Skip to main content
Log in

Microrheology of a sticking transition

  • Article
  • Published:

From Nature Physics

View current issue Submit your manuscript

Abstract

The phenomenon of sticking of one object to another, which drastically reduces their relative motion, is ubiquitous in nature. We have studied the sticking process of a colloid, suspended in a fluid medium by an optical tweezer, to a rigid substrate. The evolution of the frictional coupling between the two as a function of their separation is detected by the diffusivity of the particle and also by its phase-sensitive response to an in-plane external oscillatory drive applied to the substrate. On contact, the coupling changes abruptly from viscous to elastic for a rigid silica particle, whereas it evolves slowly with time, similar to ageing in glassy systems, for a soft and deformable polystyrene particle. Depending on the relative strengths of the particle–substrate interaction, the tweezer potential and the external drive, three regimes of dynamics—stuck, ageing and non-stuck—are observed in the dynamical phase diagram.

This is a preview of subscription content, log in via an institution to check access.

Access this article

Price excludes VAT (USA)
Tax calculation will be finalised during checkout.

Instant access to the full article PDF.

Figure 1: Variation of MSD for the sticking transition.
Figure 2: Response of the trapped particle to an external oscillatory drive applied to the substrate.
Figure 3: Microrheological quantities in the ageing regime.
Figure 4: Rheological characterization of the stuck and non-stuck regimes.
Figure 5: Dynamical phase diagram of sticking.
Figure 6: Memory effect.

Similar content being viewed by others

References

  1. Liu, A. & Nagel, S.R. Nonlinear dynamics: Jamming is not just cool anymore. Nature 396, 21–22 (1998).

    Article  ADS  Google Scholar 

  2. Trappe, V., Prasad, V., Cipelletti, L., Segre, P. N. & Weitz, D. A. Jamming phase diagram for attractive particles. Nature 411, 772–775 (2001).

    Article  ADS  Google Scholar 

  3. Bhattacharya, S. & Higgins, M. J. Dynamics of a disordered flux line lattice. Phys. Rev. Lett. 70, 2617–2620 (1993).

    Article  ADS  Google Scholar 

  4. Giamarchi, T. & Bhattacharya, S. High Magnetic Fields: Applications in Condensed Matter Physics and Spectroscopy Vol. 595, 314–360 (Lecture Notes in Physics, Springer, 2002).

    Book  Google Scholar 

  5. Reif, F. Fundamentals of Statistical and Thermal Physics Ch. 15 (McGraw-Hill, 1985).

    Google Scholar 

  6. Faxen, H. Die bewegung einer starren kugel längs der achse eines mit zährer flüssigkeit gefüllten rohres. Arkiv. Mat. Astron. Fys 17, 1–28 (1923).

    MATH  Google Scholar 

  7. Lin, B., Yu, J. & Rice, S. Direct measurements of constrained Brownian motion of an isolated sphere between two walls. Phys. Rev. E 62, 3909–3919 (2000).

    Article  ADS  Google Scholar 

  8. Dufresne, E., Squires, T., Brenner, M. & Grier, D. Hydrodynamic coupling of two Brownian spheres to a planar surface. Phys. Rev. Lett. 85, 3317–3320 (2000).

    Article  ADS  Google Scholar 

  9. Leheny, R. L. & Nagel, S. R. Frequency-domain study of physical ageing in a simple liquid. Phy. Rev. B 57, 5154–5162 (1998).

    Article  ADS  Google Scholar 

  10. Behrens, S. H., Plewa, J. & Grier, D. G. Measuring a colloidal particle’s interaction with a flat surface under nonequilibrium conditions. Eur. Phys. J. E 10, 115–121 (2003).

    Article  Google Scholar 

  11. Ghosh, S., Sharma, P. & Bhattacharya, S. Surface modes of a sessile water drop: An optical tweezer based study. Rev. Sci. Instrum. 78, 115110.1–115110.6 (2007).

    Article  Google Scholar 

Download references

Acknowledgements

We thank P. Chaikin, D. Dhar, D. Grier, M. W. Kim, S. Nagel, D. Pine and G. V. Shivashankar for helpful discussions.

Author information

Authors and Affiliations

Authors

Corresponding author

Correspondence to Shankar Ghosh.

Supplementary information

Supplementary Information

Supplementary Informations (PDF 341 kb)

Rights and permissions

Reprints and permissions

About this article

Cite this article

Sharma, P., Ghosh, S. & Bhattacharya, S. Microrheology of a sticking transition. Nature Phys 4, 960–966 (2008). https://doi.org/10.1038/nphys1105

Download citation

  • Received:

  • Accepted:

  • Published:

  • Issue Date:

  • DOI: https://doi.org/10.1038/nphys1105

  • Springer Nature Limited

This article is cited by

Navigation