Skip to main content

Part of the book series: NATO Advanced Study Institutes Series ((ASIC,volume 93))

Abstract

The possibility of carrying out temperature and concentration measurements in gases by a Raman spectroscopy analysis was suggested and demonstrated about a decade ago. Following some early publications on this subject [1,2], a massive effort was undertaken in order to evaluate the potential of spontaneous Raman scattering in the important areas of atmospheric sounding and combustion diagnostics. In these experiments, the concentrations of the molecular species are deduced from the intensities of their respective Raman bands and the temperature is obtained from the contour of any one of these bands. Detailed accounts of early experimental work can be found, among other publications, in several Project SQUID and AIAA workshop proceedings [3–5]. Important instrumental developments were accomplished, with improved collection efficiencies and signal to noise ratio enhancement. The fields of applications were rapidly delineated and it appeared that spontaneous Raman scattering could prove valuable for the investigation of such easily analyzed samples as cold or warm aerodynamic jets, but was of limited potential in low pressure gases, fluorescent samples or in luminous reactive media.

This is a preview of subscription content, log in via an institution to check access.

Access this chapter

Chapter
USD 29.95
Price excludes VAT (USA)
  • Available as PDF
  • Read on any device
  • Instant download
  • Own it forever
eBook
USD 169.00
Price excludes VAT (USA)
  • Available as PDF
  • Read on any device
  • Instant download
  • Own it forever
Softcover Book
USD 219.99
Price excludes VAT (USA)
  • Compact, lightweight edition
  • Dispatched in 3 to 5 business days
  • Free shipping worldwide - see info
Hardcover Book
USD 219.99
Price excludes VAT (USA)
  • Durable hardcover edition
  • Dispatched in 3 to 5 business days
  • Free shipping worldwide - see info

Tax calculation will be finalised at checkout

Purchases are for personal use only

Institutional subscriptions

Preview

Unable to display preview. Download preview PDF.

Unable to display preview. Download preview PDF.

References

  1. Widhopf, G.F. and Lederman, S., AIAA J., 9, 309 (1971).

    Article  CAS  Google Scholar 

  2. Lapp, M., Goldman, L.M. and Penney, C.M., Science, 175, 1112 (1972).

    Article  CAS  Google Scholar 

  3. “Laser Raman Gas Diagnostics”, Proceedings of the Project SQUID Laser Baman Workshop on the Measurement of Gas Properties, May 10–11, 1973, Schenectady, edited by M. Lapp and C.M. Penney Plenum Press, New York, London (1974).

    Google Scholar 

  4. Proceedings of Project SQUID Workshop on Combustion Measurements in Jet Propulsion Systems, Edited by B. Goulard, Purdue University, Lafayette, Indiana (1975).

    Google Scholar 

  5. “Experimental Diagnostics in Gas Phase Combustion Systems”, Progress in Astronautics and Aeronautics, Vol. 53, Edited by B.T. Zinn, Martin Summerfield Series Editor (1977).

    Google Scholar 

  6. Régnier, P.R. and Taran, J.P.E., Appl. Phys. Letters, 23, 240, (1973).

    Article  Google Scholar 

  7. Terhune, R.W., Bull. Amer. Phys. Soc., 8, 359 (1963).

    Google Scholar 

  8. Maker, P.D. and Terhune R.W., Phys. Rev., 137, A801 (1965).

    Article  CAS  Google Scholar 

  9. Yablonovitch, E., Bloembergen, N., and Wynne, J.J., Phys. Rev., B3, 2060 (1971).

    Article  Google Scholar 

  10. Akhamanov, S.A., Dmitriev, V.G., Kovrigin, A.I., Koroteev, N.I., Tunkin, V.G. and Kholodnykh, A.I., JETP Letters, 15425 (1972).

