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Radiation hazards associated with radionuclides and theoretical evaluation of indoor radon concentration from soil exhalation of Udhampur District, Jammu and Kashmir State, India

  • Soils, Sec 5 • Soil and Landscape Ecology • Research Article
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Abstract

Purpose

Soil is the prime source of radon and thoron concentrations in the household dwellings. The presence of radioactive gases in the environment is mainly due to the presence of radionuclide content in soil, rocks, and building materials. So, it is necessary to estimate the radionuclide content in the living environment. The annual effective dose has been assessed from the radionuclide content, and an effort has been made to correlate the concentration of these radionuclides with exhalation rates of their daughter products, i.e., radon and thoron. Theoretically determined indoor radon concentration has also been compared with experimentally observed results.

Material and methods

Scintillation-based Smart RnDuo monitor (SRM) and gamma spectrometry (NaI(Tl)) have been utilized for the estimation of exhalation rates and radionuclide (226Ra, 232Th, and 40K) contents in soil samples.

Results and discussions

The range of radon mass and thoron surface exhalation rate in soil samples are found to vary from 11.57 to 65.62 mBq kg−1 h−1 with an average of 28.20 mBq kg−1 h−1 and from 52 to 930 mBq m−2 s−1 with an average of 312 mBq m−2 s−1, respectively. The average activity concentrations of 226Ra, 232Th, and 40K are 24.52 Bq kg−1, 41.15 Bq kg−1, and 343 Bq kg−1, respectively.

Conclusions

The average values of 226Ra, 232Th, and 40K are well within the safe range recommended by the United Nations Scientific Committee on the Effects of Atomic Radiations. The calculated annual effective dose and radiation hazard risks have been found to be well below the recommended levels. Results obtained from theoretical evaluation are compared with experimentally obtained results and are in good agreement with each other. Different occupancy factors have also been analyzed according to the populace indoor occupancy.

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References

  • Ahmad N, Hussein AJA, Aslam (1998) Radiation doses in Jordanian dwellings due to natural radioactivity in construction materials and soil. J Environ Radioact 41:127–136

    Article  CAS  Google Scholar 

  • Avwiri GO, Osimobi JO, Agbalagba EO (2012) Evaluation of radiation hazard indices and excess lifetime cancer risk due to natural radioactivity in soil profile of Udi and Ezeagu local government areas of Enugu state, Nigeria. Environ Earth Sci 1:1–10

    Google Scholar 

  • Bangotra P, Mehra R, Jakhu R, Kaur K, Pandit P, Kanse S (2018) Estimation of 222Rn exhalation rate and assessment of radiological risk from activity concentration of 226Ra, 232Th and 40K. J Geochem Explor 184(Part B):304–310

    Article  CAS  Google Scholar 

  • Beck HL, De Campo JA, Gogolak CV (1972) In-situ Ge(Li) and NaI(Tl) gamma-ray spectrometry for the measurement of environmental radiation. USAEC-Report HASL-258

  • Beretka J, Mathew PJ (1985) Natural radioactivity of Australian building materials, industrial wastes and by-products. Health Phys 48:87–95

    Article  CAS  Google Scholar 

  • O’Brien K, Sanna R (1976) The distribution of absorbed dose-rates in humans from exposure to environmental gamma rays. Health Phys 30:71–78

    Article  Google Scholar 

  • O’Brien K, Sanna R (1978) The effect of male-female body-size difference on absorbed dose-rate distributions in humans from natural gamma rays. Health Phys 34:107–112

    Google Scholar 

  • Chad Umoren YE, Umah IH (2014) Baseline radionuclide distribution patterns in soil and radiation hazard indices for Abak, Nigeria. Advs Phys Theory Appl 32:69–79

    Google Scholar 

  • Chauhan RP, Kumar A, Chauhan N, Joshi M, Aggarwal P, Sahoo BK (2016) Ventilation effect on indoor radon–thoron levels in dwellings and correlation with soil exhalation rates. Indoor Built Environ 25(1):203–212

    Article  CAS  Google Scholar 

  • Elejalde C, Romero HF, Legarda F (1993) Influence of physical factors on radionuclide content in soil from Biscay (Spain). Toxicol Environ Chem 39:183–192

    Article  CAS  Google Scholar 

  • Ferdoas S, Saleh A, Badriah, Berzan A (2007) Measurements of natural radioactivity in some kinds of marble and granite used in Riyadh region. J Nucl Radiat Phys 2:25–36

    Google Scholar 

  • Gaware JJ, Sahoo BK, Sapra BK, Mayya YS (2011) Indigenous development and networking of online radon monitors in the underground uranium mine. Radiat Prot Environ 34:37–40

