaraj, A. Dhayal Raj, S. Kethrin Thresa, P. Akshadha, J. Mater. Sci.: Mater. Electron. 31, 20945–20953 (2020)

    CAS  Google Scholar 

  38. M. Selmi, A. Smida, S. El Kossi, J. Mater. Sci.: Mater. Electron. 32, 6014–6027 (2021)

    CAS  Google Scholar 

  39. A. Shukla, R.N.P. Choudhary, A.K. Thakur, J. Phys. Chem. Solids 70, 1401 (2009)

    Article  CAS  Google Scholar 

  40. D. Johnson, ZPlot, ZView Electrochemical Impedance Software, Version 2.3b (Scribner Associates, Inc., North Carolina, 2000).

  41. R. Charguia, S. Hcini, M. Boudard, A. Dhahri, J. Mater. Sci.: Mater. Electron. 30, 2975–2984 (2019)

    CAS  Google Scholar 

  42. H. Rahmouni, A. Selmi, K. Khirouni, N. Kallel, J. Alloys Compd. 93, 533 (2012)

    Google Scholar 

  43. H. Rahmouni, M. Nouiri, R. Jemai, N. Kallel, F. Rzigua, A. Selmi, K. Khirouni, S. Alaya, J. Magn. Magn. Mater. 316, 23–28 (2007)

    Article  CAS  Google Scholar 

  44. M. Jebli, Ch. Rayssi, J. Dhahri, M. Ben Henda, J. Mater. Sci.: Mater. Electron. 32, 26786–26797 (2021)

    CAS  Google Scholar 

  45. P.B. Macedo, C.T. Moynihan, R. Bose, Phys. Chem. Glasses 13, 171 (1972)

    CAS  Google Scholar 

  46. M.B. Hossen, M.A. Hossain, J. Adv. Ceram. 4, 217 (2015)

    Article  CAS  Google Scholar 

  47. J.R. Macdonald, Solid State Ion. 13, 147 (1984)

    Article  CAS  Google Scholar 

  48. M. Mumtaz, M. Naveed, S. Akhtar, M. Imran, M. Nasir Khan, J. Supercond. Novel Magn. 31, 2691–2698 (2018)

    Article  CAS  Google Scholar 

  49. Ah. Dhahri, E. Dhahri, E.K. Hlil, RSC Adv. 8, 9103–9111 (2018)

    Article  CAS  Google Scholar 

  50. M. Maczka, N.L.M. Costa, A. Gagor, W. Paraguassu, A. Sieradzki, J. Hanuza, Phys. Chem. Chem. Phys. 18, 13993 (2016)

    Article  CAS  Google Scholar 

  51. C. Ang, Z. Yu, L.E. Cross, Phys. Rev. B 62, 228 (2000)

    Article  Google Scholar 

  52. S. Saha, T.P. Sinha, Phys. Rev. B 65, 134103–134107 (2002)

    Article  Google Scholar 

  53. S.K. Rout, S. Parida, E. Sinha, P.K. Barhai, I.W. Kim, Curr. Appl. Phys. 10, 917 (2010)

    Article  Google Scholar 

  54. M.P. Dasari, K. Sambasiva Rao, P. Murali Krishna, G. Gopala Krishna, Acta Phys. Polonica A 119, 387–394 (2011)

    Article  CAS  Google Scholar 

  55. D.C. Sinclair, A.R. West, J. Appl. Phys. 66, 3858 (1989)

    Article  Google Scholar 

  56. R.W. Sillars, J. Inst. Electr. Eng. 80, 378–394 (1937)

    Google Scholar 

  57. S. Kulkarni, B.M. Nagabhushana, N. Parvatikar, A. Koppalkar, C. Shivakumara, R. Damle, Mater. Res. Bull. 50, 197 (2014)

