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Correlation between boson peak and thermal expansion manifested by physical aging and high pressure

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Abstract

We investigate the effects of high pressure and physical aging on the boson peak and thermal expansion of a typical metallic glass. Specifically, the thermal expansion coefficient and boson peak intensity monotonically decrease during physical aging. With the increase of high pressure, the boson peak intensity and the thermal expansion coefficient coincidently experience an incipient decrease and then a subsequent increase. The boson peak intensity shows an approximately linear relationship with the thermal expansion coefficient. The thermal expansion can be affected by structural relaxation or rejuvenation, which can reflect the flow units variation and atomic packing of a metallic glass. Our results indicate a direct link between structural relaxation or rejuvenation and fast boson peak dynamics, providing insights into the boson peak behavior and structural heterogeneity of metallic glasses.

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Funding

This work was supported by the National Natural Science Foundation of China (Grant Nos. 51801083, 11790291, 51461165101, 51801124, and 51671211), and the Natural Science Foundation of Jiangsu Province (Grant No. BK20181044).

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Authors and Affiliations

  1. Institute of Physics, Chinese Academy of Sciences, Beijing, 100190, China

    Rongjie Xue, Linzhi Zhao, Yunqi Cai, Jinguang Cheng, Ping Wen, Weihua Wang, Mingxiang Pan & Haiyang Bai

  2. School of Materials Engineering, Jiangsu University of Technology, Changzhou, 213001, China

    Rongjie Xue & Jiaojiao Yi

  3. College of Materials Science and Opto-Electronic Technology, University of Chinese Academy of Sciences, Beijing, 100049, China

    Weihua Wang & Haiyang Bai

  4. School of Physical Sciences, University of Chinese Academy of Sciences, Beijing, 100190, China

    Mingxiang Pan

  5. Songshan Lake Materials Laboratory, Dongguan, 523808, China

    Mingxiang Pan

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  1. Rongjie Xue
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  2. Linzhi Zhao
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  3. Yunqi Cai
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  4. Jiaojiao Yi
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  7. Weihua Wang
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Correspondence to Rongjie Xue, Mingxiang Pan or Haiyang Bai.

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Xue, R., Zhao, L., Cai, Y. et al. Correlation between boson peak and thermal expansion manifested by physical aging and high pressure. Sci. China Phys. Mech. Astron. 65, 246111 (2022). https://doi.org/10.1007/s11433-021-1815-8

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