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Radon diffusion and exhalation from mortar modified with fly ash: waste utilization and benefits in construction

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Abstract

The utilization of fly ash in construction and cement industry increases from last few decades. But the question on utilization of fly ash for construction purpose was raised by many investigators as it causes a source of radioactive gas radon and increase in the gamma dose. In order to optimize the utilization of fly ash in cement with additional benefit of reducing radon diffusion coefficient and exhalation rate were studied. The compressive strength of mortar is the key factor for cement industry, thus it should not be sacrificed for utilization of fly ash. Keeping this in mind, compressive strength, porosity, radon diffusion and exhalation rate study was carried out through the mortar reinforced with the blending of fly ash with cement. The results indicated decrease in effective radon diffusion coefficient from 0.363 × 10−7 to 0.013 × 10−7 m2/s for fly ash up to 50 % substitution. The addition of fly ash in cement first decreased the radon exhalation rates up to 25 % substitution then increases and similar trends were observed for compressive strength. Thus, the addition of fly ash exerts a positive effect up to a 20–25 % replacement beyond which it may introduce negative effect depending upon the level of substitution.

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References

  1. WHO (2009) Handbook on Indoor Radon, The World Health Organization

  2. Bajwa BS, Singh H, Singh J, Singh S (2009) A comparative study of indoor radon levels and inhalation dose in some areas of Punjab and Haryana, India. Indian J Phys 83:1183–1189

    Article  Google Scholar 

  3. Haucke F (2010) The cost effectiveness of radon mitigation in the existing German dwellings—a decision theoretical analysis. J Environ Manage 91:2263–2274

    Article  Google Scholar 

  4. Menetrez MY, Mosley RB, Snoddy R, Brubaker SA Jr (1996) Evaluation of radon emanation from soil with varying moisture content in a soil chamber. Environ Int 22:447–453

    Article  Google Scholar 

  5. Darby S, Hill D, Auvinen A, Barros-Dios JM, Baysson H, Bochicchio F (2005) Radon in homes and risk of lung cancer: collaborative analysis of individual data from European case–control studies. Br Med J 330:223–226

    Article  Google Scholar 

  6. BEIR-VI (1999) National Research Council Biological Effects of Ionizing Radiation (BEIR) VI Report. Health Effects of Exposure to Radon. National Academy Press, Washington

    Google Scholar 

  7. Sahoo BK, Sapra BK, Gaware JJ, Kanse SD, Mayya YS (2011) A model to predict radon exhalation from walls to indoor air based on the exhalation from building material samples. Sci Total Environ 409:2635–2641

    Article  Google Scholar 

  8. Petersen ML, Larsen T (2006) Cost benefit analyses of radon mitigation projects. J Environ Manage 81:19–26

    Article  Google Scholar 

  9. Denman AR, Phillips PS, Tornberg R (2000) A comparison of the cost and benefit of radon remediation programmes in new and existing house in Northamptonshaire. J Environ Manage 59:21–30

    Article  Google Scholar 

  10. Narula AK, Goyal SK, Saini S, Chauhan RP, Charkarvarti SK (2009) Calculation of radon diffusion coefficient and diffusion length for different building construction materials. Indian J Phys 83:1171–1175

    Article  Google Scholar 

  11. Jiranek M, Rovenska K (2012) Basic principles for the development of a common standardized method for determining the radon diffusion coefficient in waterproofing materials. Appl Radiat Isot 70:752–757

    Article  Google Scholar 

  12. Cozmuta I, Vander Graaf ER, (1999) Methods for measuring diffusion coefficients of radon in building materials. KVI Report R105, Kernfysisch Vernsneller Institut, Groningen, The Netherlands

  13. Nielson K, Rich D, Rogers V, Kalkwarf D (1982) Comparison of radon diffusion coefficients measured by transient diffusion and steady state laboratory methods. Nuclear Regulatory Commission Report NUREG/CR: 2875

  14. Daoud WZ, Renken KJ (2001) Laboratory assessment of flexible thin-film membranes as a passive barrier to radon gas diffusion. Sci Total Environ 272:127–135

    Article  Google Scholar 

  15. Keller G, Hoffmann B, Feigenspan T (2001) Radon permeability and radon exhalation of building materials. Sci Total Environ 272:85–89

    Article  Google Scholar 

  16. Burke AK, Stancato AC, Paulon VA, Guedes S, Hadler JC (2003) Study of radon emanation from polymer-modified cementitious materials. Build Environ 38:1291–1295

    Article  Google Scholar 

  17. Yu KN (1994) Mitigation of indoor radon pollution in buildings in Hong Kong: covering materials on internal building surfaces. Build Environ 29:1–3

    Article  Google Scholar 

  18. Adler PM, Perrier F (2009) Radon emanation in partially saturated porous media. Transp Porous Media 78:149–159

    Article  Google Scholar 

  19. Jiránek M, Kotrbatá M (2011) Radon diffusion coefficient in 360 waterproof materials of different chemical composition authors. Radiat Prot Dosimetry 145:178–183

