Abstract
In order to know air pollution situation and their health, environmental, and climate effects, the air quality data with high temporal and spatial resolutions are essential. The spatial and seasonal variations of six criteria pollutants were investigated in 31 provincial capital cities between April 2014 and March 2015 using hourly mean air quality monitoring data, and the cities were classified by cluster analysis based on annual variations of air pollutants. The annual mean concentrations of PM2.5 (particulate matter with aerodynamic diameter less than 2.5 μm) and PM10 (particulate matter with aerodynamic diameter less than 10 μm) were high for all cities, which exceeded Chinese Ambient Air Quality Standards (CAAQS) Grade I standards. Only Fuzhou, Haikou, Kunming, and Lasa met Grade II standards for PM2.5 and PM10. Additionally, elevated SO2 concentration was observed in northern cities, especially in winter. However, the seasonal variation of O3 was opposite to other pollutants with the lowest concentrations in the winter and the highest in the summer. Winter domestic heating has significant impact on urban air quality, especially SO2 and PM10.
Similar content being viewed by others
References
Atkinson R (2000) Atmospheric chemistry of VOCs and NOx. Atmos Environ 34:2063–2101
Bapna M (2012) Toward an environmentally sustainable future: country environmental analysis of the People’s Republic of China. 2012 The Asian Development Bank, Manila
Cao Z, Sheng L, Liu Q, Yao X, Wang W (2015) Interannual increase of regional haze-fog in North China Plain in summer by intensified easterly winds and orographic forcing. Atmos Environ 122:154–162
Chai F, Gao J, Chen Z, Wang S, Zhang Y, Zhan J, Zhang H, Yun Y, Ren C (2014) Spatial and temporal variation of particulate matter and gaseous pollutants in 26 cities in China. J Environ Sci 26:75–82
Chan CK, Yao X (2008) Air pollution in mega cities in China. Atmos Environ 42(1):1–42
Che H, Zhang X, Li Y, Zhou Z, Qu JJ, Hao X (2009) Haze trends over the capital cities of 31 provinces in China, 1981-2005. Theor Appl Climatol 97:235–242
Chen Y, Xie S (2014) Characteristics and formation mechanism of a heavy air pollution episode caused by biomass burning in Chengdu, Southwest China. Sci Total Environ 473–474:507–517
Chen J, Zhao SP, Yin DY, Qu JJ (2015) Effect of dust process on air quality in cities of Northern China. J Desert Res 35(2):423–430
Cheng H, Wang Z, Feng J, Chen H, Zhang F, Liu J (2012) Carbonaceous species composition and source apportionment of PM2.5 in urban atmosphere of Wuhan. Ecol Environ Sci 21:1574–1579
Cheng Z, Jiang J, Fajardo O, Wang S, Hao J (2013) Characteristics and health impacts of particulate matter pollution in China (2001-2011). Atmos Environ 65:186–194
Du YJ, Li TT (2016) Assessment of health-based economic costs linked to fine particulate (PM2.5) pollution: a case study of haze during January 2013 in Beijing, China. Air Qual Atmos Health 9(4):439–445
Guo S, Hu M, Zamora ML, Peng J, Shang D, Zheng J, Du Z, Wu Z, Shao M, Zeng L, Molina MJ, Zhang R (2014) Elucidating severe urban haze formation in China. Proc Natl Acad Sci U S A 111(49):17373–17378. doi:10.1073/pnas.1419604111
Han S, Bian H, Tie X, Xie Y, Sun M, Liu A (2009) Impact of nocturnal planetary boundary layer on urban air pollutants: measurements from a 250-m tower over Tianjin, China. J Hazard Mater 162:264–269
Han S, Wu J, Zhang Y, Cai Z, Feng Y, Yao Q, Li X, Liu Y, Zhang M (2014) Characteristics and formation mechanism of a winter haze-fog episode in Tianjin, China. Atmos Environ 98:323–330
Hu J, Wang Y, Ying Q, Zhang H (2014) Spatial and temporal variability of PM2.5 and PM10 over the North China Plain and the Yangtze River Delta, China. Atmos Environ 95:598–609
Huang RJ, Zhang YL, Bozzetti C, Ho KF, Cao JJ, Han YM, Daellenbach KR, Slowik JG, Platt SM, Canonaco F, Zotter P, Wolf R, Pieber SM, Bruns EA, Crippa M, Ciarelli G, Piazzalunga A, Schwikowski M, Abbaszade G, Schnelle-Kreis J, Zimmermann R, An ZS, Szidat S, Baltensperger U, El Haddad I, Prevot ASH (2014) High secondary aerosol contribution to particulate pollution during haze events in China. Nature 514(7521):218–222
