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Indications for the coexistence of closed orbit and quantum interferometer with the same cross section in the organic metal β′′-(ET)4(H3O)[ Fe(C2O4)3] .C6H4Cl2: persistence of Shubnikov-de Haas oscillations above 30 K

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Abstract

Shubnikov-de Haas (SdH) and de Haas-van Alphen (dHvA) oscillations spectra of the quasi-two dimensional charge transfer salt β′′-(ET)4(H3O)[ Fe(C2O4)3] .C6H4Cl2 have been investigated in pulsed magnetic fields up to 54 T. The data reveal three basic frequencies Fa, Fb and Fb - a, which can be interpreted on the basis of three compensated closed orbits at low temperature. However a very weak thermal damping of the Fourier component Fb, with the highest amplitude, is evidenced for SdH spectra above about 6 K. As a result, magnetoresistance oscillations are observed at temperatures higher than 30 K. This feature, which is not observed for dHvA oscillations, is in line with quantum interference, pointing to a Fermi surface reconstruction in this compound.

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Authors and Affiliations

  1. Laboratoire National des Champs Magnétiques Intenses (UPR 3228 CNRS, INSA, UJF, UPS), 143 avenue de Rangueil, 31400, Toulouse, France

    D. Vignolles & A. Audouard

  2. Institució Catalana de Recerca i Estudis Avançats (ICREA), 08010, Barcelona, Spain

    V. N. Laukhin

  3. Institut de Ciència de Materials de Barcelona (ICMAB - CSIC), Campus UAB, 08193, Bellaterra, Catalunya, Spain

    V. N. Laukhin & E. Canadell

  4. Institute of Problems of Chemical Physics, Russian Academy of Sciences, 142432, Chernogolovka, Moscow oblast, Russia

    T. G. Prokhorova & E. B. Yagubskii

Authors
  1. D. Vignolles
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  2. A. Audouard
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  3. V. N. Laukhin
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  4. E. Canadell
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  5. T. G. Prokhorova
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  6. E. B. Yagubskii
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Correspondence to A. Audouard.

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Vignolles, D., Audouard, A., Laukhin, V. et al. Indications for the coexistence of closed orbit and quantum interferometer with the same cross section in the organic metal β′′-(ET)4(H3O)[ Fe(C2O4)3] .C6H4Cl2: persistence of Shubnikov-de Haas oscillations above 30 K. Eur. Phys. J. B 71, 203–209 (2009). https://doi.org/10.1140/epjb/e2009-00306-1

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  • DOI: https://doi.org/10.1140/epjb/e2009-00306-1

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