    Google Scholar 

  11. Levenson, M.D. , Flytzanis, C. and Bloembergen, N. , Phys. Rev., 6, B3962 (1972).

    CAS  Google Scholar 

  12. Rado, W.G., Appl. Phys. Letters, 11, 123 (1967).

    CAS  Google Scholar 

  13. Hauchecorne, G., Kerhervé, F., and Mayer G., J. de Physique, 32, 47 (1971).

    Article  CAS  Google Scholar 

  14. De Martini, F., Giuliani, G.P. and Santamato, E., Optics Comm., 5, 126 (1972).

    Article  Google Scholar 

  15. Fiutak, J., and Van Kranendonk, J., Can. J. Phys. 40, 1085 (1962).

    Article  CAS  Google Scholar 

  16. Omont, A., Smith, E.W. and Cooper, J., The Astroph. J., 175, 185 (1972).

    Article  Google Scholar 

  17. Druet, S., Attal, B., Gustafson, T.K. and Taran, J.P.E., Phys. Rev. A18, 1529 (1978).

    CAS  Google Scholar 

  18. Yee, S.I., Gustafson, T.K., Druet, S.A.J, and Taran, J.P.E., Opt. Commun. 23, 1 (1977).

    Article  Google Scholar 

  19. Yee, S.Y. and Gustafson, T.K., Phys. Rev. A18, 1597 (1978).

    Article  CAS  Google Scholar 

  20. Druet, S.A.J, and Taran, J.P.E., “Coherent anti-Stokes Raman Spectroscopy”, in Chemical and Biochemical Applications of Lasers, vol. Edited by C.B. Moore (Academic Press, New York) (1979).

    Google Scholar 

  21. Bordé, C.J., Hall, J.L., Kunasz, C.V. and Hummer, D.G., Phys. Rev. A14, 236(1976).

    Article  Google Scholar 

  22. Bordé, J. and Bordé, C.J., J. Mol. Spectrosc. 78, 3530 (1979).

    Article  Google Scholar 

  23. Druet, S.A.J., Taran, J.P.E. and Bordé, C.J., J. de Physique, 40, 819, (1979), addendum, ibidem, 41, 183 (1980).

    Article  CAS  Google Scholar 

  24. Druet, S.A.J., Taran, J.P.E. and Bordé, C.J., J. de Physique, 40, 819, (1979), addendum, ibidem, 41, 183 (1980).

    CAS  Google Scholar 

  25. Druet, S.A.J, and Taran, J.P.E., Progress in Quant. Elec. 7, 1 (1981).

    Article  CAS  Google Scholar 

  26. Feynman, R.P., Quantum Electrodynamics, Benjamin, New York (1962).

    Google Scholar 

  27. Ward, J.F., Rev. Mod. Phys. 37, 1 (1965).

    Article  Google Scholar 

  28. Yariv, A., IEEE J. Quant. Elect. QE13, 943 (1977).

    Article  Google Scholar 

  29. Hanna, D.C., Cotter, D., and Yuratich, M, M., “Non linear Optics of Free Atoms and Molecules”, Edited by D.L. McAdam, Springer Series in Optical Sciences, Vol. 17, Springer Verlag, Berlin, Heidelberg, New York (1979).

    Google Scholar 

  30. Eesley, G.L., J.Q.S.R.T., 22, 507 (1979).

    Google Scholar 

  31. Bloembergen, N., Lotem, H., and Lynch, R.T., Indian J. Pure Appl. Phys. 16, 151 (1978).

    CAS  Google Scholar 

  32. Prior, Y., Bogdan, A.R., Dagenais, M. and Bloembergen, N. Phys. Rev. Letters, 46, 111 (1981).

    Article  CAS  Google Scholar 

  33. Bogdan A.R., Prior, Y. and Bloembergen, N., Opt. Letters, 6, 82 (1981).

    CAS  Google Scholar 

  34. Bloembergen, N., Bogdan, A.R. and Downer, M.W. in Laser Spectroscopy V (McKellar, Oka and Stoicheff, ed.) Springer Verlag, Berlin, Heidelberg, New York (1981).