Jia B, Wang Y, Yao Y, Xie Y (2015) A new indicator on the impact of large-scale circulation on wintertime particulate matter pollution over China. Atmos Chem Phys 15:11919–11929
Johansson C, Norman M, Gidhagen L (2007) Spatial & temporal variations of PM10 and particle number concentrations in urban air. Environ Monit Assess 127:477–487
Kan H, Chen R, Tong S (2012) Ambient air pollution, climate change, and population health in China. Environ Int 42:10–19
Karar K, Gupta AK, Kumar A, Biswas AK (2006) Seasonal variations of PM10 and TSP in residential and industrial sites in an urban area of Kolkata, India. Environ Monit Assess 118(1-3):369–381
Lewne M, Cyrys J, Meliefste K, Hoek G, Brauer M, Fischer P, Gehring U, Heinrich J, Brunekreef B, Bellander T (2004) Spatial variation in nitrogen dioxide in three European areas. Sci Total Environ 332:217–230
Li L, Qian J, Ou CQ, Zhou YX, Guo C, Guo Y (2014) Spatial and temporal analysis of air pollution index and its timescale-dependent relationship with meteorological factors in Guangzhou, China, 2001-2011. Environ Pollut 190:75–81
Liu Y, Shao M, Zhang J, Fu L, Lu S (2005) Distributions and source apportionment of ambient volatile organic compounds in Beijing city, China. J Environ Sci Heal 40:1843–1860
Martini FMS, Hasenkopf CA, Roberts DC (2015) Statistical analysis of PM2.5 observations from diplomatic facilities in China. Atmos Environ 110:174–185
Meng ZY, Xu XB, Yan P, Ding GA, Tang J, Lin WL, Xu XD, Wang SF (2009) Characteristics of trace gaseous pollutants at a regional background station in Northern China. Atmos Chem Phys 9:927–936
Pui DYH, Chen SC, Zuo Z (2014) PM2.5 in China: measurements, sources, visibility and health effects, and mitigation. Particuology 13:1–26
Qu WJ, Arimoto R, Zhang XY, Zhao CH, Wang YQ, Sheng LF, Fu G (2010) Spatial distribution and interannual variation of surface PM10 concentrations over eighty-six Chinese cities. Atmos Chem Phys 10:5641–5662
Sun Y, Zhou X, Wai K, Yuan Q, Xu Z, Zhou S, Qi Q, Wang W (2013) Simultaneous measurement of particulate and gaseous pollutants in an urban city in North China plain during the heating period: implication of source contribution. Atmos Res 134:24–34
Ta W, Wang T, Xiao H, Zhu X, Xiao Z (2004) Gaseous and particulate air pollution in the Lanzhou Valley, China. Sci Total Environ 320:163–176
Tan JH, Duan JC, Zhen NJ, He KB, Hao JM (2016) Chemical characteristics and source of size-fractionated atmospheric particle in haze episode in Beijing. Atmos Res 167:24–33
Wang S, Yuan W, Shang K (2006) The impacts of different kinds of dust events on PM10 pollution in northern China. Atmos Environ 40:7975–7982
Wang W, Ren L, Zhang Y, Chen J, Liu H, Bao L, Fan S, Tang D (2008a) Aircraft measurements of gaseous pollutants and particulate matter over Pearl River Delta in China. Atmos Environ 42:6187–6202
Wang W, Chai FH, Zhang K, Wang SL, Chen YZ, Wang XZ, Yang YQ (2008b) Study on ambient air quality in Beijing for the summer 2008 Olympic Games. Air Qual Atmos Health 1(1):31–36
Wang ZB, Hu M, Wu ZJ, Yue DL (2013) Long-term measurements of particle number size distributions and the relationships with air mass history and source apportionment in the summer of Beijing. Atmos Chem Phys 13:10159–10170
Wang LT, Wei Z, Yang J, Zhang Y, Zhang FF, Su J, Meng CC, Zhang Q (2014a) The 2013 severe haze over southern Hebei, China: model evaluation, source apportionment, and policy implications. Atmos Chem Phys 14:3151–3173
Wang S, Xing J, Zhao B, Jang C, Hao J (2014b) Effectiveness of national air pollution control policies on the air quality in metropolitan areas of China. J Environ Sci 26:13–22
Wang X, Chen J, Cheng T, Zhang R, Wang X (2014c) Particle number concentration, size distribution and chemical composition during haze and photochemical smog episodes in Shanghai. J Environ Sci 26:1894–1902
Wang Y, Ying Q, Hu J, Zhang H (2014d) Spatial and temporal variations of six criteria air pollutants in 31 provincial capital cities in China during 2013–2014. Environ Int 73:413–422
