Abstract
The possibility of carrying out temperature and concentration measurements in gases by a Raman spectroscopy analysis was suggested and demonstrated about a decade ago. Following some early publications on this subject [1,2], a massive effort was undertaken in order to evaluate the potential of spontaneous Raman scattering in the important areas of atmospheric sounding and combustion diagnostics. In these experiments, the concentrations of the molecular species are deduced from the intensities of their respective Raman bands and the temperature is obtained from the contour of any one of these bands. Detailed accounts of early experimental work can be found, among other publications, in several Project SQUID and AIAA workshop proceedings [3–5]. Important instrumental developments were accomplished, with improved collection efficiencies and signal to noise ratio enhancement. The fields of applications were rapidly delineated and it appeared that spontaneous Raman scattering could prove valuable for the investigation of such easily analyzed samples as cold or warm aerodynamic jets, but was of limited potential in low pressure gases, fluorescent samples or in luminous reactive media.
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Taran, J.P. (1982). Coherent Anti-Stokes Raman Scattering. In: Kiefer, W., Long, D.A. (eds) Non-Linear Raman Spectroscopy and Its Chemical Aplications. NATO Advanced Study Institutes Series, vol 93. Springer, Dordrecht. https://doi.org/10.1007/978-94-009-7912-3_14
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DOI: https://doi.org/10.1007/978-94-009-7912-3_14
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