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Recent Advances in Nanocasting Cobalt-Based Mesoporous Materials for Energy Storage and Conversion

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Abstract

The generation of novel mesoporous materials with well-defined structure and accessible pore networks is helpful in both fundamental and energy-related research. Nanocasting mesoporous earth-abundant materials and their composite materials offer opportunities to make electrochemically active materials that allow scalable production and cost-effectiveness. Recently, due to their intrinsic open pore structure as well as high surface areas, various mesoporous cobalt-based ordered materials have been applied to electrocatalysis, rechargeable batteries, and supercapacitors. In this review, we have critically evaluated the advancements made specifically in three- and two-dimensionally (3D/2D) electrode Co-based materials (oxides, nitrides, phosphides, and sulfides). We outline foreseeable challenges and issues for the utilization of mesostructured cobalt-based electrode materials. This review also provides guidelines for further work to those who work on energy-related applications of mesoporous cobalt-based materials.

Nanocast cobalt-based mesoporous materials hold great promise in the application of energy conversion and storage. Herein, recent advances of two-dimensional and three-dimensional mesoporous cobalt-based mesoporous oxides, nitrides, phosphides, and sulfides used for electrocatalysis, rechargeable batteries, and supercapacitors were discussed. Moreover, the structure-property relationships of these materials and current challenges in both nanoarchitecture design and their applications in electrochemical energy devices are proposed. An outlook is provided for future research.

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Funding

This work is supported by the Chinese Academy of Sciences (Grant No. 2018PS0011) and Natural Science Foundation of China (Grant No. 21471147 and 61971405) and the National Key Research and Development Plan (Grant No. 2016YFB0101205). M.Y. would like to thank the National “Thousand Youth Talents” program of China and Ningbo 3315 program for the support. T.T. acknowledges the funding from the Ministry of Electronics and Information Technology, India (Project ID: ELE1819353MEITNAK), and the Department of Science and Technology, India (Project ID: MET1617146DSTXTIJU, DST/TMD/MES/2K18/17, DST 11-IFA-PH-07, and DST/TMD/SERI/HUB/1(C), DST Solar Energy Harnessing Center, Materials for energy storage) for supporting this research work.

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Authors and Affiliations

  1. Solid State Functional Materials Research Laboratory, Ningbo Institute of Materials Technology and Engineering (NIMTE), Chinese Academy of Sciences (CAS), Ningbo, 315201, China

    Ali Saad, Zhixing Cheng, Hangjia Shen & Minghui Yang

  2. Department of Metallurgical and Materials Engineering, Indian Institute of Technology Madras, Adyar, Chennai, Tamil Nadu, 600036, India

    Tiju Thomas

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  1. Ali Saad
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  2. Zhixing Cheng
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  3. Hangjia Shen
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  4. Tiju Thomas
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  5. Minghui Yang
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Correspondence to Tiju Thomas or Minghui Yang.

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Saad, A., Cheng, Z., Shen, H. et al. Recent Advances in Nanocasting Cobalt-Based Mesoporous Materials for Energy Storage and Conversion. Electrocatalysis 11, 465–484 (2020). https://doi.org/10.1007/s12678-020-00608-9

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