Abstract
We have studied characteristics of stimulated light scattering in synthetic opal crystals made up of silica spheres. This type of light scattering results from interaction between pulsed laser radiation and dielectric nanoparticles, such as silica (SiO2) spheres in the structure of synthetic opal. The Stokes shift in the scattered radiation spectrum was 0.4–1.0 cm−1. The Stokes shift was determined as a function of scattering geometry, sphere diameter, sample temperature, and the type of dielectric in the opal pores. The results are of interest for assessing the size of nanoparticles in spatially ordered inorganic structures.
Similar content being viewed by others
References
Montagna, M., Brillouin and Raman scattering from the acoustic vibrations of spherical particles with a size comparable to the wavelength of the light, Phys. Rev. B: Condens. Matter Mater. Phys., 2008, vol. 77, paper 045 418.
Duval, E., Boukenter, A., and Champagnon, B., Vibration eigenmodes and size of microcrystallites in glass: observation by very-low-frequency Raman scattering, Phys. Rev. Lett., 1986, vol. 56, pp. 2052–2055.
Saviot, L., Combe, N., and Mlayah, A., Number of observable features in the acoustic Raman spectra of nanocrystals, Phys. Rev. B: Condens. Matter Mater. Phys., 2012, vol. 85, paper 075 405.
Li, Y., Lim, H.S., Ng, S.C., and Kuok, M.H., Selection rules for Brillouin light scattering from eigenvibrations of a sphere, Chem. Phys. Lett., 2007, vol. 440, pp. 321–323.
Ivanda, M., Furić, K., Musićl, S., Ristić, M., Gotić, M., Ristić, D., and Tonejc, A.M., Low wavenumber Raman scattering of nanoparticles and nanocomposite materials, J. Raman Spectrosc., 2007, vol. 38, no. 6, pp. 647–659.
Trofimov, V.A., Fedotov, M.V., Volkov, A.G., Tcherniega, N.V., Savranskii, V.V., and Lan, S., Computer simulation and observation of anomalous light emission from nonlinear photonic crystal with various geometry of its elements, Laser Phys., 2010, vol. 20, no. 5, pp. 1137–1143.
Zaporozhchenko, R.G., Kilin, S.Ya., and Smirnov, A.G., Stimulated Raman scattering in a photonic crystal, Kvantovaya Elektron. (Moscow), 2000, vol. 30, pp. 997–1001.
Kuok, M.H., Lim, H.S., Ng, S.C., Liu, N.N., and Wang, Z.K., Brillouin study of the quantization of acoustic modes in nanospheres, Phys. Rev. Lett., 2003, vol. 90, paper 255 502.
Gorelik, V.S., Kudryavtseva, A.D., and Tcherniega, N.V., Stimulated light scattering in three-dimensional crystals, Kratk. Soobshch. Fiz., 2006, vol. 8, pp. 43–50.
Tareeva, M.V., Gorelik, V.S., Kudryavtseva, A.D., and Chernega, N.V., Spectral and energy characteristics of stimulated globular light scattering, Bull. Lebedev Phys. Inst., 2010, vol. 37 I, pp. 331–334.
Gorelik, V.S., Kudryavtseva, A.D., Tareeva, M.V., and Tcherniega, N.V., Generation of pulsating acoustic waves in opal photonic crystals, Vestn. Mos. Gos. Tekh. Uchilishcha im. N. E. Baumana, Ser. Estestv. Nauki, 2011, vol. 2, pp. 3–15.
Lamb, H., On the vibrations of an elastic sphere, Proc. London Math. Soc., 1882, vol. 13, p. 189.
Author information
Authors and Affiliations
Corresponding author
Additional information
Original Russian Text © V.S. Gorelik, A.D. Kudryavtseva, M.V. Tareeva, N.V. Tcherniega, 2014, published in Neorganicheskie Materialy, 2014, Vol. 50, No. 12, pp. 1314–1319.
Rights and permissions
About this article
Cite this article
Gorelik, V.S., Kudryavtseva, A.D., Tareeva, M.V. et al. Stimulated light scattering in synthetic opal filled with dielectrics. Inorg Mater 50, 1217–1221 (2014). https://doi.org/10.1134/S0020168514120073
Received:
Published:
Issue Date:
DOI: https://doi.org/10.1134/S0020168514120073