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Double Exchange Interaction Between Mn3+ and Ru4+ Ions in La1−x Sr x Mn1−x Ru x O3

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Abstract

To study the magnetic interaction between Mn3+ and Ru4+, we designed and synthesized a series of samples La1−x Sr x Mn1−x Ru x O3 (0 ≤x ≤ 0.80), in which Mn and Ru ions remain as Mn3+ and Ru4+, respectively. The structural, magnetic, and transport properties of polycrystalline La1−x Sr x Mn1−x Ru x O3 (0 ≤x ≤ 0.80) were investigated. Measurements of magnetization show that Ru4+ substitution induces and enhances ferromagnetism as x≤ 0.30. According to measurements of electronic conductivity, all doping samples show the insulating behaviors without metal-insulation transition. However, with increasing Ru4+ substitution, resistivity decreases and a shoulder appears in the ρ(T) curves at around corresponding Curie temperature for 0.10 ≤ x ≤ 0.40. A large magnetoresistance effect is also observed in La0.60Sr0.40Mn0.60Ru0.40O3. All these phenomena is confirmed to be related with the double exchange interaction between Mn3+ and Ru4+ ions.

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Acknowledgments

This work was supported by National Nature Science Foundation of China through Grant No. 11204270 and Zhejiang Provincial Natural Science Foundation of China through Grant No. LQ12A04003.

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Authors and Affiliations

  1. Research Center of Magnetic and Electronic Materials, College of Materials Science and Engineering, Zhejiang University of Technology, Hangzhou, 310014, China

    Yao Ying, Jingwu Zheng, Liang Qiao, Wangchang Li, Wei Cai, Shenglei Che & Liqiang Jiang

  2. Department of Applied Physics, Nanjing University of Aeronautics and Astronautics, Nanjing, 210016, China

    Jiyu Fan

  3. Ningbo Institute of Material Technology and Engineering, Chinese Academy of Science, Ningbo, 315201, China

    Min Lin

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  1. Yao Ying
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  2. Jingwu Zheng
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  3. Liang Qiao
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  4. Wangchang Li
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  5. Wei Cai
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  8. Jiyu Fan
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  9. Min Lin
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Correspondence to Yao Ying.

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Ying, Y., Zheng, J., Qiao, L. et al. Double Exchange Interaction Between Mn3+ and Ru4+ Ions in La1−x Sr x Mn1−x Ru x O3 . J Supercond Nov Magn 28, 3117–3120 (2015). https://doi.org/10.1007/s10948-015-3146-y

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  • DOI: https://doi.org/10.1007/s10948-015-3146-y

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