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Endohedral Fullerene Complexes and In-Out Isomerism in Perhydrogenated Fullerenes

Why the Carbon Cages Cannot Be Used as the Hydrogen Containers?

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The Mathematics and Topology of Fullerenes

Part of the book series: Carbon Materials: Chemistry and Physics ((CMCP,volume 4))

Abstract

As shown by our group (Dodziuk and Nowinksi, 1998; Dodziuk et al., manuscript in preparation, 2011) endohedral fullerene complexes are objects of nontrivial topology. An insertion of a guest (atom, ion, or molecule(s)) inside the fullerene cage usually changes properties of both host and guest. Due to their size and complexity, predicting properties of the complexes is a difficult task. For instance, the numbers of endohedral hydrogen molecules in C60 and C70 have only recently been correctly determined by calculations in agreement with experimental results on the existence of only one hydrogen molecule inside the former molecule and one or two of them (in 96:4 proportion) in the C70 cage (Korona et al. 2009). Fullerenes are studied because of their exciting structure and prospects of applications. However, their use for hydrogen storage seems highly improbable.

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  1. Institute of Physical Chemistry, Polish Academy of Sciences, Kasprzaka 44/52, 01-224, Warsaw, Poland

    Helena Dodziuk

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  1. , Dept. of Materials Science, Tor Vergata University, Rome, Italy

    Franco Cataldo

  2. Faculty of Science, University of Split, Nikole Tesle 12, Split, HR–21000, Croatia

    Ante Graovac

  3. Actinium Chemical Research, Via Casilina 1626-A, Rome, 00133, Italy

    Ottorino Ori

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Dodziuk, H. (2011). Endohedral Fullerene Complexes and In-Out Isomerism in Perhydrogenated Fullerenes. In: Cataldo, F., Graovac, A., Ori, O. (eds) The Mathematics and Topology of Fullerenes. Carbon Materials: Chemistry and Physics, vol 4. Springer, Dordrecht. https://doi.org/10.1007/978-94-007-0221-9_7

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