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Ultralight, superelastic pure graphene aerogel for piezoresistive sensing application

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Abstract

Graphene aerogel (GA), with low density, high conductivity, and good mechanical properties, has important application potentials in the field of flexible electronics. Here, a balanced approach was developed in this work: Graphene oxide (GO) nanosheets were induced to assemble into a homogeneous porous hydrogel under alkali induction, and then, the oxygen-containing functional groups of GO were removed by reductant of formamidine sulfonic acid (FAS). Besides, the hydrogel of GA precursor can be quickly dried at a high temperature (150 °C) within 30 min to obtain pure GA of FGA. After further calcination, the obtained aerogel of AFGA with ordered structure has ultralow density (3.88 mg/cm3), high conductivity (7.4 S/m), supercompression recovery performance (99%), high sensitivity (S = 0.83 kPa−1), large reversible compression cycle performance (200 cycles under 90% strain), and high fatigue resistance (10,000 cycles under 70% strain), which presents excellent piezoresistive properties and can find wide applications in piezoresistive sensors as the high-performance sensing material.

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Acknowledgements

This work was funded by the National Natural Science Foundation of China (No. 51975562) and the National Basic Research Program of China (JCKY2019130C105).

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Authors and Affiliations

  1. State Key Laboratory of Solid Lubrication, Lanzhou Institute of Chemical Physics, Chinese Academy of Sciences, Lanzhou, 730000, China

    Gaochuang Yang, Tiandi Chen, Jinqing Wang, Limin Ma & Shengrong Yang

  2. Center of Materials Science and Optoelectronics Engineering, University of Chinese Academy of Sciences, Beijing, 100049, China

    Gaochuang Yang, Jinqing Wang, Limin Ma & Shengrong Yang

  3. School of Stomatology, Lanzhou University, Lanzhou, 730000, China

    Xiaoli Qin

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  1. Gaochuang Yang
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Yang, G., Qin, X., Chen, T. et al. Ultralight, superelastic pure graphene aerogel for piezoresistive sensing application. J Mater Sci 58, 850–863 (2023). https://doi.org/10.1007/s10853-022-08113-8

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