Xiao Q, Ma Z, Li S, Liu Y (2015) The impact of winter heating on air pollution in China. Plos One 10(1):e0117311. doi:10.1371/journal.pone.0117311
Xu WY, Zhao CS, Ran L, Deng ZZ, Liu PF, Ma N, Lin WL, Xu XB, Yan P, He X, Yu J, Liang WD, Chen LL (2011) Characteristics of pollutants and their correlation to meteorological conditions at a suburban site in the North China Plain. Atmos Chem Phys 11:4353–4369
Xu X, Zhao T, Liu F, Gong SL, Kristovich D, Lu C, Guo Y, Cheng X, Wang Y, Ding G (2016) Climate modulation of the Tibetan Plateau on haze in China. Atmos Chem Phys 16:1365–1375
Yang L, Cheng S, Wang X, Nie W, Xu P, Gao X, Yuan C, Wang W (2013) Source identification and health impact of PM2.5 in a heavily polluted urban atmosphere in China. Atmos Environ 75:265–269
Zhang Q, Streets DG, Carmichael GR, He KB, Huo H, Kannari A, Klimont Z, Park IS, Reddy S, Fu JS, Chen D, Duan L, Lei Y, Wang LT, Yao ZL (2009) Asian emissions in 2006 for the NASA INTEX-B mission. Atmos Chem Phys 9:5131–5153
Zhang J, Chen J, Yang L, Sui X, Yao L, Zheng L, Wen L, Xu C, Wang W (2014) Indoor PM2.5 and its chemical composition during a heavy haze-fog episode at Jinan, China. Atmos Environ 99:641–649
Zhao Y, Nielsen CP, Lei Y, McElroy MB, Hao J (2011) Quantifying the uncertainties of a bottom-up emission inventory of anthropogenic atmospheric pollutants in China. Atmos Chem Phys 11:2295–2308
Zhao XJ, Zhao PS, Xu J, Meng W, Pu WW, Dong F, He D, Shi QF (2013) Analysis of a winter regional haze event and its formation mechanism in the North China Plain. Atmos Chem Phys 13(11):5685–5696
Zhao SP, Yin DY, Qu JJ (2015a) Identifying sources of dust based on CALIPSO, MODIS satellite data and backward trajectory model. Atmos Pollut Res 6(1):36–44
Zhao SP, Yu Y, Yin DY, He JJ (2015b) Meteorological dependence of particle number concentrations in an urban area of complex terrain, Northwestern China. Atmos Res 164–165:304–317
Zhao SP, Yu Y, Xia DS, Yin DY, He JJ, Liu N, Li F (2015c) Urban particle size distributions during two contrasting dust events originating from Taklimakan and Gobi Deserts. Environ Pollut 207:107–122
Zhao SP, Yu Y, Yin DY, He JJ, Liu N, Qu JJ, Xiao JH (2016) Annual and diurnal variations of gaseous and particulate pollutants in 31 provincial capital cities based on in situ air quality monitoring data from China national environmental monitoring center. Environ Int 86:92–106
Zheng M, Salmon LG, Schauer JJ, Zeng L, Kiang CS, Zhang Y, Cass G (2005) Seasonal trends in PM2.5 source contributions in Beijing, China. Atmos Environ 39:3967–3976
Zheng S, Wang M, Wang S, Tao Y, Shang K (2013) Short-term effects of gaseous pollutants and particulate matter on daily hospital admissions for Cardio-cerebrovascular disease in Lanzhou: evidence from a heavily polluted city in China. Int J Environ Res Public Health 10:462–477
Zheng XY, Fu YF, Yang YJ, Liu GS (2015) Impact of atmospheric circulations on aerosol distributions in autumn over eastern China: observational evidence. Atmos Chem Phys 15:12115–12138
Acknowledgments
This work was financially funded by the Open Fund Program of Key Laboratory of Land Surface Process and Climate Change in Cold and Arid Regions, Chinese Academy of Sciences (No. LPCC201510), and Opening Project of Shanghai Key Laboratory of Atmospheric Particle Pollution and Prevention (LAP3) (FDLAP16005). We were very grateful to China National Environmental Monitoring Center (http://113.108.142.147:20035/emcpublish/) for the provision of air quality monitoring data used in this study.
Author information
Authors and Affiliations
Corresponding author
Rights and permissions
About this article
Cite this article
Yin, D., Zhao, S. & Qu, J. Spatial and seasonal variations of gaseous and particulate matter pollutants in 31 provincial capital cities, China. Air Qual Atmos Health 10, 359–370 (2017). https://doi.org/10.1007/s11869-016-0432-1
Received:
Accepted:
Published:
Issue Date:
DOI: https://doi.org/10.1007/s11869-016-0432-1