Skip to main content
Log in

Normal-Incidence Photoemission Electron Microscopy (NI-PEEM) for Imaging Surface Plasmon Polaritons

  • Published:
Plasmonics Aims and scope Submit manuscript

Abstract

We introduce a novel time-resolved photoemission-based near-field illumination method, referred to as femtosecond normal-incidence photoemission microscopy (NI-PEEM). The change from the commonly used grazing-incidence to normal-incidence illumination geometry has a major impact on the achievable contrast and, hence, on the imaging potential of transient local near fields. By imaging surface plasmon polaritons in normal light incidence geometry, the observed fringe spacing directly resembles the wavelength of the plasmon wave. Our novel approach provides a direct descriptive visualization of SPP wave packets propagating across a metal surface.

This is a preview of subscription content, log in via an institution to check access.

Access this article

Price excludes VAT (USA)
Tax calculation will be finalised during checkout.

Instant access to the full article PDF.

Fig. 1
Fig. 2
Fig. 3
Fig. 4
Fig. 5
Fig. 6

Similar content being viewed by others

References

  1. Ozbay E (2006) Plasmonics: merging photonics and electronics at nanoscale dimensions. Science 311(5758):189–193

    Article  CAS  Google Scholar 

  2. MacDonald KF, Samson ZL, Stockman MI, Zheludev NI (2009) Ultrafast active plasmonics. Nat Photonics 3(1):55–58

    Article  CAS  Google Scholar 

  3. Schmidt T, Heun S, Slezak J, Diaz J, Prince KC, Lilienkamp G, Bauer E (1998) Speleem: combining LEEM and spectroscopic imaging. Surf Rev Lett 5:1287–1296

    Article  CAS  Google Scholar 

  4. Wiemann C, Bayer D, Rohmer M, Aeschlimann M, Bauer M (2007) Local 2PPE-yield enhancement in a defined periodic silver nanodisk array. Surf Sci 601(20):4714–4721

    Article  CAS  Google Scholar 

  5. Chelaru LI, Meyer zu Heringdorf F-J (2007) In situ monitoring of surface plasmons in single-crystalline Ag-nanowires. Surf Sci 601:4541–4545

    Article  CAS  Google Scholar 

  6. Lemke C, Schneider C, Leißner T, Bayer D, Radke JW, Fischer A, Melchior P, Evlyukhin AB, Chichkov BN, Reinhardt C, Bauer M, Aeschlimann M (2013) Spatiotemporal characterization of spp pulse propagation in two-dimensional plasmonic focusing devices. Nano Lett 13(3):1053–1058

    Article  CAS  Google Scholar 

  7. Kubo A, Pontius N, Petek H (2007) Femtosecond microscopy of surface plasmon polariton wave packet evolution at the silver/vacuum interface. Nano Lett 7:470–475

    Article  CAS  Google Scholar 

  8. Meyer zu Heringdorf F-J, Buckanie NM (2010) Nonlinear photoemission microscopy with surface plasmon polaritons. Microsc Microanal 16:502–503

    Article  CAS  Google Scholar 

  9. Schmidt O, Bauer M, Wiemann C, Porath R, Scharte M, Andreyev O, Schönhense G, Aeschlimann M (2002) Time-resolved two photon photoemission electron microscopy. Appl Phys B 74(3):223–227

    Article  CAS  Google Scholar 

  10. Bauer M, Wiemann C, Lange J, Bayer D, Rohmer M, Aeschlimann M (2007) Phase propagation of localized surface plasmons probed by time-resolved photoemission electron microscopy. Appl Phys A 88(3):473–480

    Article  CAS  Google Scholar 

  11. Buckanie N, Kirschbaum P, Sindermann S, Meyer zu Heringdorf F-J (2013) Interaction of light and surface plasmon polaritons in Ag islands studied by nonlinear photoemission microscopy. Ultramicroscopy 130:49–53

    Article  CAS  Google Scholar 

  12. Amidror I (2000) The theory of the Moiré phenomenon. Kluwer, Dordrecht

    Book  Google Scholar 

  13. Hermann K (2012) Periodic overlayers and Moiré patterns: theoretical studies of geometric properties. J Phys Condens Matter 24:314210

    Article  Google Scholar 

  14. Lemke C, Leißner T, Jauernik S, Klick A, Fiutowski J, Kjelstrup-Hansen J, Rubahn H-G, Bauer M (2012) Mapping surface plasmon polariton propagation via counter-propagating light pulses. Opt Express 20:12877–12884

    Article  Google Scholar 

  15. Wall D, Tikhonov S, Sindermann S, Spoddig D, Hassel C, Horn-von Hoegen M, Meyer zu Heringdorf F-J (2011) Shape, orientation, and crystalline composition of silver islands on Si(111). IBM J Res Dev 55:9:1–9:6

    Article  Google Scholar 

  16. Kury P, Hild R, Thien D, Guenter H-L, Meyer zu Heringdorf F-J, Horn-von Hoegen M (2005) Compact and transferable threefold evaporator for molecular beam epitaxy in ultrahigh vacuum. Rev Sci Instrum 76:83906

    Article  Google Scholar 

  17. Meyer zu Heringdorf F-J, Belton A (2004) Flexible microprocessor-based evaporation controller. Rev Sci Instrum 75(12):5288–5292

    Article  CAS  Google Scholar 

  18. Meyer zu Heringdorf F-J, Chelaru L, Möllenbeck S, Thien D, Horn-von Hoegen M (2007) Femtosecond photoemission microscopy. Surf Sci 601:4700–4705

    Article  CAS  Google Scholar 

  19. Scharte M, Porath R, Ohms T, Aeschlimann M, Krenn JR, Ditlbacher H, Aussenegg FR, Liebsch A (2001) Do Mie plasmons have a longer lifetime on resonance than off resonance? Appl Phys B 73(4):305–310

  20. Johnson PB, Christy RW (1972) Optical constants of the noble metals. Phys Rev B 6:4370–4379

    Article  CAS  Google Scholar 

  21. Kirschbaum P, Buckanie N, Meyer zu Heringdorf F-J (2012) Impact of C60 adsorption on surface plasmon polaritons on self-assembled Ag(111) islands on Si(111). Plasmonics 7(2):229–233

Download references

Acknowledgments

Financial support from the Deutsche Forschungsgemeinschaft through SFB616 “Energy Dissipation at Surfaces” and SPP1391 “Ultrafast Nanooptics” is gratefully acknowledged.

Author information

Authors and Affiliations

Authors

Corresponding author

Correspondence to Frank-J. Meyer zu Heringdorf.

Rights and permissions

Reprints and permissions

About this article

Check for updates. Verify currency and authenticity via CrossMark

Cite this article

Kahl, P., Wall, S., Witt, C. et al. Normal-Incidence Photoemission Electron Microscopy (NI-PEEM) for Imaging Surface Plasmon Polaritons. Plasmonics 9, 1401–1407 (2014). https://doi.org/10.1007/s11468-014-9756-6

Download citation

  • Received:

  • Accepted:

  • Published:

  • Issue Date:

  • DOI: https://doi.org/10.1007/s11468-014-9756-6

Keywords

Navigation