    Article  Google Scholar 

  20. Camilleri J, Sammut M, Montesin FE (2006) Utilization of pulverized fuel ash in Malta. Waste Manag 26:853–860

    Article  Google Scholar 

  21. Telesca A, Marroccoli M, Calabrese D, Gl Valenti, Montagnaro F (2013) Flue gas desulfurization gypsum and coal fly ash as basic components of prefabricated building materials. Waste Manag 33:628–633

    Article  Google Scholar 

  22. Rajagopalan V (1999) Ministry of Environment and forests, The Gazette of India. Extraordinary Part II, F No.16-2/95-HSMD

  23. CEA (2011) Report on fly ash generation at coal/lignite based thermal power stations and its utilization in the country for the year 2010–11

  24. Ashtiani MS, Scott AN, Dhakal RP (2013) Mechanical and fresh properties of high-strength self-compacting concrete containing class C fly ash. Constr Build Mater 47:1217–1224

    Article  Google Scholar 

  25. Sukumar B, Nagamani K, Raghavan RS (2008) Evaluation of strength at early ages of self-compacting concrete with high volume fly ash. Constr Build Mater 22:1394–1401

    Article  Google Scholar 

  26. Flues M, Camargo IMC, Silva PSC, Mazzilli BP (2006) Radioactivity of coal and ashes from Figueira coal power plant in Brazil. J Radioanal Nucl Chem 270:597–602

    Article  Google Scholar 

  27. Papastefanou C (2006) Radioactivity of coals and fly ashes. J Radio Anal Nucl Chem 275:29–35

    Article  Google Scholar 

  28. Chauhan RP, Kant K, Sharma SK, Chakarvarti SK (2003) Measurement of alpha radioactive air pollutants in fly ash brick dwellings. Radiat Meas 36:533–536

    Article  Google Scholar 

  29. Kovler K (2012) Does the utilization of coal fly ash in concrete construction present a radiation hazard? Constr Build Mater 29:158–166

    Article  Google Scholar 

  30. ASTM Designation, C191, Standard method for normal consistency and setting of hydraulic cement, ASTM Annual Book of ASTM Standards, 2008

  31. Chen CG, Sun CG, Gau SH, Wu CW, Chen YL (2013) The effects of the mechanical–chemical stabilization process for municipal solid waste incinerator fly ash on the chemical reactions in cement paste. Waste Manag 33:858–865

    Article  Google Scholar 

  32. Chauhan RP, Kumar A (2013) Radon resistant potential of concrete manufactured using Ordinary Portland Cement blended with rice husk ash. Atmos Environ 81:413–420

    Article  Google Scholar 

  33. Oufni F (2003) Determination of the radon diffusion coefficient and radon exhalation rate in Moroccan quaternary samples using the SSNTD technique. J Radioanal Nucl Chem 256:581–586

    Article  Google Scholar 

  34. Cozmuta I, Vander Graaf ER (2001) Methods for measuring diffusion coefficients of radon in building materials. Sci Total Environ 272:23–335

    Article  Google Scholar 

  35. Jiranek M, Hulka J (2001) Applicability of various insulating materials for radon barriers. Sci Total Environ 272:79–84

    Article  Google Scholar 

  36. Gaware JJ, Sahoo BK, Sapra BK, Mayya YS (2011) Indigenous development and networking of online radon monitors in the underground uranium mine. Radiat Prot Environ 34:37–40

    Google Scholar 

  37. Fornier F, Groetz JE, Jacob F, Crolet JM, Lettner H (2005) Simulation of radon transport through building materials: influence of the water content on radon exhalation rate. Transp Porous Media 59:197–214

    Article  Google Scholar 

  38. Chindaprasirt P, Rukzon S (2008) Strength, porosity and corrosion resistance of ternary blend Portland cement, rice husk ash and fly ash mortar. Constr Build Mater 22:1601–1606

    Article  Google Scholar 

  39. Stoulos S, Manolopoulou M, Papastefanou C (2003) Assessment of natural radiation exposure and radon exhalation from building materials in Greece. J Environ Radioact 69:225–240

    Article  Google Scholar 

  40. Taylor-Lange SC, Juenger MCG, Siegel JA (2014) Radon emanation fractions from concretes containing fly ash and metakaolin. Sci Total Environ 466–467:1060–1065

    Article  Google Scholar 

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Acknowledgments

The authors are thankful to Board of Research in Nuclear Science, Department of Atomic Energy, Mumbai, India, for providing instruments for the present work. The help received from Civil Engineering Department, National Institute of Technology, Kurukshetra, India, is also thankfully acknowledged.

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  1. Department of Physics, National Institute of Technology, Kurukshetra, 136119, India

    Amit Kumar & R. P. Chauhan

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  1. Amit Kumar
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  2. R. P. Chauhan
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Correspondence to Amit Kumar.

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Kumar, A., Chauhan, R.P. Radon diffusion and exhalation from mortar modified with fly ash: waste utilization and benefits in construction. J Mater Cycles Waste Manag 19, 318–325 (2017). https://doi.org/10.1007/s10163-015-0424-5

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  • DOI: https://doi.org/10.1007/s10163-015-0424-5

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