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Effect of heating temperature on excess conductivity and superconducting fluctuations of (Tl0.6Pb0.4)BaSrCaCu2O7

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Abstract

The Tl(Ba/Sr)2CaCu2O7 (Tl-1212) material has a relatively high superconducting critical temperature. With proper elemental substitutions the Ba and Sr only bearing Tl-1212 phase can be readily prepared. In this work we have combined Ba:Sr in 1:1 ratio and determined the role that heating temperature plays on the fluctuations and excess conductivity of (Tl0.6Pb0.4)BaSrCaCu2O7 superconductor. The superconductors were prepared under oxygen flow at 850 to 1000 °C. The Aslamazov-Larkin model was utilized to calculated the dimensionality of fluctuation induced conductivity, λ in the superconductor. The coherence length ξc(0), Josephson coupling J, and anisotropy γ = (ξab(0)/ξc(0)) were determined by the Lawrence-Doniach model. Excess conductivity analyses indicated that as the heating temperature was increased the two-dimensional to three-dimensional conductivity transition temperature decreased. The shortest coherence length, ξc(0) = 0.868 Å, lowest Josephson coupling, and highest anisotropy (γ = 11.516) were exhibited by the sample heated at 1000 °C which also showed the highest zero-resistance–temperature, Tc-zero. These results can be useful in the search for high temperature superconductivity in the cuprates.

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Data from the work shall be provided upon reasonable request.

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Acknowledgements

The Ministry of Higher Education of Malaysia supported this research under Grant No. FRGS/1/2020/STG07/UKM/01/1.

Funding

Ministry of Higher Education, Malaysia, Grant No. (FRGS/1/2020/STG07/UKM/01/1).

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Contributions

MGR and VY performed the experiments and initial data analysis. AAS performed the excess conductivity and fluctuation analyses. RAS contributed to the experimental procedure and writing the paper.

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Correspondence to R. Abd-Shukor.

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Al-Sharabi, A., Ranjbar, M.G., Yazdanian, V. et al. Effect of heating temperature on excess conductivity and superconducting fluctuations of (Tl0.6Pb0.4)BaSrCaCu2O7. J Mater Sci: Mater Electron 33, 10671–10676 (2022). https://doi.org/10.1007/s10854-022-08050-x

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  • DOI: https://doi.org/10.1007/s10854-022-08050-x

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