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Probing Molecular Photoexcited Dynamics by Soft X-Rays

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Ultrafast Dynamics Driven by Intense Light Pulses

Part of the book series: Springer Series on Atomic, Optical, and Plasma Physics ((SSAOPP,volume 86))

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Abstract

This chapter presents a short introduction into probing photoexcited dynamics of isolated molecules by ultrashort x-ray pulses. It describes the basic concepts of electronic and nuclear dynamics in a molecule after optical excitation and shows basic concepts like element and site specific probing associated with x-rays. It discusses ultrafast x-ray sources for molecular spectroscopy and presents some of the very first gas phase molecular dynamics results that this young field has produced.

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Acknowledgments

I would like to acknowledge all my colleagues in the PULSE Institute and at the LCLS for many discussions and fruitful collaborations. I would like to acknowledge especially the whole team of colleagues in the LCLS thymine experiment: B.K. McFarland, J.P. Farrell, S. Miyabe, F. Tarantelli, A. Aguilar, N. Berrah, C. Bostedt, J.D. Bozek, P.H. Bucksbaum, J.C. Castagna, R.N. Coffee, J.P. Cryan, L. Fang, R. Feifel, K.J. Gaffney, J.M. Glownia, T.J. Martinez, M. Mucke, B. Murphy, A. Natan, T. Osipov , V.S. Petrović, S. Schorb, Th. Schultz, L.S. Spector, M. Swiggers, I. Tenney, S. Wang, J.L. White, and W. White. This work was supported by the AMOS program within the Chemical Sciences, Geosciences, and Biosciences Division of the Office of Basic Energy Sciences, Office of Science, U.S. Department of Energy. I acknowledge funding via the Office of Science Early Career Research Program through the Office of Basic Energy Sciences, U.S. Department of Energy.

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    Markus Gühr

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    Markus Kitzler

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Gühr, M. (2016). Probing Molecular Photoexcited Dynamics by Soft X-Rays. In: Kitzler, M., Gräfe, S. (eds) Ultrafast Dynamics Driven by Intense Light Pulses. Springer Series on Atomic, Optical, and Plasma Physics, vol 86. Springer, Cham. https://doi.org/10.1007/978-3-319-20173-3_14

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