Skip to main content
Log in

Chemical Composition Change in TSP Due to Dust Storm at Gosan, Korea: Do the Concentrations of Anthropogenic Species Increase Due to Dust Storm?

  • Published:
Water, Air, and Soil Pollution Aims and scope Submit manuscript

Abstract

Aerosol composition change between dust storm and non-dust storm periods in spring is studied using the total suspended particle data measured at Gosan, a background area in Korea. The concentrations of eight inorganic ions and 12 elements were analyzed for the TSP samples collected from March 1992 to May 2006. Two-step statistical analyses were carried out for the data: F test and t test. The concentrations of anthropogenic ionic species showed increasing trend since 2003. The absolute concentrations of most anthropogenic species such as sulfate or nitrate increased (from 7.33 to 9.25 µg m−3 and from 2.04 to 4.84 µg m−3, respectively) during the dust storm period. However, the enrichment factors or normalized concentrations based on Al of most anthropogenic species decreased during dust storm period (factor of 0.1–0.5). It suggests that, in general, relative importance of anthropogenic species during dust storm would be not high.

This is a preview of subscription content, log in via an institution to check access.

Access this article

Price excludes VAT (USA)
Tax calculation will be finalised during checkout.

Instant access to the full article PDF.

Fig. 1
Fig. 2
Fig. 3
Fig. 4
Fig. 5
Fig. 6
Fig. 7
Fig. 8

Similar content being viewed by others

References

  • Akimoto, H., Ohara, T., Kurokawa, J., & Horii, N. (2006). Verification of energy consumption in China during 1996–2003 by using satellite observation data. Atmospheric Environment, 40, 7663–7667. doi:10.1016/j.atmosenv.2006.07.052.

    Article  CAS  Google Scholar 

  • Arimoto, R., Duce, R. A., Savoie, D. L., Prospero, J. M., Talbot, R., Cullen, J. D., et al. (1996). Relationships among aerosol constituents from Asia and the North Pacific during PEM-West A. Journal of Geophysical Research, 101, 2011–2023. doi:10.1029/95JD01071.

    Article  CAS  Google Scholar 

  • Arimoto, R., Kim, Y. J., Kim, Y. P., Quinn, P. K., Bates, T. S., Anderson, T. L., et al. (2006). Characterization of Asian dust during ASCE-Asia. Global and Planetary Change, 52, 23–56. doi:10.1016/j.gloplacha.2006.02.013.

    Article  Google Scholar 

  • Bae, M. S., Hong, C. S., Kim, Y. J., Han, J. S., Moon, K. J., Kondo, Y., et al. (2007). Intercomparison of two different thermal-optical elemental carbons and optical black carbon during ABC-EAREX2005. Atmospheric Environment, 41, 2791–2803. doi:10.1016/j.atmosenv.2006.11.040.

    Article  CAS  Google Scholar 

  • BP.www.bp.com/statisticalreview, 2008.

  • Carmichael, G. R., Hong, M.-S., Ueda, H., Chen, L.-L., Murano, K., Park, J. K., et al. (1997). Aerosol composition at Cheju Island, Korea. Journal of Geophysical Research, 102, 6047–6061. doi:10.1029/96JD02961.

    Article  CAS  Google Scholar 

  • Chen, L.-L., Carmichael, G. R., Hong, M.-S., Ueda, H., Shim, S., Song, C. H., et al. (1997). Influence of continental outflow events on the aerosol composition at Cheju Island, South Korea. Journal of Geophysical Research, 102, 28551–28574. doi:10.1029/97JD01431.

    Article  CAS  Google Scholar 

  • Choi, M. S., & Bang, E. J. (1999). Trace metals in airborne particulate collected at Cheju Island, Korea. Journal of Korean Society for Atmospheric Environment, 15, 727–738.

    Google Scholar 

  • Han, J. S., Moon, K. J., Ryu, S. Y., Kim, Y. J., & Perry, D. (2005). Source estimation of anthropogenic aerosols collected by a DRUM sampler during spring of 2002 at Gosan, Korea. Atmospheric Environment, 39, 3113–3125. doi:10.1016/j.atmosenv.2005.01.047.

    Article  CAS  Google Scholar 

  • Huebert, B. J., Bates, T., Russell, P. B., Shi, G., Kim, Y. J., Kawamura, K., et al. (2003). An overview of ACE-Asia: strategies for quantifying the relationships between Asian aerosols and their climatic impacts. Journal of Geophysical Research, 108. doi:10.1029/2003JD003550.

    Google Scholar 

  • Kang, C.-H., Kim, W.-H., Hu, C.-G., Kim, Y.-P., Shim, S.-G., & Hong, M.-S. (2001). Composition Analysis and Characteristics of Aerosols Collected at Kosan Site in Cheju Island, Korea during 1992–1999. The 12th World Clean Air & Environment Congress and Exhibition, Seoul.

  • Kim, N. K., & Kim, Y. P. (2008). Major factors affecting the ambient particulate nitrate level at Gosan, Korea. Atmospheric Research, 90, 104–114. doi:10.1016/j.atmosres.2007.10.017.

    Article  CAS  Google Scholar 

  • Kim, Y. P., Shim, S.-G., & Moon, K. C. (1998). Monitoring of air pollutants at Kosan, Cheju Island, Korea, during March–April 1994. Journal of Applied Meteorology, 37, 1117–1126. doi:10.1175/1520-0450(1998)037<1117:MOAPAK>2.0.CO;2.

    Article  Google Scholar 

  • Kim, Y. S., Kim, J. Y., Kim, Y., Moon, K. C., Moon, K. J., Han, J. S., et al. (2003). Concentrations variations of persistent organic pollutants in Gosan, Jeju during the polluted period in November 2001 and the yellow sand period in spring 2002. Journal of Korean Society for Atmospheric Environment, 19, 469–490.

