Abstract
This study concerns the concentrations of particulates in ambient air, dry deposited particulates, particulate-bound mercury (Hg(p)), and Hg(p) that is dry deposited in both total suspended particulates and on a dry deposition plate at Long Cyuan Elementary School (LCYES), Lung Ching Elementary School (LCHES), and Long Shan Primary School (LSPS) in Longjing. The LCHES site had the highest particulate Hg(p) concentrations in October and November, and the least dry deposition of particulates in October. The LSPS site had the lowest Hg(p) dry depositions in October. The LCYES site had the lowest particulate and Hg(p) concentrations in November and October, and had the highest dry deposition of particulates and Hg(p) in November and December. These particulates originated from the northwest of Taiwan and were transported by way of mainland China in October. A back trajectory analysis supported this finding. Therefore, particulate concentrations in ambient air were highest in October and the major sources of particulate-bound mercury Hg(p) in ambient air were in mainland China, especially in October and December. Mainland China and Taichung Thermal Power Plant were the main sources of particles and Hg(p) in ambient air.
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References
AMAP/UNEP (2013) Technical background report for the Global Mercury Assessment 2013 Arctic Monitoring and Assessment Programme, Oslo, Norway/UNEP Chemicals Branch Geneva, Switzerland
Amos HM, Jacob DJ, Streets DG, Sunderland EM (2013) Legacy impacts of all-time anthropogenic emissions on the global mercury cycle. Glob Biogeochem Cycles 27:410–421
Bergan T, Gallardo L, Rodhe H (1999) Mercury in the global troposphere: a three-dimensional model study. Atmos Environ 33:1575–1585
Choi EM, Kim SH, Holsen TM, Yi SM (2009) Total gaseous concentrations in mercury in Seoul, Korea: local sources compared to long-range transport from China and Japan. Environ Pollut 157(3):816–822
Clarkson TW (1993) Mercury: major issues in environmental health. Environ Health Perspect 100:31–38
Dockery DW, Pope CA III, Xu X, Spengler JD, Ware JH, Fay ME, Ferris BG Jr, Speizer FE (1993) An association between air pollution and mortality in six U.S. cities. N Engl J Med 329:1753–1759
Draxler RR (1999) HYSPLIT4 user’s guide. NOAA Tech. Memo. ERL ARL-230, NOAA Air Resources Laboratory, Silver Spring
Facemire C, Augspurger T, Bateman D, Brim M, Conzelmann P, Delchamps S, Douglas E, Inmon L, Looney K, Lopez F, Mason, Morrison D, Morse N, Robison A (1995) Impacts of mercury contamination in the southeastern United States. Water Air Soil Pollut 80:923–932
Fang GC, Cheng MT, Chang CN (1997) Monitoring and modeling the mass, heavy metal and ion species dry deposition in central Taiwan. J Environ Sci Health A 32(8):2183–2199
Fang GC, Lin SJ, Chang SY, Chou CCK (2009a) Effect of typhoon on atmospheric particulates in autumn in central Taiwan. Atmos Environ 43(38):6039–6048
Fang GC, Basu N, Nam DH, Yang IL (2009b) Characterization of ambient air particulates and particulate mercury at Sha-Lu, Central Taiwan. Environ Forensics 10(4):277–285
Fang GC, Yang IL, Liu CK (2010) Measure and modeling the ambient air particles and particle bound mercury Hg(p) at a traffic sampling site. Atmos Res 97(1–2):97–105
Fu X, Feng X, Sommar J, Wang S (2012) A review of studies on atmospheric mercury in China. Sci Total Environ 421:73–81
Han YJ, Kim JE, Kim PR, Kim WJ, Yi SM, Seo YS, Kim SH (2014) General trends of atmospheric mercury concentrations in urban and rural areas in Korea and characteristics of high-concentration events. Atmos Environ 94:754–764
Kelly FJ (2003) Oxidative stress: its role in air pollution and adverse health effects. Occup Environ Med 60:612–616
