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Nuclear Data for the Thorium Fuel Cycle and the Transmutation of Nuclear Waste

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Thorium Energy for the World

Abstract

Neutron-induced reaction cross sections play an important role in a wide variety of research fields, ranging from stellar nucleosynthesis, the investigation of nuclear level density studies, to applications of nuclear technology, including the transmutation of nuclear waste, accelerator-driven systems, and nuclear fuel cycle investigations. Simulations of nuclear technology applications largely rely on evaluated nuclear data libraries. These libraries are based both on experimental data and theoretical models. An outline of experimental nuclear data activities at CERN’s neutron time-of-flight facility, n_TOF, will be presented.

F. Gunsing presented this paper at the Thorium Energy Conference 2013 (ThEC13)

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References

  1. Koning, A.J., Bauge, E., Dean, C.J., et al.: Status of the JEFF nuclear data library. J. Korean Phys. Soc. 59(2), 1057–1062 (2011)

    Google Scholar 

  2. Chadwick, M.B., Herman, M., Oblozinsky, P., et al.: ENDF/B-VII.1 Nuclear data for science and technology: Cross sections, covariances, fission product yields and decay data. Nucl. Data Sheets 112(12), 2887–2996 (2011)

    Article  ADS  Google Scholar 

  3. Shibata, K.: Nuclear databases for science and technology. J. Nucl. Sci. Technol. 50(5), 449–469 (2013)

    Article  Google Scholar 

  4. Qaim, S.M.: New trends in nuclear data research for medical radionuclide production. Radiochim. Acta 101(8), 473–480 (2013)

    Google Scholar 

  5. Aliberti, G., Palmiotti, G., Salvatores, M., et al.: Impact of nuclear data uncertainties on transmutation of actinicles in accelerator-driven assemblies. Nucl. Sci. Eng. 146(1), 13–50 (2004)

    Article  Google Scholar 

  6. Nuttin, A., Heuer, D., Billebaud, A., et al.: Potential of thorium molten salt reactors: Detailed calculations and concept evolution with a view to large scale energy production. Prog. Nucl. Energy 46(1), 77–99 (2005)

    Article  Google Scholar 

  7. Nuttin, A., Guillemin, P., Bidaud, A., et al.: Comparative analysis of high conversion achievable in thorium-fueled slightly modified CANDU and PWR reactors. Ann. Nucl. Energy 40(1), 171–189 (2012)

    Article  Google Scholar 

  8. von Egidy, T., Bucurescu, D.: Systematics of nuclear level density parameters. Phys. Rev. C 73(4), 049901 (2006)

    Article  ADS  Google Scholar 

  9. Weidenmuller, H.A., Mitchell, G.E.: Random matrices and chaos in nuclear physics: Nuclear structure. Rev. Modern Phys. 81(2), 539–589 (2009)

    Article  ADS  Google Scholar 

  10. Woosley, S.E., Heger, A., Rauscher, T., et al.: Nuclear data needs for the study of nucleosynthesis in massive stars. Nucl. Phys. A 718, 3C–12C (2003)

    Article  ADS  Google Scholar 

  11. Kappeler, F., Gallino, R., Bisterzo, S., et al.: The s process: Nuclear physics, stellar models, and observations. Rev. Modern Phys. 83(1), 157–193 (2011)

    Article  ADS  Google Scholar 

  12. Rauscher, T.: Challenges in nucleosynthesis of trans-iron elements. AIP Adv. 4(4), 041012 (2014)

    Article  ADS  Google Scholar 

  13. Otuka, N., Dunaeva, S., Dupont, E., et al.: The role of the nuclear reaction data centres in experimental nuclear data knowledge sharing. J. Korean Phys. Soc. 59(2), 1292–1297 (2011)

    Google Scholar 

  14. Wagner, W., Gröschel, F., Thomsen, K., Heyck, H.: MEGAPIE at SINQ The first liquid metal target driven by a megawatt class proton beam. J. Nucl. Mater. 377, 12 (2008)

    Article  ADS  Google Scholar 

  15. Rubbia, C., et al.: A high resolution spallation driven facility at the CERN-PS to measure neutron cross-sections in the interval from 1 eV to 250 MeV. Tech. rep. CERN/LHC/98-02 (1998)

    Google Scholar 

  16. Guerrero, C., Tsinganis, A., Berthoumieux, E., et al.: Performance of the neutron time-of-fight facility n TOF at CERN. Eur. Phys. J. A 49(2), 27 (2013)

