Skip to main content
Log in

Mechanical and Biodegradable Properties of Jute/Flax Reinforced PLA Composites

  • Regular Article
  • Published:
Fibers and Polymers Aims and scope Submit manuscript

Abstract

Green composites possessing biodegradable or recyclable characteristics have gained interest in recent years due to their ecofriendly, sustainable and lightweight characteristics over the conventional plastic-based materials. In this study, flax and jute natural fibers have been used individually and as hybrid reinforcement into Poly Lactic Acid (PLA) matrix. The composites developed are suitable to be used in biodegradable products in packaging and automobile industries. Hot press compression molding was used to fabricate samples of PLA/flax, PLA/jute and PLA/flax/jute (hybrid composites). The concentration of natural fibers in individual fiber-based composites was varied (between 0–50 %) by weight to investigate its effect on tensile and impact properties. Maximum tensile properties were obtained for 40 wt% single-fiber reinforced into PLA. This reinforcement content (40 wt%) was used as reference for hybrid composites. Hybrid composites were fabricated with different combinations of jute and flax fibers by keeping the total concentration of reinforcement equal to 40 % by weight. Tensile and Charpy impact tests were performed to evaluate the mechanical properties of the composites. Scanning Electron Microscopy of the tensile fractured surfaces was performed to observe the failure mechanism and adhesion at fibermatrix interfaces in the composites. Further characterizations included Fourier Transform Infra-Red spectroscopy and Biodegradability tests, which were performed according to ASTM standards. Fourier Transform Infrared analysis revealed interaction between the natural fibers (jute and flax) and PLA matrix in hybrid composites. The enhanced interaction in hybrid composites resulted in their improved impact resistance. Based on the results obtained in this study, the improved mechanical and biodegradable properties of these composites make it suitable for use in applications like food-packaging and indoor plastic products in automobiles, to reduce synthetic plastic pollution.

This is a preview of subscription content, log in via an institution to check access.

Access this article

Price excludes VAT (USA)
Tax calculation will be finalised during checkout.

Instant access to the full article PDF.

Similar content being viewed by others

References

  1. Z. Sun, L. Zhang, D. Liang, W. Xiao, and J. Lin, Int. J. Polym. Sci., 2017, 1 (2017).

    Google Scholar 

  2. R. M. Bajracharya, D. S. Bajwa, and S. G. Bajwa, Procedia Eng., 200, 370 (2017).

    Article  CAS  Google Scholar 

  3. R. Ranjan, P. K. Bajpai, and R. K. Tyagi, Eng. Int., 1, 39 (2013).

    Article  Google Scholar 

  4. K. Okubo, T. Fujii, and E. T. Thostenson, Compos Part A-Appl. S., 40, 469 (2009).

    Article  Google Scholar 

  5. E. Hassan, Y. Wei, H. Jiao, and Y. M. Huo, Int. J. Eng. Sci. Technol., 4 (2012).

  6. P. K. Bajpai, I. Singh, and J. Madaan, J. Thermoplast., 27, 52 (2012).

    Article  Google Scholar 

  7. C. Nyambo, A. K. Mohanty, and M. Misra, Biomacromolecules, 11, 1654 (2010).

    Article  CAS  Google Scholar 

  8. Y. Cheng, S. Deng, P. Chen, and R. Ruan, Front. Chem. China, 4, 259 (2009).

    Article  Google Scholar 

  9. R. Mehta, V. Kumar, H. Bhunia, and S. N. Upadhyay, J. Macromol. Sci., Polym. Rev., 45, 325 (2005).

    Article  Google Scholar 

  10. M. S. Huda, L. T. Drzal, M. Misra, A. K. Mohanty, K. Williams, and D. F. Mielewski, Ind. Eng. Chem. Res., 44, 5593 (2005).

    Article  CAS  Google Scholar 

  11. I. Widiastuti, Ph. D. Dissertation, IRIS, Melbourne, 2014.

  12. R. Siakeng, M. Jawaid, H. Ariffin, S. M. Sapuan, M. Asim, and N. Saba, Polym. Compos., 40, 446 (2018).

    Article  Google Scholar 

  13. A. Sangregorio, N. Guigo, J. C. van der Waal, and N. Sbirrazzuoli, Compos. Sci. Technol., 171, 70 (2019).

    Article  CAS  Google Scholar 

  14. A. Q. Dayo, A. A. Babar, Q.-R. Qin, S. Kiran, J. Wang, A. H. Shah, A. Zegaoui, H. A. Ghouti, and W.-B. Liu, Compos. Part A-Appl. S., 128 (2019).

  15. F. A. T. Owolabi, A. G. Deepu, T. Sabu, J. Shima, R. Samsul, N. A. Sri Aprilia, and H. P. S. Abdul Khalil, “Encyclopedia of Renewable and Sustainable Materials”, 1st ed. (S. Hashmi and I. A. Choudhary Eds.), pp.81–94, Elsevier Science, 2020.

