Skip to main content
Log in

Growth of atomically flat thin films of the electronically phase-separated manganite (La0.5Pr0.5)0.67Ca0.33MnO3

  • Published:
Applied Physics A Aims and scope Submit manuscript

Abstract

Atomically flat and epitaxial thin films of the electronically phase-separated compound \((\hbox {La}_{0.5}\hbox {Pr}_{0.5})_{0.67}\hbox {Ca}_{0.33}\hbox {MnO}_{3}\) were grown on as-received and treated (110) \(\hbox {NdGaO}_{3}\) substrates by fine tuning of oxygen pressure during deposition. The optimal conditions were determined using surface morphology, transport, magnetization, and X-ray diffraction measurements. Optimal thin films show step flow growth mode and bulk-like physical properties compared to thin films grown in off-optimal oxygen pressures, viz. the highest maximum temperature coefficient of resistance, the highest peak resistivity temperature, and reduced coercive fields.

This is a preview of subscription content, log in via an institution to check access.

Access this article

Price excludes VAT (USA)
Tax calculation will be finalised during checkout.

Instant access to the full article PDF.

Fig. 1
Fig. 2
Fig. 3

Similar content being viewed by others

References

  1. W. Prellier, P. Lecoeur, B. Mercey, J. Phys.: Condens. Matter 13, R915 (2001)

    ADS  Google Scholar 

  2. H.M. Christen, G. Eres, J. Phys.: Condens. Matter 20, 264005 (2008)

    ADS  Google Scholar 

  3. W.S. Choi, Z. Marton, S.Y. Jang, S.J. Moon, B.C. Jeon, J.H. Shin, S.S.A. Seo, T.W. Noh, K. Myung-Whun, H.N. Lee, Y.S. Lee, J. Phys. D: Appl. Phys. 42, 165401 (2009)

    Article  ADS  Google Scholar 

  4. Z. Marton, S.S.A. Seo, T. Egami, H.N. Lee, J. Cryst. Growth 312, 2923 (2010)

    Article  ADS  Google Scholar 

  5. H. Jeen, W.S. Choi, J.W. Freeland, H. Ohta, C.U. Jung, H.N. Lee, Adv. Mater. 25, 3651 (2013)

    Article  Google Scholar 

  6. D.G. Schlom, L.Q. Chen, C.B. Eom, K.M. Rabe, S.K. Streiffer, J.M. Triscone, Annu. Rev. Mater. Res. 37, 589 (2007)

    Article  ADS  Google Scholar 

  7. S. Jin, T.H. Tiefel, M. McCormack, R.A. Fastnacht, R. Ramesh, L.H. Chen, Science 264, 413 (1994)

    Article  ADS  Google Scholar 

  8. M. Uehara, S. Mori, C.H. Chen, S.W. Cheong, Nature 399, 560 (1999)

    Article  ADS  Google Scholar 

  9. K.H. Ahn, T. Lookman, A.R. Bishop, Nature 428, 401 (2004)

    Article  ADS  Google Scholar 

  10. Y. Suzuki, H.Y. Hwang, S.W. Cheong, T. Siegrist, R.B. van Dover, A. Asamitsu, Y. Tokura, J. Appl. Phys. 83, 7064 (1998)

    Article  ADS  Google Scholar 

  11. A. Biswas, M. Rajeswari, R.C. Srivastava, Y.H. Li, T. Venkatesan, R.L. Greene, A.J. Millis, Phys. Rev. B 61, 9665 (2000)

    Article  ADS  Google Scholar 

  12. A. Bhattacharya, S.J. May, S.G.E. te Velthuis, M. Warusawithana, X. Zhai, B. Jiang, J.M. Zuo, M.R. Fitzsimmons, S.D. Bader, J.N. Eckstein, Phys. Rev. Lett. 100, 257203 (2008)

    Article  ADS  Google Scholar 

  13. T.Z. Ward, J.D. Budai, Z. Gai, J.Z. Tischler, L. Yin, J. Shen, Nat. Phys. 5, 885 (2009)

    Article  Google Scholar 

  14. H. Boschker, M. Mathews, E.P. Houwman, H. Nishikawa, A. Vailionis, G. Koster, G. Rijnders, D.H.A. Blank, Phys. Rev. B 79, 214425 (2009)

    Article  ADS  Google Scholar 

  15. H. Jeen, A. Biswas, Phys. Rev. B 88, 024415 (2013)

    Article  ADS  Google Scholar 

  16. Y. Chen, J. Washburn, Phys. Rev. Lett. 77, 4046 (1996)

    Article  ADS  Google Scholar 

  17. A. Gupta, G.Q. Gong, G. Xiao, P.R. Duncombe, P. Lecoeur, P. Trouilloud, Y.Y. Wang, V.P. Dravid, J.Z. Sun, Phys. Rev. B 54, R15629 (1996)

    Article  ADS  Google Scholar 

  18. A.S. Ogale, S.R. Shinde, V.N. Kulkarni, J. Higgins, R.J. Choudhary, D.C. Kundaliya, T. Polleto, S.B. Ogale, R.L. Greene, T. Venkatesan, Phys. Rev. B 69, 235101 (2004)

