Summary
Ozone for a ten year period obtained from the Total Ozone Mapping Spectrometer (TOMS) has been compared with velocity potential for the same period. It has been found that the global-scale circulation serves to modulate the ozone concentration over the tropical Atlantic Ocean. Examination of the low frequency modes reveal close correspondence between the two parameters, especially at the annual timescale. Descending motion over southern Africa reduces precipitation, thereby enhancing biomass burning and the subsequent release of trace gases and the possible photochemical production of ozone. Transport to the ozone maximum region over the tropical Atlantic Ocean occurs mainly from tropical Africa. Little evidence has been found on a climatological time-scale to support the theory of stratospheric infusion into the troposphere above the tropical Atlantic Ocean.
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Andreae, M. O., Browell, E. V., Garstang, M., Gregory, G. L., Harriss, R. C., Hill, G. F., Jacob, D. J., Pereira, M. C., Sachse, G. W., Setzer, A. W., Silva Dias, P. L., Talbot, R. W., Torres, A. L., Wofsy, S. C., 1988: Biomass-burning emissions and associated haze layers over Amazonia.J. Geophys. Res.,93, 1509–1527.
Barnes, S. L., 1964: A technique for maximizing details in numerical weather map analysis.J. Appl. Meteor.,3, 396–409.
Bensman, E. L., 1993: Climatological investigation and advective modeling of the tropospheric ozone maximum over the tropical South Atlantic Ocean Unpublished M. S. Dissertation, Department of Meteorology, Florida State University, Tallahassee, 98pp.
Chatfield, R. B., Delany, A. C., 1990: Convection links biomass burning to increased tropical ozone: However, models will tend to overpredict O3.J. Geophys. Res.,95, 18473–18488.
Cros, B., Delmas, R., Ngaga, D., Chirac, B., 1988: Seasonal trends of ozone in equatorial Africa: Experimental evidence of photochemical formation.J. Geophys. Res.,93, 8355–8366.
Fishman, J., 1991: Probing planetary pollution from space.Environ. Sci. Technol.,25, 613–620.
Fishman, J., Larsen, J. C., 1987: Distribution of total ozone and stratospheric ozone in the tropics: Implications for the distribution of tropospheric ozone.J. Geophys. Res.,92, 6627–6634.
Fishman, J., Solomon, S., Crutzen, P. J., 1979: Observational and theoretical evidence in support of a significant in situ photochemical source of trophospheric ozone.Tellus,31B, 422–446.
Fishman, J., Minnis, P., Reichle, H. G., 1986: The use of satellite data of study tropospheric ozone in the tropics.J. Geophys. Res.,91, 14451–14465.
Fishman, J., Watson, C. E., Larsen, J. C., Logan, J. A., 1990: Distribution of tropospheric ozone determined from satellite data.J. Geophys. Res.,95, 3599–3617.
Fishman, J., Fakhruzzaman, B., Cros, B., Nganga, D., 1991: Identification of widespread pollution in the southern hemisphere deduced from satellite analysis.Sci.,252, 1693–1696.
Funk, J. P., Garnham, G. L., 1962: Australian ozone observations and a suggested 24 month cycle.Tellus,14, 378–381.
Hamming, R. W., 1977:Digital Filters. Englewood Cliffs, NY: Prentice-Hall, 226pp.
Hasebe, F., 1983: Interannual variations of global total ozone revealed from Nimbus 4 BUV and ground based observations.J. Geophys. Res.,88, 6819–6834.
Hastenrath, S., 1991:Climate Dynamics of the Tropics. Dordrecht: Kluwer, 488pp.
Hastenrath, S., Wu, M.-C., 1982: Oscillations of upperair circulation and anomalies in the surface climate of the tropics.Arch. Meteor. Geophys. Biokl., Ser. B,31, 1–37.
Hilsenrath, E., Heath, D. F., Schlesinger, B. M., 1979: Seasonal and interannual variations in total ozone revealed by the Nimbus 4 backscattered ultraviolet experiment.J. Geophys. Res.,84, 6969–6979.
Hingane, L. S., 1990: Ozone valley in the subtropics.J. Atmos. Sci.,47, 1814–1816.
Julian, P. R., Chervin, R. M., 1978: A study of the Southern Oscillation and Walker Circulation phenomenon.Mon. Wea. Rev. 106, 1433–1451.
Kirchhoff, V. W. J. H., Nobre, C. A., 1986: Atmospheric chemistry research in Brazil: Ozone measurements at Natal, Manuas and Cuiba.Rev. Geofis.,24, 95–108.
Knutson, T. R., Weickmann, K. M., 1987: 30–60 day atmospheric oscillations: Composite life cycles of convection and circulation anomalies.Mon. Wea. Rev.,115, 1407–1436.
