Summary
A model of the polluted arctic troposphere is constructed to estimate the magnitude and seasonal variation of the climate forcing function of arctic haze. Using a pill-box “bathtub model” for the Arctic and envisioning it to be filled with pollution from industrial sources in Eurasia, we estimate that maximum climate perturbation from arctic contamination occurs in the spring months. The major perturbation to the radiation budget is a lowering of the albedo (heating) of the earth-atmosphere system around the vernal equinox and is due to a trace amount (about 5% by mass) of black carbon associated with the removal-resistant submicron mode of aerosols. The black carbon over the reflecting polar ice/snow introduces a heating of about 1.5 degree per day into the haze layer.
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Agarwal, J. K., Sem, G. J., 1980: Continuous flow, single-particle-counting condensation nucleus counter.J. Aerosol Sci.,11, 343–357.
Barrie, L. A., Hoff, R. M., 1984: The oxidation rate and residual time of sulfur dioxide in the Arctic atmosphere.Atmos. Environ.,18, 2711–2722.
Barrie, L., 1986: Arctic air chemistry: an overview, pp. 5–24. In: Stonehouse, B. (ed.),Arctic Air Pollution. Cambridge: Cambridge University Press, 328 pp.
Barry, R. G., 1967: Seasonal location at the Arctic front over North America.Geographical Bull.,9, 79–95.
Blanchet, J. P., List, R., 1983: Estimation of optical properties of arctic haze using a numerical model.Atmos. Ocean,21, 444–465.
Blanchet, J. P., 1991: Potential climate change from arctic aerosol pollution. In: Sturges, W. T. (ed.),Pollution of the Arctic Atmosphere. New York: Elsevier Science Publishers, pp. 289–322.
Chuan, R. L., 1970: A new method for measuring particulate mass.J. Aerosol. Sci.,7, 111–114.
Djupström, M., Pacyma, J. M., Maenhaut, W., Winchester, J. W., Li, S. M., Shaw, G. E., 1993: Contamination of Arctic air during a haze even in late winter 1986.Atmos. Env. (in press).
Fox, J. D., 1993: Calculated Angstrom's turbidity coefficients for Fairbanks, Alaska.J. Climate (in press).
Hansen, A. D. A., Rosen, H., 1984: The set balemeter — an instrument for the real-time measurement of optical absorption by aerosol particles.Sci. Total Env.,36, 191–196.
Hinds, W. C., Kraske, G., 1986: Performance of PMS micro LAS optical particle counter.J. Aerosol Sci.,17, 67.
Kead, P. B., Quauy, F. R., Sem, G. J., 1983: Differential mobility particle sizer: A new instrument for high-resolution aerosol size distribution measurements below 1 micron.TSI Quarterly,9, 3–11.
Knutson, E. O., 1989: Personal computer programs for use in radon/thoron progeny measurements, Env. Measurements Laboratory, U.S. Dept. of Energy report EML-517, available from NTIS.
Rosen, H., Novakov, T., 1993: Identification of combustion generated carbon particles in the Arctic atmosphere.Nature (in press).
Rosen, H., Hansen, A. D. A., Gendel, L., Novakov, T., 1978: Identification of the graphitic carbon component of source and ambient particulate by Raman spectroscopy and an optical attenuation technique.Appl. Optics,17, 3859–3861.
Shaw, G. E., Stamnes, K., 1980: Arctic Haze: Perturbation of the Polar Radiation Budget.Annals of the New York Academy of Science,338, 533–539.
Shaw, G. E., 1981: Eddy diffusion transport of Arctic pollution from the mid-latitudes: a preliminary model.Atmos. Environ.,15, 1483–1490.
Shaw, G. E., 1982: Atmospheric turbidity in the polar regions.J. Appl. Meteor.,21, 1080–1800.
Shaw, G. E., 1987: Aerosols as climate regulators: a climate-biosphere linkage.Atmos. Env.,21, 985–986.
Shaw, G. E., Khalil, M. A. K., 1989: Arctic Haze,Handbook of Environmental Chemistry,4, Part B, 70–111. Berlin: Springer.
Shaw, G. E., 1991: Aerosol chemical components in Alaska air masses. 1. Aged pollution.J. Geophys. Res.,96, 21357–21368.
Sinclair, D., Hoopes, B. S., 1975: A novel form of diffusion battery.J. Amer. Ind. Hygiene Assoc.,36, 39–42.
Stamnes, K., Tsay, S.-C., Wiscombe, W. J., Jayaweera, K., 1988: Numerically stable algorithm for discrete-ordinate-method radiative transfer in multiple scattering and emitting layered media.Applied Optics,27, 2502–2509.
Stamnes, K., Tsay, S. C., 1990: Optimum spectral resolution for computing atmospheric heating and photodissociation rates.Planet. Space Sci.,38, 807–820.
Sturgis, W. T., Shaw, G. E., Dutton, O. 1993: Halogens in aerosols in central Alaska. (in preparation).
Tsay, S.-C., Stephens, G. L.: A physical/optical model for atmospheric aerosols with applications to visibility problems, ISSN 0737-5352-16, p 34, Report available from Department of Atmospheric, Colorado State University, Fort Collins, CO 80523.
Tsay, S.-C., Stamnes, K., Jayaweera, K., 1990: Radiative transfer in stratified atmospheres: Description and validation of a unified model.J. Quant. Spectrosc. Radiat. Transfer,43, 133–148.
Whitby, K., 1978: The physical characteristics of sulfur aerosols.Atmos. Env.,12, 135–159.
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Shaw, G.E., Stamnes, K. & Hu, Y.X. Arctic haze: Perturbation to the radiation field. Meteorl. Atmos. Phys. 51, 227–235 (1993). https://doi.org/10.1007/BF01030496
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DOI: https://doi.org/10.1007/BF01030496