    Google Scholar 

  • GSI (1977) Geology and mineral resources of the state India, part X—J&K State, pub. no. 30. Controller of Publications, Delhi

    Google Scholar 

  • Hassan NM, Ishikawa T, Hosoda M, Sorimachi A, Tokonami S, Fukushi M, Sahoo SK (2010) Assessment of the natural radioactivity using two techniques for the measurement of radionuclide concentration in building materials used in Japan. J Radioanal Nucl Chem 283:15–21

    Article  CAS  Google Scholar 

  • Huy NQ, Hien PD, Luyen TV, Hoang DV, Hiep TP, Quang NH, Long NQ, Nhan DD, Binh NT, Hai PS, Ngo NT (2012) Natural radioactivity and external dose assessment of surface soils in Vietnam. Radiat Prot Dosim 151(3):522–531

    Article  CAS  Google Scholar 

  • IAEA (1989) Regional workshop on environmental sampling and measurements of radioactivity for monitoring purpose, Kalpakkam, India. 9:85–92

  • ICRP (International Commission on Radiological Protection) (2000) Protection of the public in situations of prolonged radiation exposure. In: ICRP publication 82. Pergamon, Oxford. Ann, pp 1–2

  • ICRP (International Commission on Radiological Protection) (2010) Conversion coefficients for radiological protection quantities for external radiation exposures. Oxford: Elsevier (ICRP Publication 116), Ann ICRP 40 (2–5)

  • James JP, Dileep BN, Mulla RM, Joshi RM, Vishnu MS, Nayak PD (2013) Evaluation of internal dose to members of the public at the Kaiga site, India, due to the ingestion of primordial radionuclide 40K. Radiat Prot Dosim 53:56–63

    Article  Google Scholar 

  • Kanse SD, Sahoo BK, Sapra BK, Gaware JJ, Mayya YS (2013) Powder sandwich technique: a novel method for determining the thoron emanation potential of powders bearing high 224Ra content. Radiat Meas 48:82–87

    Article  CAS  Google Scholar 

  • Khan MS, Srivastava DS, Azam A (2012) Study of radium content and radon exhalation rates in soil samples of Northern India. Environ Earth Sci 67(5):1363–1371

    Article  CAS  Google Scholar 

  • Kumar A, Chauhan RP, Joshi M, Sahoo BK (2014) Modeling of indoor radon concentration from radon exhalation rates of building materials and validation through measurements. J Environ Radioact 127:50–55

    Article  CAS  Google Scholar 

  • Kumar A, Sharma S, Mehra R, Kanwar I, Mishra R, Kaur I (2018) Assessment of radon concentration and heavy metal contamination in ground water samples of Udhampur District, Jammu & Kashmir, India. Environ Geochem Health 40:815–831

    Article  CAS  Google Scholar 

  • Kumar A, Sharma S, Mehra R, Narang S, Mishra R (2018b) Assessment of indoor radon, thoron, concentration and their relationship with seasonal variation and geology of Udhampur District, Jammu & Kashmir, India. Int J Occup Environ Health 23(2):202–214

    Google Scholar 

  • Kumar A, Vij R, Sharma S, Sarin A, Narang S (2018a) Assessment of radionuclides concentration and exhalation studies in soil of lesser Himalayas of Jammu & Kashmir, India. Acta Geophys. https://doi.org/10.1007/s11600-018-0119-0

  • Malanca A, Gaidolif L, Pessina V, Dallara G (1996) Distribution of 226Ra, 232Th and 40K in soils of Rio Grande do Norte (Brazil). J Environ Radioact 30:55–67

    Article  CAS  Google Scholar 

  • Menon SR, Sahoo BK, Balasunder S, Gaware JJ, Jose MT, Venktaraman B, Mayya YS (2015) A comparative study between the dynamic method and passive can technique of radon exhalation measurements from samples. Appl Radiat Isot 99:172–178

    Article  Google Scholar 

  • Mir FA, Rather SA (2015) Measurement of radioactive nuclides present in soil samples of district Ganderbal of Kashmir Province for radiation safety purposes. J Radiat Res Appl Sci 8:155–159

    Article  CAS  Google Scholar 

  • Moed BA, Nazaroff WW, Sextro RG (1988) Soil as a source of indoor radon: generation, migration and entry. In: Nazaroff WW, Nero AV Jr (eds) Radon and its decay products in indoor air. Wiley, New York, pp 57–112

    Google Scholar 

  • Myrick TE, Berven BA, Haywood FF (1983) Determination of concentrations of selected radionuclides in surface soil in the U.S. Health Phys 45:631–642

    Article  CAS  Google Scholar 

  • Nazaroff WW, Nero AV Jr (1988) Radon and its decay products in indoor air. Wiley, New York