    Article  CAS  Google Scholar 

  58. N.K. Singh, A. Panigrahi, R.N.P. Chaudhary, Mater. Lett. 50, 1 (2001)

    Article  CAS  Google Scholar 

  59. T. Kar, R.N.P. Chaudhary, Mater. Sci. Eng. 90, 224 (2002)

    Article  Google Scholar 

  60. N.V. Prasad, G. Prasad, T. Bhimasankaran, S.V. Suryanarayana, G.S. Kumar, Bull. Mater. Sci. 19, 639 (1996)

    Article  CAS  Google Scholar 

  61. C.G. Koops, Phys. Rev. 83, 121 (1951)

    Article  CAS  Google Scholar 

  62. S. Aydi, W. Chérif, F. Khammassi, A.J.M. Sales, N.M. Ferreira, N. Zouari, Appl. Phys. A 127, 931 (2021)

    Article  CAS  Google Scholar 

  63. Ch. Rayssi, SEl. Kossi, J. Dhahri, K. Khirouni, J. Alloys Compd. 759, 93–99 (2018)

    Article  CAS  Google Scholar 

Download references

Funding

The authors extend their appreciation to the deputyship for Research & Innovation, Ministry of Education in Saudi Arabia for funding this research work through the project number (IFP-2020-139).

Author information

Authors and Affiliations

  1. Faculté des Sciences de Monastir, Laboratoire de la Matière Condensée et des Nanosciences, Université de Monastir, LR 11 ES 40, Monastir, 5019, Tunisie

    E. Bouzaiene, Ch. Rayssi, J. Dhahri & Ab. Afef

  2. Institut National de Sciences Appliquées de Lyon, INSA Lyon, Villeurbanne, France

    Ab. Afef

  3. Department of Physics, College of Science at Zulfi, Majmaah University, Zulfi, 11932, Saudi Arabia

    Hafedh Belmabrouk & M. A. Albedah

Authors
  1. E. Bouzaiene
    View author publications

    You can also search for this author in PubMed Google Scholar

  2. Ch. Rayssi
    View author publications

    You can also search for this author in PubMed Google Scholar

  3. J. Dhahri
    View author publications

    You can also search for this author in PubMed Google Scholar

  4. Ab. Afef
    View author publications

    You can also search for this author in PubMed Google Scholar

  5. Hafedh Belmabrouk
    View author publications

    You can also search for this author in PubMed Google Scholar

  6. M. A. Albedah
    View author publications

    You can also search for this author in PubMed Google Scholar

Contributions

EB Conceptualization, Formal analysis, Investigation, Visualization, Writing—original draft, Writing—review and editing. CHR Formal analysis and Investigation review and editing. EBA Formal analysis and Investigation. JD Visualization and Investigation. HB Visualization and Investigation. MAA Visualization and Investigation.

Corresponding authors

Correspondence to E. Bouzaiene or M. A. Albedah.

Ethics declarations

Conflict of interest

The authors (E. Bouzaiene et al.) declare that there are no conflicts of interest regarding this manuscript.

Additional information

Publisher's Note

Springer Nature remains neutral with regard to jurisdictional claims in published maps and institutional affiliations.

Rights and permissions

Springer Nature or its licensor (e.g. a society or other partner) holds exclusive rights to this article under a publishing agreement with the author(s) or other rightsholder(s); author self-archiving of the accepted manuscript version of this article is solely governed by the terms of such publishing agreement and applicable law.

Reprints and permissions

About this article

Check for updates. Verify currency and authenticity via CrossMark

Cite this article

Bouzaiene, E., Rayssi, C., Dhahri, J. et al. Impedance analysis, modulus behavior, and dielectric properties of La0.6Bi0.1Sr0.15Ca0.15Mn0.9Cu0.1O3 ceramic prepared by sol–gel reaction. J Mater Sci: Mater Electron 34, 285 (2023). https://doi.org/10.1007/s10854-022-09673-w

Download citation

  • Received:

  • Accepted:

  • Published:

  • DOI: https://doi.org/10.1007/s10854-022-09673-w

Search

Navigation