    Google Scholar 

  • Lee, K. H., & Hu, C. G. (1995). A study on chemical composition of dustfall sampled in Cheju area: 2. Identification of source. Journal of Korean Society for Atmospheric Environment, 15, 101–111.

    Google Scholar 

  • Lee, J. H., Kim, Y. P., Moon, K.-C., Kim, H.-K., & Lee, J. B. (2001). Fine particles measurement at two background sites in Korea between 1996 and 1997. Atmospheric Environment, 35, 635–643. doi:10.1016/S1352-2310(00)00378-2.

    Article  CAS  Google Scholar 

  • Nishikawa, M., Hao, Q., & Morita, M. (2000). Preparation and evaluation of certified reference materials for Asian mineral dust. Global Environmental Research, 4, 103–113.

    CAS  Google Scholar 

  • Park, M. H., Kim, Y. P., & Kang, C.-H. (2003). Aerosol composition change due to dust storm: measurements between 1992 and 1999 at Gosan, Korea. Water Air and Soil Pollution Focus, 3, 117–128. doi:10.1023/A:1023278104910.

    Article  CAS  Google Scholar 

  • Park, M. H., Kim, Y. P., Kang, C.-H., & Shim, S.-G. (2004). Aerosol composition change between 1992 and 2002 at Gosan, Korea. Journal of Geophysical Research, 109. doi:10.1029/2003JD004110.

  • Richter, A., Burrows, J., Nub, H., Granier, C., & Niemeier, U. (2005). Increase in tropospheric nitrogen dioxide over China observed from space. Nature, 437, 129–132. doi:10.1038/nature04092.

    Article  CAS  Google Scholar 

  • Song, C. H., & Carmichael, G. R. (2001a). A three-dimensional modeling investigation of the evolution processes of dust and sea-salt particles in east Asia. Journal of Geophysical Research, 106, 18131–18154. doi:10.1029/2000JD900352.

    Article  CAS  Google Scholar 

  • Song, C. H., & Carmichael, G. R. (2001b). Gas–particle partitioning of nitric acid modulated by alkaline aerosol. Journal of Atmospheric Chemistry, 40, 1–22. doi:10.1023/A:1010657929716.

    Article  CAS  Google Scholar 

  • State Environmental Protection Administration (2008). http://english.mep.gov.cn/standards_reports/soe/SOE2006/200711/t20071106_112569.htm.

  • Sun, L., Zhou, X., Lu, J., Kim, Y. P., & Chung, Y.-S. (2003). Climatology, trend analysis and prediction of sandstorms and their associated dustfalls in China. Water Air and Soil Pollution Focus, 3, 41–50. doi:10.1023/A:1023213801276.

    Article  Google Scholar 

  • Takahashi, A., & Fujita, S.-I. (2000). Long-term trends in nitrate to non-seasalt sulfate ratio in precipitation collected in western Japan. Atmospheric Environment, 34, 4551–4555. doi:10.1016/S1352-2310(00)00145-X.

    Article  CAS  Google Scholar 

  • Underwood, G. M., Song, C. H., Phadnis, M., Carmichael, G. R., & Grassian, V. H. (2001). Heterogeneous reactions of NO2 and HNO3 on oxides and mineral dust: a combined laboratory and modeling study. Journal of Geophysical Research, 106, 18055–18066. doi:10.1029/2000JD900552.

    Article  CAS  Google Scholar 

  • Wang, Y., Zhuang, G., Tang, A., Zhang, W., Sun, Y., Wang, Z., et al. (2007). The evolution of chemical components of aerosols at five monitoring sites of China during dust storms. Atmospheric Environment, 41, 1091–1106. doi:10.1016/j.atmosenv.2006.09.015.

    Article  CAS  Google Scholar 

  • Whang, H. J., & Ro, C. U. (2006). Direct observation of nitrate and sulfate formations from mineral dust and sea-salts using low-Z particle election probe X-ray microanalysis. Atmospheric Environment, 40, 3869–3880. doi:10.1016/j.atmosenv.2006.02.022.

    Article  Google Scholar 

  • Whang, H. J., Kim, H. K., & Ro, C. U. (2008). Single-particle characterization of aerosol samples collected before and during an Asian dust storm in Chuncheon, Korea. Atmospheric Environment, 42, 8738–8746. doi:10.1016/j.atmosenv.2008.08.038.

    Article  Google Scholar 

  • Yates, D., Moore, D., & McCabe, G. (1998). The practice of statistics. New York: Freeman.

    Google Scholar 

Download references

Acknowledgments

This work was supported by the Korea Science and Engineering Foundation (KOSEF) through the National Research Lab. Program (No. R0A-2006-000-10221-0) and the SRC Program (the Climate Environment System Research Center). We thank Prof. C.-H. Kang at the Cheju National University, Korea for providing the sampling data.

Author information

Authors and Affiliations

Authors

Corresponding author

Correspondence to Yong Pyo Kim.

Rights and permissions

Reprints and permissions

About this article

Cite this article

Kim, N.K., Park, HJ. & Kim, Y.P. Chemical Composition Change in TSP Due to Dust Storm at Gosan, Korea: Do the Concentrations of Anthropogenic Species Increase Due to Dust Storm?. Water Air Soil Pollut 204, 165–175 (2009). https://doi.org/10.1007/s11270-009-0035-7

Download citation

  • Received:

  • Accepted:

  • Published:

  • Issue Date:

  • DOI: https://doi.org/10.1007/s11270-009-0035-7

Keywords

Navigation