Abstract
Conductive polymer composites based strain sensors have been widely investigated in recent years. However, the integration of a wide strain detection range and high sensitivity is still challenging. In this work, a double-percolation structured fiber strain sensor based on a carbon nanotube (CNT)/styrene butadiene styrene (SBS) conductive phase and a thermoplastic polyurethane (TPU) insulating phase (CNT/SBS@TPU) was fabricated using a simple melt mixing and fused filament fabrication strategy. The effect of SBS: TPU ratios on the electrical and sensing properties of samples was investigated, at 1 wt% CNT loading. It was shown that the SBS: TPU ratios significantly affected the performance of sensors. The highest conductivity of 1.08 × 10–3 S/m was obtained for SBS/5-TPU/5 (SBS: TPU = 5: 5). Due to the squeezing and interruptive effects of the insulating phase, SBS/5-TPU/5 showed a high sensitivity of 2,645,866, wide detection range (0.2%-92% strain), high linearity (R2 = 0.95 at 0–10% strain) and excellent stability (2000 cycles). Additionally, the SBS/5-TPU/5 sensor could effectively monitor varying frequencies within 0.05–1 Hz and showed prospective applications in human motion monitoring and tactile recognition. This work provides a route for manufacturing high-performance fiber strain sensors used for wearable intelligent devices and human-computer interaction.
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The datasets generated during and/or analysed during the current study are available from the corresponding author on reasonable request.
References
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Funding
This work was supported by the National Natural Science Foundation of China (12102374, 52173301), the Sichuan Science and Technology Program (2021YFH0031, 2022JDGD0015 and 2022YFH0019), the International Cooperation Project of Chengdu (2019-GH02-00054-HZ), Special Funded Postdoctoral Program of Sichuan Province (021609912), Open Experimental Program of SWPU (2021KSP05008), and Innovative Research Team of SWPU (2017CXTD01).
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Dong Xiang and Libing Liu contributed equally to this work.
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Xiang, D., Liu, L., Xu, F. et al. Highly Sensitive Flexible Strain Sensor Based on a Double-percolation Structured Elastic Fiber of Carbon Nanotube (CNT)/Styrene Butadiene Styrene (SBS) @ Thermoplastic Polyurethane (TPU) for Human Motion and Tactile Recognition. Appl Compos Mater 30, 307–322 (2023). https://doi.org/10.1007/s10443-022-10084-7
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DOI: https://doi.org/10.1007/s10443-022-10084-7