Skip to main content
Log in

Polar Fe(IO3)3 nanocrystals as local probes for nonlinear microscopy

  • Published:
Applied Physics B Aims and scope Submit manuscript

Abstract

We have investigated nanocrystals of Fe(IO3)3 by polarization-sensitive second harmonic generation (SHG) microscopy. As the nonlinear optical properties of this material were only poorly characterized, we have first determined the relative values of the elements of its second-order susceptibility tensor, by the global fitting of the polarization-resolved SHG response of an ensemble of nanocrystals. This information allows one to optically retrieve the orientation of individual particles in the sample. The high SHG efficiency measured for nanocrystals of Fe(IO3)3 and their polar nature could make them very attractive for nonlinear microscopy of biological samples.

This is a preview of subscription content, log in via an institution to check access.

Access this article

Price excludes VAT (USA)
Tax calculation will be finalised during checkout.

Instant access to the full article PDF.

Similar content being viewed by others

References

  1. J.I. Dadap, J. Shan, K.B. Eisenthal, T.F. Heinz, Phys. Rev. Lett. 83, 4045 (1999)

    Article  ADS  Google Scholar 

  2. J. Mertz, L. Moreaux, Opt. Commun. 196, 325 (2001)

    Article  ADS  Google Scholar 

  3. Y. Pavlyukh, W. Hubner, Phys. Rev. B 70, 245434 (2004)

    Article  ADS  Google Scholar 

  4. K. Nappa, I. Russier-Antoine, E. Benichou, C. Jonin, P.F. Brevet, Chem. Phys. Lett. 415, 246 (2005)

    Article  ADS  Google Scholar 

  5. J. Nappa, G. Revillod, I. Russier-Antoine, E. Benichou, C. Jonin, P.F. Brevet, Phys. Rev. B 71, 165407 (2005)

    Article  ADS  Google Scholar 

  6. M.L. Sandrock, C.D. Pibel, F.M. Geiger, C.A. Foss, J. Phys. Chem. B 103, 2668 (1999)

    Article  Google Scholar 

  7. S.W. Chan, R. Barille, J.M. Nunzi, K.H. Tam, Y.H. Leung, W.K. Chan, A.B. Djurisic, Appl. Phys. B 84, 351 (2006)

    Article  ADS  Google Scholar 

  8. J.C. Johnson, H. Yan, R.D. Schaller, P.B. Petersen, P. Yang, R.J. Saykally, Nano Lett. 2, 279 (2002)

    Article  ADS  Google Scholar 

  9. Y.Z. Shen, P. Markowicz, J. Winiarz, J. Swiatkiewicz, P.N. Prasad, Opt. Lett. 26, 725 (2001)

    Article  ADS  Google Scholar 

  10. S. Brasselet, V. Le Floc’h, F. Treussart, J.F. Roch, J. Zyss, E. Botzung-Appert, A. Ibanez, Phys. Rev. Lett. 92, 207401 (2004)

    Article  ADS  Google Scholar 

  11. L. Moreaux, O. Sandre, J. Mertz, J. Opt. Soc. Am. B 17, 1685 (2000)

    Article  ADS  Google Scholar 

  12. L. Cognet, Lasers et Technologies Femtosecondes, 1st edn. (Publications de l’Université, Saint-Etienne, 2005)

  13. G.S. Harms, L. Cognet, P.H.M. Lommerse, G.A. Blab, T. Schmidt, Biophys. J. 80, 2396 (2001)

    Article  Google Scholar 

  14. M. Nirmal, B.O. Dabbousi, M.G. Bawendi, J.J. Macklin, J.K. Trautman, T.D. Harris, L.E. Brus, Nature 383, 802 (1996)

    Article  ADS  Google Scholar 

  15. X. Brokmann, J.P. Hermier, G. Messin, P. Desbiolles, J.P. Bouchaud, M. Dahan, Phys. Rev. Lett. 90, 120601 (2003)

    Article  ADS  Google Scholar 

  16. R.M. Williams, W.R. Zipfel, W.W. Webb, Curr. Opin. Chem. Biol. 5, 603 (2001)

    Article  Google Scholar 

  17. J. Mertz, Curr. Opin. Neurobiol. 14, 610 (2004)

    Google Scholar 

  18. J.M. Dela Cruz, I. Pastirk, M. Comstock, V.V. Lozovoy, M. Dantus, Proc. Nat. Acad. Sci. USA 101, 16996 (2004)

    Article  ADS  Google Scholar 

  19. C. Galez, Y. Mugnier, J. Bouillot, Y. Lambert, R. Le Dantec, J. Alloys Compd. 416, 261 (2006)

    Article  Google Scholar 

  20. K. Komorowska, S. Brasselet, G. Dutier, I. Ledoux, J. Zyss, L. Poulsen, M. Jazdzyk, H. Egelhaaf, J. Gierschner, M. Hanack, Chem. Phys. 318, 12 (2005)

    Article  ADS  Google Scholar 

  21. J.P. Jolivet, C. Froidefond, A. Pottier, C. Chaneac, S. Cassaignon, E. Tronc, P. Euzen, J. Mater. Chem. 14, 3281 (2004)

    Article  Google Scholar 

  22. K. Nassau, J.W. Shiever, B.E. Prescott, J. Solid State Chem. 7, 186 (1973)

    Article  ADS  Google Scholar 

  23. S.C. Abrahams, R.C. Sherwood, J.L. Bernstein, K. Nassau, J. Solid State Chem. 7, 205 (1973)

    Article  ADS  Google Scholar 

  24. R.L. Sutherland, Handbook of Nonlinear Optics, 2nd edn. (Marcel Dekker, London, 2003)

  25. E.Y.S. Yew, C.J.R. Sheppard, Opt. Express 14, 1167 (2006)

    Article  ADS  Google Scholar 

  26. J.X. Cheng, X.S. Xie, J. Opt. Soc. Am. B 19, 1604 (2002)

    Article  ADS  Google Scholar 

  27. W. Débarre, D. Supatto, E. Beaurepaire, Opt. Lett. 30, 2134 (2005)

    Article  ADS  Google Scholar 

  28. M. Siltanen, S. Cattaneo, E. Vuorimaa, H. Lemmetyinen, T.J. Katz, K.E.S. Phillips, M. Kauranen, J. Chem. Phys. 121, 1 (2004)

    Article  ADS  Google Scholar 

  29. E. Delahaye, N. Tancrez, T. Yi, I. Ledoux, J. Zyss, S. Brasselet, R. Clément, Chem. Phys. Lett. 429, 533 (2006)

    Article  ADS  Google Scholar 

Download references

Author information

Authors and Affiliations

Authors

Corresponding author

Correspondence to Y. Mugnier.

Additional information

PACS

42.70.Mp; 78.67.Bf

Rights and permissions

Reprints and permissions

About this article

Cite this article

Bonacina, L., Mugnier, Y., Courvoisier, F. et al. Polar Fe(IO3)3 nanocrystals as local probes for nonlinear microscopy. Appl. Phys. B 87, 399–403 (2007). https://doi.org/10.1007/s00340-007-2612-z

Download citation

  • Received:

  • Published:

  • Issue Date:

  • DOI: https://doi.org/10.1007/s00340-007-2612-z

Keywords

Navigation