Krishnamurti, T. N., Fuelberg, H. E., Sinha, M. C., Oosterhof, D., Bensman, E., Kumar, V. B., 1993: The environment of the tropospheric ozone maximum over the tropical south Atlantic Ocean, Part I: Atmospheric circulations.J. Geophys. Res.,98 10621–10641.
Lindesay, J. A., 1988: The southern oscillation and atmospheric circulation changes over southern Africa. Unpublished PhD Thesis, University of the Witwatersrand, Johannesburg, 284pp.
Logan, J. A., Kirchhoff, V. W. C. H., 1986: Seasonal variations of tropospheric ozone at Natal, Brazil,J. Geophys. Res.,91, 7875–7882.
Lyons, S. W., 1991: Origins of convective instability over equatorial southern Africa.J. Climatol.,4, 23–29.
Newell, R. E., Gould-Stewart, S., 1981: A stratospheric foundtain?J. Atmos. Sci.,38, 2789–2796.
Oltmans, S., 1981: Surface ozone measurements in clean air.J. Geophys. Res.,86, 1174–1180.
Pickering, K. E., Thompson, A. M., Wang, Y., Tao, W.-K., McNamara, D. P., Kirchoff, V. W. J. H., Heikes, B. G., Sachse, G. W., Bradshaw, J. D., Gregory, G. L., Blake, D. R., 1996: Convective transport of biomass burning emissions over Brazil during TRACE-A.J. Geophys. Res., (In press).
Piotrowicz, S. R., Rasmussen, R. A., Hanson, K. J., Fischer, C. J., 1989: Ozone in the boundary layer of the equatorial Atlantic Ocean.Tellus,41B, 314–322.
Piotrowicz, S. R., Bezdek, H. F., Harvey, G. R., Springer-Young, M., 1991: On the ozone minimum over the equatorial Pacific Ocean.J. Geophys. Res.,96, 18769–18787.
Ramage, C. S., 1983: Teleconnections and the seige of time.J. Climatol.,3, 223–231.
Stephens, J. J., Johnson, K. W., 1978: Rotational and divergent wind potentials.Mon. Wea. Rev.,106, 1452–1458.
Swap, R., Garstang, M. Macko, S. A., Tyson, P. D., Maenhaut, W., Artaxo, P., Kållberg, P., Talbot, R., 1996: The long-range transport of southern African aerosols to the tropical South Atlantic.J. Geophys. Res., SAF ARI Special Edition, (In press).
Thompson, A. M., McNamara, D. P., Pickering, K. E., McPeters, R. D., 1993a: Effect of marine stratocumulus on TOMS ozone.J. Geophys. Res.,98, 23051–23057.
Thompson, A. M., Johnson, J. E., Torres, A. L., Bates, T. S., Kelly, K. C., Atlas, E., Greenberg, J. P., Donahue, N. M., Yvon, S. A., Saltzman, E. S., Heikes, B. G., Mosher, B. W., Shashkow, A. A., Yegorov, V. I., 1993b: Ozone observations and a model of marine boundary layer photochemistry during SAGA 3.J. Geophys. Res.,98, 16955–16968.
Thompson, A. M., Zenker, T., Bodeker, G. E., McNamara, D. P., 1996: Ozone over southern Africa: Patterns and influences. In: Lindesay, J. A., Andreae, M. O., Tyson, P. D., Wilgen, B. van (eds.)Fire in Southern African Savanna: Ecological and Atmospheric Perspectives. In press.
Tolson, R. H., 1981: Spatial and temporal variations of monthly mean total columnar ozone derived from 7 years of BUV data.J. Geophys. Res.,86, 7312–7330.
Tyson, P. D., 1986:Climatic Change and Variability in Southern Africa. Cape Town: Oxford University Press, 220pp.
Watson, C. E., Fishman, J., Reichle, H. G., 1990: The significance of biomass burning as a source of carbon monoxide and ozone in the southern hemisphere tropics.J. Geophys. Res.,95, 16443–16450.
Weickmann, K. M., Lussky, G. R., Kutzbach, J. E., 1985: Intraseasonal (30–60 day) fluctuations of outgoing longwave radiation and 250 hPa streamfunction during northern winter.Mon. Wea. Rev.,113, 941–961.
Winker, P., 1988: Surface ozone over the Atlantic Ocean.J. Atmos. Chem.,7, 73–91.
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D'Abreton, P.C. Atmospheric circulation and the tropospheric ozone maximum over the tropical South Atlantic Ocean. Meteorl. Atmos. Phys. 61, 75–87 (1996). https://doi.org/10.1007/BF01029713
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DOI: https://doi.org/10.1007/BF01029713