    Article  ADS  Google Scholar 

  17. Aerts, G., Abbondanno, U., Alvarez, H., et al.: Neutron capture cross section of 232Th measured at the n TOF facility at CERN in the unresolved resonance region up to 1 MeV. Phys. Rev. C 73(5), 054610 (2006)

    Article  ADS  Google Scholar 

  18. Gunsing, F., Berthoumieux, E., Aerts, G., et al.: Measurement of resolved resonances of 232Th(n, γ) at the n TOF facility at CERN. Phys. Rev. C 86(1), 019902 (2012)

    Article  ADS  Google Scholar 

  19. Massimi, C., Koehler, P., Bisterzo, S., et al.: Resonance neutron-capture cross sections of stable magnesium isotopes and their astrophysical implications. Phys. Rev. C 85(4), 044615 (2012)

    Article  ADS  Google Scholar 

  20. Tagliente, G., Fujii, K., Milazzo, P.M., et al.: Neutron capture cross section of 90Zr: Bottleneck in the s-process reaction flow. Phys. Rev. C 77(3), 035802 (2008)

    Article  ADS  Google Scholar 

  21. Tagliente, G., Milazzo, P.M., Fujii, K., et al.: Experimental study of the 91Zr(n, γ) reaction up to 26 keV. Phys. Rev. C 78(4), 045804 (2008)

    Article  ADS  Google Scholar 

  22. Tagliente, G., Milazzo, P.M., Fujii, K., et al.: The 92Zr(n, γ) reaction and its implications for stellar nucleosynthesis. Phys. Rev. C 81(5), 055801 (2010)

    Article  ADS  Google Scholar 

  23. Tagliente, G., Milazzo, P.M., Fujii, K., et al.: Neutron capture on 94Zr: Resonance parameters and Maxwellian-averaged cross sections. Phys. Rev. C 84(1), 015801 (2011)

    Article  ADS  Google Scholar 

  24. Tagliente, G., Milazzo, P.M., Fujii, K., et al.: 96Zr(n, γ) measurement at the n_TOF facility at CERN. Phys. Rev. C 84(5), 055802 (2011)

    Article  ADS  Google Scholar 

  25. Terlizzi, R., Abbondanno, U., Aerts, G., et al.: The 139La(n, γ) cross section: Key for the onset of the s-process. Phys. Rev. C 75(3), 035807 (2007)

    Article  ADS  Google Scholar 

  26. Abbondanno, U., Aerts, G., Alvarez-Velarde, F., et al.: Neutron capture cross section measurement of 151Sm at the CERN neutron time of light facility (n_TOF). Phys. Rev. Lett. 93(16), 161103 (2004)

    Article  ADS  Google Scholar 

  27. Marrone, S., Abbondanno, U., Aerts, G., et al.: Measurement of the 151Sm(n, γ)152Sm cross section at n_TOFNucl. Phys. A 758, 533C (2005)

    Article  ADS  Google Scholar 

  28. Marrone, S., Abbondanno, U., Aerts, G., et al.: Measurement of the 151Sm(n, γ) cross section from 0.6 eV to 1 MeV via the neutron time-of-light technique at the CERN n_TOF facility. Phys. Rev. C 73(3), 034604 (2006)

    Article  ADS  Google Scholar 

  29. Fujii, K., Mosconi, M., Mengoni, A., et al.: Neutron physics of the Re/Os clock. III. Resonance analyses and stellar (n, γ) cross sections of 186Os, 187Os, 188Os. Phys. Rev. C 82(1), 015804 (2010)

    Article  ADS  Google Scholar 

  30. Mosconi, M., Fujii, K., Mengoni, A., et al.: Neutron physics of the Re/Os clock. I. Measurement of the (n, γ) cross sections of Os-186,Os-187,Os-188 at the CERN n_TOF facility. Phys. Rev. C 82(1), 015802 (2010)

    Article  ADS  Google Scholar 

  31. Domingo-Pardo, C., Abbondanno, U., Aerts, G., et al.: Measurement of the neutron capture cross section of the s-only isotope 204Pb from 1 eV to 440 keV. Phys. Rev. C 75(1), 015806 (2007)

    Article  ADS  Google Scholar 

  32. Domingo-Pardo, C., Abbondanno, U., Aerts, G., et al.: Measurement of the radiative neutron capture cross section of 206Pb and its astrophysical implications. Phys. Rev. C 76(4), 045805 (2007)

    Article  ADS  Google Scholar 

  33. Domingo-Pardo, C., Abbondanno, U., Aerts, G., et al.: The measurement of the 206Pb(n, γ) cross section and stellar implications. J. Phys. G: Nucl. Part. Phys. 35(1), 014020 (2008)