Laks DR (2010) Luteinizing hormone provides a causal mechanism for mercury associated disease. Med Hypotheses. 74(4): 698-701. http://www.medicinenet.com/mercury_poisoning/article.htm. Accessed 26 April 2015
Meyer MW, Evers DC, Daulton T, Braselton WE (1995) Common loons (Gavia immer) nesting on low pH lakes in northern Wisconsin have elevated blood mercury content. Water Air Soil Pollut 80:871–880
Pacyna EG, Pacyna JM, Sundseth K, Munthe J, Kindbom K, Wilson S, Steenhuisen F, Maxson P (2010) Global emission of mercury to the atmosphere from anthropogenic sources in 2005 and projections to 2020. Atmos Environ 44:2487–2499
Parran DK, Barone S Jr, Mundy WR (2003) Methyl mercury decreases NGF-induced TrkA autophosphorylation and neurite outgrowth in PC12 cells. Dev Brain Res 141(1–2):71–81
Pope CA III, Burnett RT, Thun MJ, Calle EE, Krewski D, Ito K, Thurston GD (2002) Lung cancer, cardiopulmonary mortality, and long-term exposure to fine particulate air pollution. J Am Med Assoc 287:1132–1141
Sakata M, Marumoto K (2002) Formation of atmospheric particulate mercury in the Tokyo metropolitan area. Atmos Environ 36(2):239–246
Schleicher NJ, Schäfer J, Blanc G, Chen Y, Chai F, Cen K, Norra S (2015) Atmospheric particulate mercury in the megacity Beijing: Spatio-temporal variations and source apportionment. Atmos Environ (in Press)
Seigneur C, Vijayaraghavan K, Lohman K, Karamchandani P, Scott C (2004) Global source attribution for mercury deposition in the United States. Environ Sci Technol 38:555–569
Selin NE (2009) Global biogeochemical cycling of mercury: a review. Annu Rev Environ Resour 34:43–63
Shafer TJ, Meacham CA, Barone S Jr (2002) Effects of prolonged exposure to nanomolar concentrations of methylmercury on voltage-sensitive sodium and calcium currents in PC12 cells. Dev Brain Res 136(2):151–164
Szücs A, Angiello C, Salánki J, Carpenter DO (1997) Effects of inorganic mercury and methylmercury on the ionic currents of cultured rat hippocampal neurons. Cell Mol Neurobiol 17(3):273–288
Tarabova B, Kurejova M, Sulova Z, Drabova M, Lacinova L (2006) Inorganic mercury and methyl mercury inhibit the Cav3.1 channel expressed in human embryonic kidney 293 cells by different mechanisms. J Pharmacol Exp Ther 317:418–427
Wang L, Wang SX, Zhang L, Wang YX, Zhang YX, Nielsen C, McElroy MB, Hao JM (2014) Source apportionment of atmospheric mercury pollution in China using the GEOS-Chem model. Environ Pollut 190:166–175
Wong CSC, Duzgoren-Aydin NS, Aydin A, Wong MH (2006) Sources and trends of environmental mercury emissions in Asia. Sci Total Environ 368(2–3):649–662
Wu Y, Wang SX, Streets DG, Hao JM, Chan M, Jiang JK (2006) Trends in anthropogenic mercury emissions in China from 1995 to 2003. Environ Sci Technol 40:5312–5318
Yoshino Y, Mozai T, Nakao K (1966) Biochemical changes in the brain in rats poisoned with an alky mercury compound, with special reference to the inhibition of protein synthesis in brain cortex slices. J Neurochem 13:1223–1230
Zhang X, Siddiqi Z, Song X, Mandiwana KL, Yousafa M, Lu J (2012) Atmospheric dry and wet deposition of mercury in Toronto. Atmos Environ 50:60–65
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The authors gratefully acknowledge the National Science Council of the ROC (Taiwan) for financially supporting this work under Project no. 103-2221-E-241 -004 -MY3.
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Fang, GC., Lo, CT., Zhuang, YJ. et al. Sources of ambient air particulates and Hg(p) pollutants at Freeway, Industrial, Thermal power plant F.I.T. characteristic sites. Environ Earth Sci 75, 103 (2016). https://doi.org/10.1007/s12665-015-5057-4
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DOI: https://doi.org/10.1007/s12665-015-5057-4