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Aluminum speciation in drinking water distribution system: A case study in northeastern China

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Abstract

This study aimed to investigate the variation of aluminum species in a drinking water distribution system in a city in northeastern China. The aluminum species were determined by fluorometric methods. Results showed that suspended aluminum (Sus-Al) was the major species in the drinking water supplied by plant B and accounted for about 42% of the total aluminum (Tol-Al). The concentrations of Sus-Al and Tol-Al could be controlled effectively by introducing reservoir water. In the water source switching process, the water quality variation led to the suddenly release of Sus-Al, especially in a cast iron pipeline that had been in service for more than 30 years, but the soluble aluminum varied little. In the plant A service areas, the average concentrations of the inorganic monomeric aluminum (IM-Al), monomeric aluminum (Mon-Al), and soluble aluminum (Sol-Al) were 0.008 mg L−1, 0.03 mg L−1, and 0.04 mg L−1, respectively, and their concentrations in the plant B service areas were higher. The pH and fluoride were the major parameters affecting the soluble aluminum speciation. With a solution pH of 6.5–7.5 and fluoride below 0.3 mg L−1, the Sol-Al could be controlled within 0.1 mg L−1. Water quality regulation and terminal filtration were suggested for residual aluminum control.

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References

  1. S. C. Christopher and L. S. Carl, Science, 204, 304 (1979).

    Article  Google Scholar 

  2. F. Gerhard, L.P. Brian, U. Kai-Uwe, P. Rosemarie and H.C. William, Science, 297, 2245 (2002).

    Article  Google Scholar 

  3. C. T. Driscoll and R. D. Letterman, J. Environ. Eng., 114, 21 (1988).

    Article  CAS  Google Scholar 

  4. F. Y. Cui, M. C. Hu, Y. Zhang and C.W. Cui, China Water and Wastewater, 18, 4 (2002).

    Google Scholar 

  5. R. D. Miller, F. C. Kopfler, K. C. Kelty, J.A. Stober and N. S. Ulmer, J. American Water Works Association, 76, 84 (1984).

    CAS  Google Scholar 

  6. R. D. Letterman and C. T. Driscoll, J. American Water Works Association, 80, 154 (1988).

    CAS  Google Scholar 

  7. C. J. Sollars, A. M. Bragg, A. M. Simpson and R. Perry, Environ. Technol. Lett., 10, 130 (1989).

    Article  Google Scholar 

  8. P. T. Srinivasan, T. Viraraghavan and K. S. Subramanian, Water SA, 25, 47 (1999).

    CAS  Google Scholar 

  9. S. Kvech and M. Edwards, J. American Water Works Association, 93, 104 (2001).

    Google Scholar 

  10. R. Fuge, N. J. G. Pearce and W. T. Perkins, Environ. Geochem. Health, 14, 15 (1992).

    Article  CAS  Google Scholar 

  11. R. D. Shea, Public Works, 124, 54 (1993).

    Google Scholar 

  12. D. Kriewall, R. Harding, E. Naisch and L. Schantz, Public Works, 127, 28 (1996).

    Google Scholar 

  13. A. A. Havics, Microscope, 49, 1 (2001).

    CAS  Google Scholar 

  14. J. D. Birchall, Colloid Chemistry of Silica, 234, 601 (1994).

    Article  CAS  Google Scholar 

  15. R. B. Martin, J. Inorg. Biochem., 44, 141 (1991).

    Article  CAS  Google Scholar 

  16. J. E. Van Benschoten and J. K. Edzwald, J. American Water Works Association, 82, 71 (1990).

    Google Scholar 

  17. C. Y. Wang, S. P. Bi, C. H. Zhang, Z. C. Zhang and W. H. Yang, J. Inst. Anal., 23, 1 (2004).

    Google Scholar 

  18. C. Exley and J. D. Birchall, Polyhedron, 12, 1007 (1993).

    Article  CAS  Google Scholar 

  19. U.S. EPA. Office of Groundwater and Drinking Water, Inorganic Contaminant Accumulation in Potable Water Distribution Systems, USEPA:31 (2006).

  20. H. Z. Lian, Y. F. Kang, A. Yasen, S. P. Bi and D. N. Li, Spectroscopy and Spectral Analysis, 24, 1391 (2004).

    CAS  Google Scholar 

  21. State Environmental Protection Administration of China. Analysis Method of the Water and Wastewater (Revision 4). Environmental Science Press of China: Beijing, 340 (2002).

    Google Scholar 

  22. W. D. Wang, H.W. Yang, H. Z. Zhao and Z. P. Jiang, J. Environ. Sci., 19, 897 (2007).

    Article  CAS  Google Scholar 

  23. W.D. Wang, H.W. Yang, X. C. Wang, J. Jiang and W. P. Zhu, J. Environ. Sci., 22, 211 (2010).

    Article  CAS  Google Scholar 

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Correspondence to Wen-Dong Wang.

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Wang, WD., Yang, HW., Jiang, J. et al. Aluminum speciation in drinking water distribution system: A case study in northeastern China. Korean J. Chem. Eng. 28, 1227–1232 (2011). https://doi.org/10.1007/s11814-010-0495-x

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  • DOI: https://doi.org/10.1007/s11814-010-0495-x

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