    Article  ADS  Google Scholar 

  34. Domingo-Pardo, C., Abbondanno, U., Aerts, G., et al.: Resonance capture cross section of 207Pb. Phys. Rev. C 74(5), 055802 (2006)

    Article  ADS  Google Scholar 

  35. Domingo-Pardo, C., Abbondanno, U., Aerts, G., et al.: New measurement of neutron capture resonances in 209Bi. Phys. Rev. C 74(2), 025807 (2006)

    Article  ADS  Google Scholar 

  36. Guerrero, C., Cano-Ott, D., Mendoza, E., et al.: Measurement and resonance analysis of the 237Np neutron capture cross section. Phys. Rev. C 85(4), 044616 (2012)

    Article  ADS  Google Scholar 

  37. Mendoza, E., Cano-Ott, D., Guerrero, C., et al.: \Measurement and analysis of the 243Am neutron capture cross section at the n_TOF facility at CERN. Phys. Rev. C 90(3), 034608 (2014)

    Article  ADS  Google Scholar 

  38. Calviani, M., Praena, J., Abbondanno, U., et al.: High-accuracy 233U(n,f) cross-section measurement at the white-neutron source n_TOF from near-thermal to 1 MeV neutron energy. Phys. Rev. C 80(4), 044604 (2009)

    Article  ADS  Google Scholar 

  39. Belloni, F., Calviani, M., Colonna, N., et al.: Neutron-induced fission cross-section of 233U in the energy range 0.5 E-n 20 MeV. Eur. Phys. J. A 47(1), 2 (2011)

    Article  ADS  Google Scholar 

  40. Karadimos, D., Vlastou, R., Ioannidis, K., et al.: Neutron-induced fission cross section of 234U measured at the CERN n_TOF facility. Phys. Rev. C 89(4), 044606 (2014)

    Article  ADS  Google Scholar 

  41. Sarmento, R., Calviani, M., Praena, J., et al.: Measurement of the 236U(n,f) cross section from 170 meV to 2 MeV at the CERN n_TOF facility. Phys. Rev. C 84(4), 044618 (2011)

    Article  ADS  Google Scholar 

  42. Belloni, F., Calviani, M., Colonna, N., et al.: Measurement of the neutron-induced fission cross-section of 241Am at the time-of-flight facility n_TOF. Eur. Phys. J. A 49(1), 2 (2013)

    Article  ADS  Google Scholar 

  43. Belloni, F., Calviani, M., Colonna, N., et al.: Measurement of the neutron-induced fission cross-section of 243Am relative to 235U from 0.5 to 20 MeV. Eur. Phys. J. A 47(12), 160 (2011)

    Article  ADS  Google Scholar 

  44. Calviani, M., Meaze, M.H., Colonna, N., et al.: Neutron-induced fission cross section of 245Cm: New results from data taken at the time-of-light facility n_TOF. Phys. Rev. C 85(3), 034616 (2012)

    Article  ADS  Google Scholar 

  45. Paradela, C., Tassan-Got, L., Audouin, L., et al.: Neutron-induced fission cross section of 234U and 237Np measured at the CERN Neutron Time-of-Flight (n_TOF) facility. Phys. Rev. C 82(3), 034601 (2010)

    Article  ADS  Google Scholar 

  46. Leal-Cidoncha, E., Durn, I., Paradela, C., et al.: Study of 234U(n,f) Resonances Measured at the {CERN} n_TOF Facility. Nucl. Data Sheets 119, 42 (2014)

    Article  ADS  Google Scholar 

  47. Tarrio, D., Tassan-Got, L., Audouin, L., et al.: Neutron-induced fission cross section of natPb and 209Bi from threshold to 1 GeV: An improved parametrization. Phys. Rev. C 83(4), 044620 (2011)

    Article  ADS  Google Scholar 

  48. Tarrio, D., Leong, L.S., Audouin, L., et al.: Measurement of the angular distribution of fission fragments using a PPAC assembly at CERN n_TOF. Nucl. Instr. Methods in Phys. Res. Section A–Accelerators Spectrometers Detectors and Associated Equipment 743, 79 (2014)

    Google Scholar 

  49. Weiss, C., Guerrero, C., Griesmayer, E., et al.: The (n, α) Reaction in the s-process branching point 59Ni". Nucl. Data Sheets 120, 208 (2014)

    Article  ADS  Google Scholar 

  50. Massimi, C., Koehler, P., Mingrone, F., et al.: New measurement of the 25Mg(n, γ) reaction cross section. Nucl. Data Sheets 119, 110 (2014)

