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Characterization and source identification of ambient VOCs in Jinan, China

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Abstract

For 2 years, the concentrations and variance of 56 VOCs were continuously monitored with an on-line gas chromatography and the data were analyzed to characterize the local volatile organic compounds (VOCs) in the atmosphere and identify the major sources of the pollutants. The abundant VOCs were found to consist of C3~C5 alkanes, propylene, cis-2-butene, toluene, and m/p-xylene. The results showed that the seasonal average concentrations of VOCs followed in decreasing order: summer > winter > autumn > spring. In summer, the alkane pollution was the most severe. The diurnal variation of alkanes, alkenes, and VOCs showed a bimodal distribution with two peaks, one in the morning and one in the evening. This profile was consistent with local traffic rush hours, and the average hourly toluene/benzene ratio was less than two. Based on the principal component analysis (PCA), it was found that the major sources of VOCs were consistent with automobile exhaust, industry, and biomass combustion in this study.

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References

  • Bergin MH, Cass GR, Xu J, Fang C, Zeng LM, Yu T, Salmon LG, Kiang CS, Tang XY, Zhang YH (2001) Aerosol radiative, physical, and chemical properties in Beijing during June 1999. J Geophys Res Atmos 106:17969–17980

    Article  CAS  Google Scholar 

  • Cai CJ, Geng FH, Tie XX, Yu Q, Peng L, Zhou GQ (2010) Characteristics of ambient volatile organic compounds (VOCs) measured in Shanghai, China. Sensors 10:7843–7862

    Article  CAS  Google Scholar 

  • Cerón-Bretón JG, Cerón-Bretón RM, Kahl JDW, Ramírez-Lara E, Guarnaccia C, Aguilar-Ucán CA, Montalvo-Romero C, Anguebes-Franseschi F, López-Chuken U (2014) Diurnal and seasonal variation of BTEX in the air of monterrey, Mexico: preliminary study of sources and photochemical ozone pollution. Air Qual Atoms Health. doi:10.1007/s11869-014-0296-1

    Google Scholar 

  • Chan LY, Chu KW, Zou SC, Chan CY, Wang XM, Barletta B, Blake DR, Guo H, Tsai WY (2006) Characteristics of nonmethane hydrocarbons (NMHCs) in industrial, industrial–urban, and industrial–suburban atmospheres of the pearl river delta (PRD) region of south China. J Geophys Res Atmos. doi:10.1029/2005JD006481

    Google Scholar 

  • Das M, Aneja VP (2003) Regional analysis of nonmethane volatile organic compounds in the lower troposphere of the Southeast United States. J Environ Sci 129:1085–1103

    CAS  Google Scholar 

  • Derwent RG, Jenkin ME, Saunders SM, Pilling MJ, Simmonds PG, Passant NR, Dollard GJ, Dumitrean P, Kent A (2003) Photochemical ozone formation in north west Europe and its control. Atmos Environ 37:1983–1991

    Article  CAS  Google Scholar 

  • Guo H, Wang T, Blake DR, Simpson IJ, Kwok YH, Li YS (2006) Regional and local contributions to ambient non-methane volatile organic compounds at a polluted rural/coastal site in Pearl River Delta, China. Atmos Environ 40:2345–2359

    Article  CAS  Google Scholar 

  • Jacobson MC, Hansson HC, Noone KJ, Charlson RJ (2000) Organic atmospheric aerosols: review and state of the science. Rev Geophys 38:267–294

    Article  CAS  Google Scholar 

  • Jia C, Batterman S, Godwin C (2008) VOCs in industrial, urban and suburban neighborhoods, part 1: indoor and outdoor concentrations, variation, and risk drivers. Atmos Environ 42:2083–2100

    Article  CAS  Google Scholar 

  • Kumar A, Tyagi SK (2006) Benzene and toluene profiles in ambient air of Delhi as determined by active sampling and GC analysis. J Sci India Res India 65:252–257

    CAS  Google Scholar 

  • Laaksonen A, Kulmala M, O’Dowd CD, Joutsensaari J, Vaattovaara P, Mikkonen S, Lehtinen KEJ, Sogacheva L, Maso MD, Aalto P (2008) The role of VOC oxidation products in continental new particle formation. Atmos Chem Phys 8:2657–2665

    Article  CAS  Google Scholar 

  • Liu Y, Shao M, Fu L, Lu S, Zeng L, Tang D (2008a) Source profiles of volatile organic compounds (VOCs) measured in China: part I. Atmos Environ 42:6247–6260

    Article  CAS  Google Scholar 

  • Liu Y, Shao M, Lu S, Chang C-C, Wang J-L, Chen G (2008b) Volatile organic compound (VOC) measurements in the pearl river delta (PRD) region, China. Atmos Chem Phys 8:1531–1545

