Skip to main content
Log in

Comparative study and TALYS 1.6 code calculations for the excitation functions of P and α-induced reactions on Bi target with special attention to the medical radioisotope 211At

  • Regular Article
  • Published:
The European Physical Journal Plus Aims and scope Submit manuscript

Abstract

The induced reactions by light ions such as protons, deuterons, 3He and α-particles on 209Bi, as the heaviest stable isotope in the periodic table, are important for the production of heavy radioactive isotopes. These radioactive isotopes are mainly α-emitters and could be used in cancer therapy. In this study, 209Bi(p,2n)208Po, 209Bi(p,3n)207Po, 209Bi(p,4n)206Po and 209Bi(p,5n)205Po reactions were studied by collecting the previously measured excitation functions, holding an inter-comparison and performing code calculations using the TALYS 1.6 code. As a result of the inter-comparison, mathematical fit for each reaction was given. α-induced reactions on 209Bi target leading to the formation of 210,211At and 210Po radioisotope were also studied through this work. The production of 211At without considerable isotopic 210At impurities was discussed. The previously measured excitation functions were fitted as before, and TALYS 1.6 code calculation was performed. The code calculations were compared with the mathematical fitted excitation functions.

This is a preview of subscription content, log in via an institution to check access.

Access this article

Price excludes VAT (USA)
Tax calculation will be finalised during checkout.

Instant access to the full article PDF.

Fig. 1
Fig. 2
Fig. 3
Fig. 4
Fig. 5
Fig. 6
Fig. 7

Similar content being viewed by others

References

  1. S.K. Imam, Advancements in cancer therapy with alpha-emitters: a review. Int. Radiat. Oncol. Phys. 51, 271–278 (2001)

    Google Scholar 

  2. A.J. Koning, S. Hilaire, S. Goriely, TALYS-1.6: A Nuclear Reaction Program. User Manual, Netherlands. http://www.talys.edy/download-talys. Accessed Dec 2015

  3. TableCurve 2D,Version 4.06, Copyright 1989–1996, AISN Software

  4. https://www.nndc.bnl.gov/nudat2/. Accessed 7 Nov 2018

  5. C.G. Andre, J.R. Huizenga, J.F. Mechi, W.J. Ramler, E.G. Rauh, S.R. Rocklin, Proton cross sections of Bi-209. Phys. Rev. 101, 645 (1956)

    Google Scholar 

  6. P.J. Daly, P.F.D. Sahw, Radiative proton capture cross-sections in heavy nuclei. Nucl. Phys. 56, 322 (1964)

    Google Scholar 

  7. K. Miyano, H. Nakahara, The cross section and the recoil range study of the 209Bi(p,n) and (p,2n) reactions. J. Phys. Soc. Jpn. 35(4), 953 (1973)

    Google Scholar 

  8. R.E. Bell, H.M. Skarsgard, Cross sections of (p,xn) reactions in the isotopes of lead and bismuth. Can. J. Phys. 34, 745 (1956)

    Google Scholar 

  9. C. Birattari, E. Gadioli, A.M. Grassi, G. Strini, G. Tagliaferri, L. Zetta, (P,XN) Reactions induced in 169Tm, 181Ta and 209Bi with 20 to 45 MeV protons. Nucl. Phys. Sect. A 166, 605 (1971)

    Google Scholar 

  10. Z. Bao, J. Chen, J. Meng, S. Huang, The measurement of the ratio gamma-F/gamma-n and the fission barrier height for p+209Bi. Chin. J. Nucl. Phys. (Beijing) 12(1), 55 (1990)

    Google Scholar 

  11. J. Kuhnhenn, U. Herpers, W. Glasser, R. Michel, P. W. Kubik, M. Suter, Thin target cross sections for proton-induced production of radionuclides from lead and bismuth over the proton energy range from 9 to 71 MeV. Radiochim. Acta 89(11–12), 697–702 (2001)

    Google Scholar 

  12. L. Mochtari Oranj, N.S. Jung, M. Bakhtiari, A. Lee, H.S. Lee, Cross section of proton-induced reactions on bismuth and lead up to 100 MeV. Phys. Rev. C95, 044609 (2017)

    Google Scholar 

  13. L. Milazzo-Colli, G.M. Braga-Marcazzan, M. Milazzo, Further measurements of the probability of alpha cluster pre-formation by means of (p,alpha) reactions in heavy elements. Nuovo Cimento A 30, 632 (1975)

    Google Scholar 

  14. E.L. Kelly, E. Segre, Some excitation functions of bismuth. Phys. Rev. 75, 999 (1949)

    Google Scholar 

  15. W.J. Ramler, J. Wing, D.J. Henderson, J.R. Huizenga, Excitation functions of bismuth and lead. Phys. Rev. 114, 154 (1959)

    Google Scholar 

  16. K.J. Hofstetter, J.D. Stickler, Comparison of 3He-, 4He-, and 12C-induced nuclear reactions in heavy-mass targets at medium excitation energies. Experimental cross sections. Phys. Rev. Part C Nucl. Phys. 9, 1064 (1974)

    Google Scholar 

  17. R.M. Lambrecht, S. Mirzadeh, Cyclotron isotopes and radiopharmaceuticals astatine-211. Appl. Radiat. Isot. 36(6), 443 (1985)

    Google Scholar 

  18. A. Hermanne, F. Tarkanyi, S. Takacs, Z. Szucs, Y.N. Shubin, A.I. Dityuk, Experimental study of the cross sections of alpha-particle induced reactions on Bi-209. Appl. Radiat. Isot. 63, 1 (2005)

    Google Scholar 

  19. L. MacFadden, G.R. Satchler, Nucl. Phys. 84, 177 (1960)

    Google Scholar 

  20. P. Demetrion, C. Grama, S. Goriely, Nucl. Phys. A707, 253 (2002)

    Google Scholar 

  21. A.J. Koning, D. Rochman, Modern nuclear data evaluation with the TALYS code system. Nucl. Data Sheets 113, 2841–2934 (2012)

    Google Scholar 

  22. I.A. Rizvi, M.K. Bhardwaj, M. Afzal Ansari, A.K. Chaubey. Non-equilibrium reaction mechanism in alpha-particle induced excitation function for 209Bi up to 60 MeV, Appl. Radiat. Isot. 41, 215 (1990)

    Google Scholar 

  23. N.L. Singh, S. Mukherjee, D.R.S. Somayajulu, Non-equilibrium analysis of (a, xn) reactions on heavy nuclei. Nuovo Cimento A 107, 1635 (1994). (Italy)

    Google Scholar 

  24. H.B. Patel, D.J. Shah, N.L. Singh, Study of (α,xn) Reactions on 169Tm, 181Ta and 209Bi up to 70 MeV. Nuovo Cimento A 112, 1439 (1999)

    Google Scholar 

Download references

Author information

Authors and Affiliations

Authors

Corresponding author

Correspondence to A. Azzam.

Rights and permissions

Reprints and permissions

About this article

Check for updates. Verify currency and authenticity via CrossMark

Cite this article

Azzam, A., Alharby, A.A. Comparative study and TALYS 1.6 code calculations for the excitation functions of P and α-induced reactions on Bi target with special attention to the medical radioisotope 211At. Eur. Phys. J. Plus 135, 192 (2020). https://doi.org/10.1140/epjp/s13360-020-00223-z

Download citation

  • Received:

  • Accepted:

  • Published:

  • DOI: https://doi.org/10.1140/epjp/s13360-020-00223-z

Navigation