    Article  ADS  Google Scholar 

  51. Giubrone, G., Domingo-Pardo, C., Tan, J., et al.: Measurement of the 54, 57Fe(n, γ) cross section in the resolved resonance region at {CERN} n_TOF. Nucl. Data Sheets 119, 117 (2014)

    Article  ADS  Google Scholar 

  52. Zugec, P., Barbagallo, M., Colonna, N., et al.: Experimental neutron capture data of 58Ni from the CERN n_TOF facility. Phys. Rev. C 89(1), 14605 (2014) mn

    Google Scholar 

  53. Lederer, C., Massimi, C., Berthoumieux, E., et al.: 62Ni(n, γ) and 63Ni(n, γ) cross sections measured at the n_TOF facility at CERN. Phys. Rev. C 89(2), 025810 (2014)

    Article  ADS  Google Scholar 

  54. Lederer, C., Massimi, C., Altstadt, S., et al.: Neutron capture cross section of unstable 63Ni: Implications for stellar nucleosynthesis. Phys. Rev. Lett. 110(2), 022501 (2013)

    Article  ADS  Google Scholar 

  55. Gunsing, F., Fraval, K., Mathelie, M., et al.: Spin measurements of n + 87Sr for level density studies. Nucl. Data Sheets 119, 132–136 (2014)

    Article  ADS  Google Scholar 

  56. Tagliente, G., Milazzo, P.M., Fujii, K., et al.: The 93Zr(n, γ) reaction up to 8 keV neutron energy. Phys. Rev. C 87(1), 014622 (2013)

    Article  ADS  Google Scholar 

  57. Massimi, C., Domingo-Pardo, C., Vannini, G., et al.: 197Au(n, γ) cross section in the resonance region. Phys. Rev. C 81(4), 044616 (2010)

    Article  ADS  Google Scholar 

  58. Lederer, C., Colonna, N., Domingo-Pardo, C., et al.: 197Au(n, γ) cross section in the unresolved resonance region. Phys. Rev. C 83(3), 034608 (2011)

    Article  ADS  Google Scholar 

  59. Balibrea, J., Mendoza, E., Cano-Ott, D., et al.: Measurement of the neutron capture cross section of the fissile isotope 235U with the {CERN} n_TOF total absorption calorimeter and a fission tagging based on micromegas detectors. Nucl. Data Sheets 119, 10 (2014)

    Article  ADS  Google Scholar 

  60. Barbagallo, M., Colonna, N., Vermeulen, M., et al.: Capture cross section of 236U: the n_TOF results. Nucl. Data Sheets 119, 45–47 (2014)

    Article  ADS  Google Scholar 

  61. Mingrone, F., Massimi, C., Altstadt, S., et al.: Measurement of the 238U radiative capture cross section with {C6D6} at the {CERN} n_TOF facility. Nucl. Data Sheets 119, 18–21 (2014)

    Article  ADS  Google Scholar 

  62. Wright, T., Guerrero, C., Billowes, J., et al.: High-precision measurement of the 238U(n,γ) cross section with the rotal absorption calorimeter (TAC) at n_TOF, {CERN}. Nucl. Data Sheets 119, 26–30 (2014)

    Article  ADS  Google Scholar 

  63. Fraval, K., Gunsing, F., Altstadt, S., et al.: Measurement and analysis of the 241Am(n,γ) cross section with liquid scintillator detectors using time-of-light spectroscopy at the n_TOF facility at CERN. Phys. Rev. C 89(4), 044609 (2014)

    Article  ADS  Google Scholar 

  64. Mendoza, E., Cano-Ott, D., Guerrero, C., et al.: Measurement of the 241Am and the 243Am neutron capture cross sections at the n_TOF facility at {CERN}. Nucl. Data Sheets 119, 65 (2014)

    Article  ADS  Google Scholar 

  65. Tsinganis, A., Berthoumieux, E., Guerrero, C., et al.: Measurement of the 242Pu(n,f) cross section at the {CERN} n_TOF facility. Nucl. Data Sheets 119, 58 (2014)

    Article  ADS  Google Scholar 

  66. Zugec, P., Colonna, N., Bosnar, D., et al.: Measurement of the 12C(n,p)12B cross section at n_TOF at CERN by in-beam activation analysis. Phys. Rev. C 90(2), 021601 (2014)

    Article  ADS  Google Scholar 

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Gunsing, F. et al. (2016). Nuclear Data for the Thorium Fuel Cycle and the Transmutation of Nuclear Waste. In: Revol, JP., Bourquin, M., Kadi, Y., Lillestol, E., de Mestral, JC., Samec, K. (eds) Thorium Energy for the World. Springer, Cham. https://doi.org/10.1007/978-3-319-26542-1_32

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