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Comparison of focusing optics for femtosecond X-ray diffraction

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Abstract

We characterize and compare four different types of focusing optics for hard X-rays, suitable for femtosecond X-ray diffraction experiments, usinga tabletop femtosecond laser-based plasma source. We demonstrate a 23 μmfocus with a toroidally bent Ge single crystal. A maximum flux of 7× 108 photons/(s mm2) is generated in a 32 μm focus using a multi-layer mirror. An elliptical glass capillary yields the highest number of photons per Bragg angle [2× 105 photons/(s mrad)]. The largest number of photons[3× 106 photons/s] per second is obtained in the 105 μm focus of a poly-capillary optical lens system. All numbers are given for characteristic Cu K α photons.

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References

  1. K. Sokolowski-Tinten, C. Blome, J. Blums, A. Cavalleri, C. Dietrich, A. Tarasevitch, I. Uschmann, E. Foerster, M. Kammler, M. Horn-von-Hoegen, D. von der Linde, Femtosecond X-ray measurement of coherent lattice vibrations near the Lindemann stability limit. Nature 422, 287 (2003)

    PubMed  Google Scholar 

  2. K. Sokolowski-Tinten, C. Blome, C. Dietrich, A. Tarasevitch, M.H. von Hoegen, D. von der Linde, A. Cavalleri, J. Squier, M. Kammler, Femtosecond X-ray measurement of ultrafast melting and large acoustic transients. Phys. Rev. Lett. 87, 225701 (2001)

    Article  PubMed  Google Scholar 

  3. A. Cavalleri, C.W. Siders, F.L.H. Brown, D.M. Leitner, C. Tóth, J.A. Squier, C.P.J. Barty, K.R. Wilson, K. Sokolowski-Tinten, M. Horn von Hoegen, D. von der Linde, M. Kammler, Anharmonic lattice dynamics in germanium measured with ultrafast X-ray diffraction. Phys. Rev. Lett. 85, 586 (2000)

    Article  PubMed  Google Scholar 

  4. C. Rose-Petruck, R. Jiminez, T. Guo, A. Cavalleri, C. Siders, F. Raksi, J. Squier, B. Walker, K. Wilson, C. Barty, Picosecond milliangstrom lattice dynamics measured by ultrafast X-ray diffraction. Nature 398, 310 (1999)

    Article  Google Scholar 

  5. C. Rischel, A. Rousse, I. Uschmann, P. Albouy, J. Geindre, P. Audebert, J. Gauthier, E. Förster, J. Martin, A. Antonetti, Femtosecond time-resolved X-ray diffraction from laser-heated organic films. Nature 390, 490 (1997)

    Article  Google Scholar 

  6. C.W. Siders, A. Cavalleri, K. Sokolowski-Tinten, C. Toth, T. Guo, M. Kammler, M.H. von Hoegen, K.R. Wilson, D. von der Linde, C.P.J. Barty, Detection of non-thermal melting by ultrafast X-ray diffraction. Science 286, 1340 (1999)

    Article  PubMed  Google Scholar 

  7. A. Rousse, C. Rischel, S. Fourmaux, I. Uschmann, S. Sebban, G. Grillon, Ph. Balcou, E. Foerster, J.P. Geindre, P. Audebert, J.C. Gauthier, D. Hulin, Non-thermal melting in semiconductors measured at femtosecond resolution. Nature 410, 65 (2001)

    PubMed  Google Scholar 

  8. M. Bargheer, N. Zhavoronkov, Y. Gritsai, D.H. Woo, D.S. Kim, M. Woerner, T. Elsaesser, Femtosecond X-ray diffraction from coherent atomic motions in nano-structures. Science 306, 1771 (2004)

    Article  PubMed  Google Scholar 

  9. G. Hildebrandt, H. Bradaczek, Approaching real X-ray optics. Rikagu J. 17, 13 (2000)

    Google Scholar 

  10. A.M. Khounsary, A.K. Freund, T. Ishikawa, G. Srajer, J. Lang (eds.), X-ray Optics Design, Performance and Applications, Proceedings of SPIE (SPIE, Denver, Colorado, 1999)

    Google Scholar 

  11. T. Missalla, I. Uschmann, E. Förster, G. Jenke, D. von der Linde, Monochromatic focusing of subpicosecond X-ray pulses in the keV range. Rev. Sci. Instrum. 70, 1288 (1999)

    Article  Google Scholar 

  12. I. Tomov, P. Chen, P. Renzepis, Pulse broadening in femtosecond X-ray diffraction. J. Appl. Phys. 83, 5546 (1998)

    Article  Google Scholar 

  13. F. Chukhovskii, E. Förster, Time-dependent X-ray Bragg diffraction. Acta Cryst. A 51, 668 (1995)

    Article  Google Scholar 

  14. P. Kirkpatrick, A. Baez, Formation of optical images by X-rays. J. Opt. Soc. Am. 38, 766 (1948)

    Google Scholar 

  15. M. Schuster, H. Gobel, Parallel-beam coupling into channel-cut monochromators using curved graded multilayers. J. Phys. D 28, 270 (1995)

    Article  Google Scholar 

  16. N. Zhavoronkov, Y. Gritsai, G. Korn, T. Elsaesser, Ultra-short efficient laser driven hard X-ray source operated at a kHz repetition rate. Appl. Phys. B 79, 663 (2004)

    Article  Google Scholar 

  17. N. Zhavoronkov, Y. Gritsai, M. Bargheer, M. Woerner, T. Elsaesser, Microfocus Cu K index alpha source for femtosecond X-ray science, Opt. Lett., in press

  18. I. Tomov, J. Chen, X. Ding, P. Rentzepis, Efficient focusing of hard X-rays generated by femtosecond laser driven plasma. Chem. Phys. Lett. 389, 363 (2004)

    Google Scholar 

  19. R. Tommasini, R. Bruch, E. Fill, A. Bjeoumikhov, Convergent beam diffraction of ultrashort hard X-ray pulses focused by a capillary lens. Rev. Sci. Instrum., in press (2004)

  20. F. Benesch, T. Lee, Y. Jiang, C.G. Rose-Petruck, Ultrafast laser-driven X-ray spectrometer for X-ray absorption spectroscopy of transition metal complexes. Opt. Lett. 29, 1028 (2004)

    Article  PubMed  Google Scholar 

  21. A. Bjeoumikhov, N. Langhoff, S. Bjeoumikhova, R. Wedell, Capillary optics for micro X-ray fluorescence analysis. Rev. Sci. Instrum., submitted for publication (2005)

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Bargheer, M., Zhavoronkov, N., Bruch, R. et al. Comparison of focusing optics for femtosecond X-ray diffraction. Appl. Phys. B 80, 715–719 (2005). https://doi.org/10.1007/s00340-005-1792-7

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  • DOI: https://doi.org/10.1007/s00340-005-1792-7

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