    Article  CAS  Google Scholar 

  • Lu SH, Bai YH, Chen YK, Zhao J, Wang ZH (2003) The characteristics of volatile organic compounds (VOCs) emitted from motor vehicle in Beijing. China Environ Sci 23:127–130

    Google Scholar 

  • Niu Z, Zhang H, Xu Y, Liao X, Xu L, Chen J (2012) Pollution characteristics of volatile organic compounds in the atmosphere of Haicang District in Xiamen City, Southeast China. J Environ Monitor 14:1144–1151

    CAS  Google Scholar 

  • Pekey H, Arslanbaş D (2008) The relationship between indoor, outdoor and personal VOC concentrations in homes, offices and schools in the metropolitan region of Kocaeli, Turkey. Water Air Soil Pollut 191:113–129

    Article  CAS  Google Scholar 

  • Rehwagen M, Schlink U, Herbarth O (2003) Seasonal cycle of VOCs in apartments. Indoor Air 13:283–291

    Article  CAS  Google Scholar 

  • Shi J, Deng H, Bai Z, Kong S, Wang X, Hao J, Han X, Ning P (2015) Emission and profile characteristic of volatile organic compounds emitted from coke production, iron smelt, heating station and power plant in Liaoning Province, China. Sci Total Environ 515:101–108

    Article  Google Scholar 

  • Steinemann A (2015) Volatile emissions from common consumer products. Air Qual Atoms Health. doi:10.1007/s11869-015-0327-6

    Google Scholar 

  • Stock TH, Chung KC, Smith T, Alesch A, Swift J, Afshar M (2010) Investigation of spatial and seasonal variation of VOCs at the Ysleta del Sur Pueblo American Indian nation. Air Qual Atoms Health 3:213–224

    Article  CAS  Google Scholar 

  • Tiwari V, Hanai Y, Masunaga S (2010) Ambient levels of volatile organic compounds in the vicinity of petrochemical industrial area of Yokohama, Japan. Air Qual Atoms Health 3:65–75

    Article  CAS  Google Scholar 

  • Toro R, Seguel RJ (2014) Ozone, nitrogen oxides, and volatile organic compounds in a central zone of Chile. Air Qual Atoms Health. doi:10.1007/s11869-014-0306-3

    Google Scholar 

  • Tsai SM, Zhang J, Smith KR, Ma Y, Rasmussen RA, Khalil MAK (2003) Characterization of non-methane hydrocarbons emitted from various cookstoves used in China. Environ Sci Technol 37:2869–2877

    Article  CAS  Google Scholar 

  • Tsigaridis K, Kanakidou M (2007) Secondary organic aerosol importance in the future atmosphere. Atmos Environ 41:4682–4692

    Article  CAS  Google Scholar 

  • Watson JG, Chow JC, Fujita EM (2001) Review of volatile organic compound source apportionment by chemical mass balance. Atmos Environ 35:1567–1584

    Article  CAS  Google Scholar 

  • Wei W, Cheng S, Li G, Wang G, Wang H (2014) Characteristics of volatile organic compounds (VOCs) emitted from a petroleum refinery in Beijing, China. Atmos Environ 89:358–366

    Article  CAS  Google Scholar 

  • Zheng J, Shao M, Che W, Zhang L, Zhong L, Zhang Y, Streets D (2009) Speciated VOC emission inventory and spatial patterns of ozone formation potential in the Pearl River Delta, China. Environ Sci Technol 43:8580–8586

    Article  CAS  Google Scholar 

  • Zheng J, Yu Y, Mo Z, Zhang Z, Wang X, Yin S, Peng K, Yang Y, Feng X, Cai H (2013) Industrial sector-based volatile organic compound (VOC) source profiles measured in manufacturing facilities in the Pearl River Delta, China. Sci Total Environ 456:127–136

    Article  Google Scholar 

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Acknowledgments

This work was supported by the National Science Foundation of China Funding Agency [Grant No. 21407097] and the Doctoral Research Foundation at Shandong Jianzhu University [Grant No. 000601485]. Dr. Eric A. Evans from HDR Engineering is appreciated for the preparation of the paper.

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Authors and Affiliations

  1. School of Municipal and Environmental Engineering, Shandong Jianzhu University, Jinan, 250101, China

    Zechang Liu, Na Li & Ning Wang

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  1. Zechang Liu
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  2. Na Li
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  3. Ning Wang
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Correspondence to Ning Wang.

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Liu, Z., Li, N. & Wang, N. Characterization and source identification of ambient VOCs in Jinan, China. Air Qual Atmos Health 9, 285–291 (2016). https://doi.org/10.1007/s11869-015-0339-2

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