    Article  ADS  Google Scholar 

  19. H.L. Ju, J. Gopalakrishnan, J.L. Peng, Q. Li, G.C. Xiong, T. Venkatesan, R.L. Greene, Phys. Rev. B 51, 6143 (1995)

    Article  ADS  Google Scholar 

  20. G.J.H.M. Rijnders, G. Koster, D.H.A. Blank, H. Rogalla, Appl. Phys. Lett. 70, 1888 (1997)

    Article  ADS  Google Scholar 

  21. H. Lee, H. Christen, M. Chisholm, C. Rouleau, D. Lowndes, Nature 433, 395 (2005)

    Article  ADS  Google Scholar 

  22. G. Eres, J.Z. Tischler, M. Yoon, B.C. Larson, C.M. Rouleau, D.H. Lowndes, P. Zschack, Appl. Phys. Lett. 80, 3379 (2002)

    Article  ADS  Google Scholar 

  23. J. Dho, N.H. Hur, I.S. Kim, Y.K. Park, J. Appl. Phys. 94, 7670 (2003)

    Article  ADS  Google Scholar 

  24. M. Huijben, L.W. Martin, Y.-H. Chu, M.B. Holcomb, P. Yu, G. Rijnders, D.H.A. Blank, R. Ramesh, Phys. Rev. B 78, 094413 (2008)

    Article  ADS  Google Scholar 

  25. H. Boschker, M. Huijben, A. Vailionis, J. Verbeeck, S. van Aert, M. Luysberg, S. Bals, G. van Tendeloo, E.P. Houwman, G. Koster, D.H.A. Blank, G. Rijnders, J. Phys. D: Appl. Phys. 44, 205001 (2011)

    Article  ADS  Google Scholar 

  26. V. Podzorov, B.G. Kim, V. Kiryukhin, M.E. Gershenson, S.W. Cheong, Phys. Rev. B 64, 140406 (2001)

    Article  ADS  Google Scholar 

  27. H. Jeen, A. Biswas, Phys. Rev. B 83, 064408 (2011)

    Article  ADS  Google Scholar 

  28. W. Prellier, M. Rajeswari, T. Venkatesan, R.L. Greene, Appl. Phys. Lett. 75, 1446 (1999)

    Article  ADS  Google Scholar 

  29. V. Leca, Ph.D. Thesis (University of Twente, 2003)

  30. T. Dhakal, J. Tosado, A. Biswas, Phys. Rev. B 75, 092404 (2007)

    Article  ADS  Google Scholar 

  31. J.A. Collado, C. Frontera, J.L. Garcia-Munoz, C. Ritter, M. Brunelli, M.A.G. Aranda, Chem. Mater. 15, 167 (2003)

    Article  Google Scholar 

  32. J. Tosado, T. Dhakal, A. Biswas, J. Phys.: Condens. Matter 21, 192203 (2009)

    ADS  Google Scholar 

  33. A. Urushibara, Y. Moritomo, T. Arima, A. Asamitsu, G. Kido, Y. Tokura, Phys. Rev. B 51, 14103 (1995)

    Article  ADS  Google Scholar 

  34. P. Schiffer, A.P. Ramirez, W. Bao, S.W. Cheong, Phys. Rev. Lett. 75, 3336 (1995)

    Article  ADS  Google Scholar 

  35. H.Y. Hwang, S.W. Cheong, N.P. Ong, B. Batlogg, Phys. Rev. Lett. 77, 2041 (1996)

    Article  ADS  Google Scholar 

  36. Z.L. Wang, J.S. Yin, Philos. Mag. B 77, 49 (1998)

    Article  ADS  Google Scholar 

  37. S.B. Adler, J. Am. Ceram. Soc. 84, 2117 (2001)

    Article  Google Scholar 

  38. Y.-M. Kim, J. He, M.D. Biegalski, H. Ambaye, V. Lauter, H.M. Christen, S.T. Pantelides, S.J. Pennycook, S.V. Kalinin, A.Y. Borisevich, Nat. Mater. 11, 888 (2012)

    Article  ADS  Google Scholar 

  39. T. Taniyama, M. Yamasaki, Y. Yamazaki, Appl. Phys. Lett. 81, 4562 (2002)

    Article  ADS  Google Scholar 

  40. S.H. Yun, Ph.D. Thesis (University of Florida, 2008)

  41. P. Orgiani, R. Ciancio, A. Galdi, S. Amoruso, L. Maritato, Appl. Phys. Lett. 96, 032501 (2010)

    Article  ADS  Google Scholar 

Download references

Acknowledgments

This work was supported by NSF DMR-1410237. H.J. acknowledges financial support from the Research Fund Program of Research Institute for Basic Sciences, Pusan National University, Korea, 2014, Project No. RIBS-PNU-2014-304. The authors are grateful for discussion with H. N. Lee. X-ray diffraction was conducted at major analytical instrumentation center, University of Florida.

Author information

Authors and Affiliations

Authors

Corresponding author

Correspondence to Amlan Biswas.

Rights and permissions

Reprints and permissions

About this article

Check for updates. Verify currency and authenticity via CrossMark

Cite this article

Jeen, H., Javed, R. & Biswas, A. Growth of atomically flat thin films of the electronically phase-separated manganite (La0.5Pr0.5)0.67Ca0.33MnO3 . Appl. Phys. A 122, 35 (2016). https://doi.org/10.1007/s00339-015-9543-z

Download citation

  • Received:

  • Accepted:

  • Published:

  • DOI: https://doi.org/10.1007/s00339-015-9543-z

Keywords

Navigation