  16. W. Liu, T. Chen, M.-E. Fei, R. Qiu, D. Yu, T. Fu, and J. Qiu, Compos. Part B-Eng., 171, 87 (2019).

    Article  CAS  Google Scholar 

  17. V. Mazzanti, R. Pariante, A. Bonanno, O. Ruiz de Ballesteros, F. Mollica, and G. Filippone, Compos. Sci. Technol., 180, 51 (2019).

    Article  CAS  Google Scholar 

  18. N. Sumrith, S. M. Rangappa, R. Dangtungee, S. Siengchin, M. Jawaid, and C. I. Pruncu, “Bio-based Polymers and Nanocomposites” (M. L. Sanyang and M. Jawaid Eds.), pp.255–272, Springer International Publishing, Cham, 2019.

  19. H. Ku, H. Wang, N. Pattarachaiyakoop, and M. Trada, Compos. Part B-Eng., 42, 856 (2011).

    Article  Google Scholar 

  20. Y. Tao, L. Yan, and R. Jie, T. Nonferr. Metal. Soc., 19, s651 (2009).

    Article  Google Scholar 

  21. S. H. Kamarudin, L. C. Abdullah, M. M. Aung, and C. T. Ratnam, IOP Conf. Ser. Mater. Sci. Eng., 368, 012011 (2018).

    Article  Google Scholar 

  22. A. Araujo, M. Oliveira, R. Oliveira, G. Botelho, and A. V. Machado, Environ. Sci. Pollut. Res. Int., 21, 9477 (2014).

    Article  CAS  Google Scholar 

  23. X. Qi, Y. Ren and X. Wang, Int. Biodeter. Biodegr., 117, 215 (2017).

    Article  CAS  Google Scholar 

  24. T. P. Haider, C. Volker, J. Kramm, K. Landfester, and F. R. Wurm, Angew. Chem. Int. Ed. Engl., 131, 50 (2019).

    Article  Google Scholar 

  25. N. D. Yaacob, H. Ismail, and S. Sung Ting, Bioresources, 11 (2015).

  26. R. Siakeng, M. Jawaid, H. Ariffin, and M. S. Salit, J. Bionic Eng., 15, 1035 (2018).

    Article  Google Scholar 

  27. A. Rubio-López, J. Artero-Guerrero, J. Pernas-Sánchez, and C. Santiuste, Polym. Test., 59, 127 (2017).

    Article  Google Scholar 

  28. M. N. Prabhakar, A. U. Rehman Shah, and J. I. Song, Carbohydr. Polym., 168, 201 (2017).

    Article  CAS  Google Scholar 

  29. J. P. Mofokeng, A. S. Luyt, T. Tábi, and J. Kovács, J. Thermoplast., 25, 927 (2011).

    Article  Google Scholar 

  30. M. R. Sanjay, P. Madhu, M. Jawaid, P. Senthamaraikannan, S. Senthil, and S. Pradeep, J. Clean. Prod., 172, 566 (2018).

    Article  CAS  Google Scholar 

  31. M. S. Islam, M. B. Ahmad, M. Hasan, S. A. Aziz, M. Jawaid, M. K. M. Haafiz, and S. A. H. Zakaria, Bioresources, 10, 1394 (2015).

    Article  Google Scholar 

  32. R. Gunti, A. V. Ratna Prasad, and A. V. S. S. K. S. Gupta, Polym. Compos., 39, 1125 (2016).

    Article  Google Scholar 

  33. L. Duan, W. Yu, and Z. Li, J. Eng. Fiber Fabr., 12, 33 (2017).

    CAS  Google Scholar 

  34. R. Siakeng, M. Jawaid, H. Ariffin, and S. M. Sapuan, Polym. Compos., 40, 2000 (2019).

    Article  CAS  Google Scholar 

  35. R. D. J. Johnson, V. Arumugaprabu, E. Rajasekar, G. Santhosh, and M. Saravanakumar, Mater. Today-Proc., 5, 6815 (2018).

    Article  CAS  Google Scholar 

  36. P. Tripathi and K. Yadav, Int. Res. J. Eng. Technol., 4, 2707 (2017).

    Google Scholar 

  37. M. Brebu, Polymers, 12, 166 (2020).

    Article  CAS  Google Scholar 

Download references

Acknowledgement

This work was jointly supported by HITEC University Taxila (Pakistan), and Basic Science Research Program through the National Research Foundation of Korea (NRF) funded by Ministry of Science Education Korea (2018R1A6A 1A03024509).

Author information

Authors and Affiliations

Authors

Corresponding authors

Correspondence to Atta Ur Rehman Shah or Jung-il Song.

Rights and permissions

Reprints and permissions

About this article

Check for updates. Verify currency and authenticity via CrossMark

Cite this article

Ejaz, M., Azad, M.M., Shah, A.U.R. et al. Mechanical and Biodegradable Properties of Jute/Flax Reinforced PLA Composites. Fibers Polym 21, 2635–2641 (2020). https://doi.org/10.1007/s12221-020-1370-y

Download citation

  • Received:

  • Revised:

  • Accepted:

  • Published:

  • Issue Date:

  • DOI: https://doi.org/10.1007/s12221-020-1370-y

Keywords

Navigation