Abstract
In the previous Chapters we analyzed in some detail the ‘forward’ progression of the theoretical treatments that allow one to obtain dynamic observables from first principles. This meant that we had to define an interaction Hamiltonian between colliding partners, compute the corresponding potential forms at various levels of accuracy and then go on to evaluate detailed, state-to-state total and differential cross sections that involved transitions between levels of the rotational and vibrational structures of the colliding partners in their lowest electronic states, usually closed- shell configurations.
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Gianturco, F.A. (1979). Rotovibrational Relaxation Models in Simple Gases. In: The Transfer of Molecular Energies by Collision: Recent Quantum Treatments. Lecture Notes in Chemistry, vol 11. Springer, Berlin, Heidelberg. https://doi.org/10.1007/978-3-642-93122-2_7
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DOI: https://doi.org/10.1007/978-3-642-93122-2_7
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