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Synthesis, structure and dielectric properties of zirconium and titanium oxide-doped lead oxide nano-crystalline films fabricated by sol–gel techniques for energy-storage application

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Abstract

This work aimed to improve the energy storage properties of lead zirconate (PZ) thin films by doping titanium content. Thin films of Pb(0.9)-Zr(0.1) (PZ) and Pb(0.9)-(Zr0.05.Ti0.05)O2 (PZT) were grown epitaxially on a glass substrate by a sol–gel colloidal route at low temperature. The structure of the obtained nanocrystals was checked by X-ray diffraction (XRD), transmission electron microscope (TEM), and electron diffraction (ED). Nanocrystals were distributed evenly of 7 ± 0.2 for PZ and 7.5 ± 0.2 for PZT nm in size and were closely packed. The frequency dependence of dielectric properties and the ferroelectric characteristics were detected. The energy-storage density and energy-storage efficiency estimated from hysteresis loops were about 35.15 J/cm3 and 65.8% for (PZ) and 68.25 J/cm3 and 66.6%for (PZT) for one layer, respectively. Results showed that the titanium content had a clear effect on the dielectric properties, ferroelectric properties, and structural properties, and on the other hand, (PZ) and (PZT) thin films had a potential application in the energy-storage device.

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Acknowledgements

Thanks to the Academy of Scientific Research and Technology (ASRT), this research is a specialized project and was supported financially by the (ASRT), Egypt, Grant No. (6573).

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Authors and Affiliations

  1. Department of Physics, Faculty of Science, Al-Arish University, Al-Arish, Egypt

    F. A. Ibrahim

  2. Academy of Scientific Research and Technology of the Arab Republic of Egypt, Cairo, Egypt

    F. A. Ibrahim

  3. Department of Physics, Faculty of Science, Suez University, Suez, Egypt

    M. M. El-Desoky

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  1. F. A. Ibrahim
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Correspondence to F. A. Ibrahim.

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Ibrahim, F.A., El-Desoky, M.M. Synthesis, structure and dielectric properties of zirconium and titanium oxide-doped lead oxide nano-crystalline films fabricated by sol–gel techniques for energy-storage application. J Mater Sci: Mater Electron 32, 19754–19763 (2021). https://doi.org/10.1007/s10854-021-06500-6

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