Abstract
We present an exact closed formulation of the reversible diffusion-limited coagulation-growth reactions 2A ↔ A with irreversible input B → A in one spatial dimension. The treatment here accommodates spatial as well as temporal variations in the particle density with a complete account of microscopic fluctuations and correlations. Moreover, spatial and/or temporal variations in the transport and reaction coefficients can be included in the model. A general solution to the reversible process is presented, and we explore the phenomenon of wavefront propagation.
Similar content being viewed by others
References
G. Nicolis and I. Prigogine,Self Organization in Nonequilibrium Systems (Wiley, New York, 1977); H. Haken,Synergetics: An Introduction (Springer, Berlin, 1978).
A. M. Turing,Phil. Trans. R. Soc. Lond. B 237:37 (1952); H. Meinhardt,Models of Biological Pattern Formation (Academic Press, London, 1982); J. D. Murray,Mathematical Biology (Springer, Berlin, 1989).
P. Ortoleva, G. Auchmuty, J. Chadam, J. Hettner, E. Merino, C. H. Moore, and E. Ripley,Physica D 19:334 (1988); T. Dewers and P. Ortoleva,J. Phys. Chem. 93:2842 (1989).
B. Röhricht, J. Parisi, J. Peinke, and O. E. Rössler, Z.Phys. B 65:259 (1986); H.-G. Purwins, C. Radehaus, and J. Berkemeier,Z. Naturforsch 43a:17 (1988).
K. Kang and S. Redner,Phys. Rev. A 32:435 (1985); R. Kopelman,Science 241:1620 (1988).
R. Szostak,Molecular Sieves-Principles of Synthesis and Identification (Van Nostrand Reinhold, New York, 1989); R. M. Barrer, inInclusion Compounds 1, J. L. Atwood, J. E. D. Davies, and D. D. MacNicol (Academic Press, London, 1984); A. Dyer,An. Introduction to Zeolite Molecular Sieves (Wiley, New York, 1988).
C. R. Doering and D. Ben-Avraham,Phys. Rev. A 38:3035 (1988); C. R. Doering and D. ben-Avraham,Phys. Rev. Lett. 62:2563 (1989); M. A. Burschka, C. R. Doering, and D. ben-Avraham,Phys. Rev. Lett. 63:700 (1989); C. R. Doering and M. A. Burschka,Phys. Rev. Lett. 64:245 (1990).
D. Ben-Avraham, M. A. Burschka, and C. R. Doering,J. Stat. Phys. 60:695 (1990).
M. A. Burschka,J. Stat. Phys. 45:715 (1986).
C. E. Smith and H. C. Tuckwell, inLecture Notes in Biomathematics, Vol. 2, S. Levin, ed. (Springer, Berlin, 1974); F. Schlögl, Z.Physik. 253:147 (1972).
P. C. Fife,Mathematical Aspects of Reacting and Diffusing Systems (Springer, Berlin, 1979); J. J. Tyson,The Belousov-Zhabotinskii Reaction (Springer, Berlin, 1976); P. Kaliappan,Physica D 11:368 (1984).
N. G. van Kampen,Int. J. Quantum Chem. Quantum Chem. Symp. 16:101 (1982); J. C. Lin, C. R. Doering, and ben-Avraham,Chem. Phys. 146:355 (1990).
M. Abramowitz and I. A. Stegun,Handbook of Mathematical Functions (Dover, New York, 1965).
W. Horsthemke and R. Lefever,Noise Induced Transitions (Springer, Berlin, 1984).
C. R. Doering, H. R. Brand, and R. E. Ecke, eds., Proceedings of the workshop on external noise and its interaction with spatial degrees of freedom in nonlinear dissipative systems,J. Stat. Phys. 54(5/6) (1989).
M. A. Burschka, Exact solution of theN-body initial value problem for the diffusionlimited logistic diffusion-reaction system, preprint (1991).
Author information
Authors and Affiliations
Rights and permissions
About this article
Cite this article
Doering, C.R., Burschka, M.A. & Horsthemke, W. Fluctuations and correlations in a diffusion-reaction system: Exact hydrodynamics. J Stat Phys 65, 953–970 (1991). https://doi.org/10.1007/BF01049592
Issue Date:
DOI: https://doi.org/10.1007/BF01049592