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Electrical and energy storage properties of nickel substituted barium bismuth niobate nano-ceramics prepared by chemical route

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Abstract

Nanosized barium nickel bismuth niobate (Ba1−xNixBi2Nb2O9) powders with x = 0.5, abbreviated as BNiBN is prepared through aqueous based chemical method. X-ray diffraction (XRD) analysis and electrical measurements are performed. XRD analysis establishes the orthorhombic structure of BNiBN with A21am (36) space group. The highest intensity peak is (115), which supports bismuth layer structured ferroelectrics of (112m + 1) type. The dielectric study establishes the relaxor behaviour with temperature maxima 150 °C at 10 kHz. Cole–Cole plot of impedance have single semicircle that correlate with grain conductivity. Imaginary impedance versus frequency has relaxation behaviour and activation energy of 0.75 eV is observed. The ac conductivity at high temperature exhibits the hopping behaviour. The charging and discharging energy density and charge–discharge efficiency are calculated from the polarization study at different electric field. The material exhibits a high energy density (> 12 J cm−3) and a high charge–discharge efficiency (> 83%) at room temperature.

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Acknowledgements

Author thanks SERB, DST, New Delhi, India for financial support (Grant No. SR/FT-CS-125,2010). Author also thanks WB DST, Govt. of West Bengal, India (Grant No. 674(Sanc)/ST/P/S&T/15G/5/ 2016 dated 09/11/2016) for financial support. M.K. Adak is thankful to the Council of Scientific and Industrial Research (CSIR), Government of India for the Senior Research Fellowship [Sanction No. 09/1156(0004)/18-EMR-I].

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Authors and Affiliations

  1. Department of Chemistry, Sidho-Kanho-Birsha University, Purulia, 723104, India

    Mrinal K. Adak, Arnab Mukherjee, Anirban Chowdhury, Julekha Khatun & Debasis Dhak

  2. Department of Industrial Chemistry, Ramkrishna Mission Vidyamandira, Belur Math, Howrah, 711202, India

    Uttam K. Ghorai

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  1. Mrinal K. Adak
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Adak, M.K., Mukherjee, A., Chowdhury, A. et al. Electrical and energy storage properties of nickel substituted barium bismuth niobate nano-ceramics prepared by chemical route. J Mater Sci: Mater Electron 29, 15847–15858 (2018). https://doi.org/10.1007/s10854-018-9671-2

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