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Structural variations during aging of the particles synthesized by laser ablation of copper in water

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Abstract

The formation of particles during ablation of copper (Cu) in distilled water by different pulse duration (5 ns, 200 ps and 30 fs), wavelength (1064 and 355 nm of 5 ns pulses), and energy is demonstrated. It is found that the initial particles of Cu rapidly oxidize to form cupric oxide (CuO) and cuprous oxide (Cu2O) particles. Pulse duration and wavelength play a crucial role during the process of formation, morphology change, and aging of particles. We demonstrate that ultra-short pulses allow obtaining particles with smaller sizes and narrower distribution. It is shown that the morphology of CuO/Cu2O particles in this case becomes more stable.

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Funding

The financial support from National Key Research and Development Program of China (2017YFB1104700, 2018YFB1107202), National Natural Science Foundation of China (NSFC, 91750205, 61774155, 61705227), Scientific Research Project of the Chinese Academy of Sciences (QYZDB-SSW-SYS038), Jilin Provincial Science & Technology Development Project (20180414019GH) and The Key Program of the International Partnership Program of CAS (181722KYSB20160015) is appreciated. R.A.G. thanks the financial support from Chinese Academy of Sciences President’s International Fellowship Initiative (Grant No. 2018VSA0001).

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Authors and Affiliations

  1. The Guo China-US Photonics Laboratory, State Key Laboratory of Applied Optics, Changchun Institute of Optics, Fine Mechanics and Physics, Chinese Academy of Sciences, Changchun, 130033, China

    Ke Zhang, Rashid A. Ganeev, Ganjaboy S. Boltaev & Chunlei Guo

  2. University of Chinese Academy of Sciences, Beijing, 100049, China

    Ke Zhang

  3. Faculty of Physics, Voronezh State University, University Square, Voronezh, 394018, Russia

    Rashid A. Ganeev

  4. The Institute of Optics, University of Rochester, Rochester, NY, 14627, USA

    Chunlei Guo

  5. Department of Physics, American University of Sharjah, PO Box 26666, Sharjah, UAE

    Rashid A. Ganeev & Ganjaboy S. Boltaev

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  1. Ke Zhang
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  2. Rashid A. Ganeev
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  3. Ganjaboy S. Boltaev
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Zhang, K., Ganeev, R.A., Boltaev, G.S. et al. Structural variations during aging of the particles synthesized by laser ablation of copper in water. Appl. Phys. A 125, 698 (2019). https://doi.org/10.1007/s00339-019-2992-z

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