    Google Scholar 

  35. Carreira, L.A., Gross, L.P. and Malloy, T.B., J. Chem. Phys. 69, 855 (1978).

    Article  CAS  Google Scholar 

  36. Grynberg, M., J. Phys. B. Atom Mol. Phys. 14, 2089 (1981)

    Article  CAS  Google Scholar 

  37. Eckbreth, A.C. Appl., Phys. Letters, 32, 421 (1978).

    Article  CAS  Google Scholar 

  38. Rahn, L.A., Zych, L.J., and Mattern, P.L., Opt. Comm. 30, 249, (1979).

    Article  CAS  Google Scholar 

  39. Roh, W.B., Schreiber, P.W. and Taran, J.P.E., Appl. Phys. Letters, 29, 174 (1976).

    Article  CAS  Google Scholar 

  40. Attal, B., Péalat, M. and Taran J.P.E., J. Energy 4, 135 (1980).

    Article  CAS  Google Scholar 

  41. Song, J.J., Eesley, G.L. and Levenson, M.D., Appl. Phys. Letters, 29, 567 (1976).

    Article  CAS  Google Scholar 

  42. Régnier, P.R. and Taran, J.P.E., Appl. Phys. Letters, 23, 240, (1973).

    Article  Google Scholar 

  43. Péalat, M., Taran, J.P.E., Taillet, J., Bacal M., and Bruneteau, A.M., J. Appl. Phys. 52, 2687 (1981).

    Article  Google Scholar 

  44. Bacal, M. and Hamilton, G.W., Phys. Rev. Letters 42, 1538 (1979).

    CAS  Google Scholar 

  45. Nibler, J.W., Shaub, W.M. , McDonald, J.R. and Harvey, A.B., “Coherent Anti-Stokes Raman Spectroscopy” in Vibrational Spectra and Structure (Durig J.R. , Editor), Vol. 6, Elsevier, Amsterdam, New York, (1977).

    Google Scholar 

  46. Müller-Dethlefs, K. , Péalat, M. and Taran, J.P.E., Ber. Bunsenges, Phys. Chem. 85, 803 (1981).

    Google Scholar 

  47. Flossdorf, J., Jost, W. and Wagner, H. Cg., Ber. Bunsenges, Phys. Chem. 78, 378 (1974).

    CAS  Google Scholar 

  48. Bouchardy, P., Gicquel, P., P00E9alat, M. and Taran, J.P.E., To be published.

    Google Scholar 

  49. Bédué, J., Gastebois, P., Bailly, R., Péalat, M, and Taran, J.P.E. To be published.

    Google Scholar 

  50. Gross, K.P., Guthals, D.M. and Nibler, J.W., J. Chem. Phys. 70., 4673 (1979).

    Article  CAS  Google Scholar 

  51. Hetherington III, W.M. , Korenowski, G.M., and Eisenthal, K.B., Chem. Phys. Letters 77, 275 (1981)

    Article  CAS  Google Scholar 

  52. Guthals, D.M., Gross, K.P., and Nibler, J.W., J. Chem. Phys. 70, 2393 (1979).

    CAS  Google Scholar 

  53. McIlwain, M.E. and Hindman, J.C., J. Chem. Phys. 73, 68 (1980).

    Article  CAS  Google Scholar 

  54. Beckman, A., Fietz, H., Baierl, P., and Kiefer, W., Chem. Phys. Letters 86, 140 (1982).

    Article  CAS  Google Scholar 

  55. Attal, B., Müller-Dethlefs, K., Débarre, D., and Taran, J.P.E., to be published.

    Google Scholar 

  56. Luc, P., Amiot, C., Debarre, D., Attal, B., Müller-Dethlefs, K., “New Analysis of the C2Swan system”, to be published.

    Google Scholar 

  57. Phillips, J.G., and Davis, S.P., The Berkeley analysis of molecular spectra, Vol. 2 (a), University of California Press, (1968).

    Google Scholar 

  58. Hänsch, Th. and Toschek, P., Z. Phys. 236, 213 (1970).

    Article  Google Scholar 

Download references

Author information

Authors and Affiliations

Authors

Editor information

Editors and Affiliations

Rights and permissions

Reprints and permissions

Copyright information

© 1982 D. Reidel Publishing Company

About this paper

Cite this paper

Taran, J.P. (1982). Coherent Anti-Stokes Raman Scattering. In: Kiefer, W., Long, D.A. (eds) Non-Linear Raman Spectroscopy and Its Chemical Aplications. NATO Advanced Study Institutes Series, vol 93. Springer, Dordrecht. https://doi.org/10.1007/978-94-009-7912-3_14

Download citation

  • DOI: https://doi.org/10.1007/978-94-009-7912-3_14

  • Publisher Name: Springer, Dordrecht

  • Print ISBN: 978-94-009-7914-7

  • Online ISBN: 978-94-009-7912-3

  • eBook Packages: Springer Book Archive

Publish with us

Policies and ethics