    Google Scholar 

  • OECD (Organization for Economic Cooperation and Development) (1979) Exposure to radiation from the natural radioactivity in building materials. In: Report by a group of experts of the OECD Nuclear Energy Agency. France

  • Quindos LS, Fernandez PL, Soto J (1987) Building material as source of exposure in houses. Indoor Air 87(2):365

    Google Scholar 

  • Rogers VC, Nielson KK, Holt RB, Snoddy R (1994) Radon diffusion coefficients for residential concretes. Health Phys 67:261–265

    Article  CAS  Google Scholar 

  • Sahoo BK, Agarwal TK, Gaware JJ, Sapra BK (2014) Thoron interference in radon exhalation rate measured by solid stat nuclear track detector based can technique. J Radioanal Nucl Chem 302:1417–1420

    Article  CAS  Google Scholar 

  • Sahoo BK, Nathwani D, Eappen KP, Ramachandran TV, Gaware JJ, Mayya YS (2007) Estimation of radon emanation factor in Indian building materials. Radiat Meas 42:1422–1425

    Article  CAS  Google Scholar 

  • Sahoo BK, Sapra BK, Gaware JJ, Kanse SD, Mayya YS (2011) A model to predict radon exhalation from walls to indoor air based on the exhalation from building material samples. Sci Total Environ 409:2635–2641

    Article  CAS  Google Scholar 

  • Sasaki T, Gunji Y, Okuda T (2004) Mathematical modelling of radon emanation. J Nucl Sci Technol 41:142–151

    Article  CAS  Google Scholar 

  • Shanthi G, Kumaran JT, Raj GA, Maniyan CG (2010) Natural radionuclides in the South Indian foods and their annual dose. Nucl Inst Methods Phys Res A 619:436–440

    Article  CAS  Google Scholar 

  • Sharma DK, Kumar A, Kumar M, Singh S (2003) Study of uranium, radium and radon exhalation rate in soil samples from some areas of Kangra District, Himachal Pradesh, India using solid state nuclear track detector. Radiat Meas 36:363–366

    Article  CAS  Google Scholar 

  • Sharma S, Kumar A, Mehra R (2017a) Variation of ambient gamma dose rate and indoor radon/thoron concentration in different villages of Udhampur District, Jammu & Kashmir, India. Radiat Prot Environ 40:133–141

    Article  Google Scholar 

  • Sharma S, Kumar A, Mehra R, Mishra R (2017) Ingestion doses and hazard quotients due to intake of uranium in drinking water from Udhampur District of Jammu & Kashmir State, India. Radioprotection 52:109–118

    Article  CAS  Google Scholar 

  • Sharma S, Kumar A, Mehra R, Kaur M, Mishra R (2018) Assessment of progeny concentrations of 222Rn/220Rn, and related doses using deposition-based progeny sensors. Environ Sci Pollut Res 25:11440–11453

    Article  CAS  Google Scholar 

  • Singh P, Sahoo BK, Bajwa BS (2016) Theoretical modeling of indoor radon concentration and its validation through measurements in South-East Haryana, India. J Environ Manag 171:35–41

    Article  CAS  Google Scholar 

  • Singh P, Singh P, Bajwa BS, Sahoo BK (2017a) Radionuclide contents and their correlation with radon-thoron exhalation in soil samples from mineralized zone of Himachal Pradesh, India. J Radioanal Nucl Chem 311(1):253–261

    Article  CAS  Google Scholar 

  • Singh P, Singh P, Saini K, Bajwa BS (2017b) Radionuclide measurements along with exhalation study in subsoil of Southeast Haryana, India. Environ Earth Sci 76. https://doi.org/10.1007/s12665-017-6650-5

  • Singh S, Sharma DK, Dhar S, Kumar A, Kumar A (2007) Uranium, radium and radon measurements in the environs of Nurpur area, Himachal Himalayas, India. Environ Monit Assess 128:301–309

    Article  CAS  Google Scholar 

  • Stoulos S, Manolopoulou M, Papastefanou C (2003) Assessment of natural radiation exposure and radon exhalation from building materials in Greece. J Environ Radioact 69:225–240

    Article  CAS  Google Scholar 

  • Tufail M, Rashid T, Mahmood AB, Ahmad N (1994) Radiation doses in Pakistani houses. Sci Total Environ 142:171–177

    Article  CAS  Google Scholar 

  • Ujic P, Celikovic I, Kandic A, Vukanac I, Durasevic M, Dragosavac D, Zunic ZS (2010) Internal exposure from building materials exhaling 222Rn and 220Rn as compared to external exposure due to their natural radioactivity content. Appl Radiat Isot 68:201–206

    Article  CAS  Google Scholar 

  • UNSCEAR (United Nations Scientific Committee on the Effects of Atomic Radiation) (1993) Sources and biological effects of ionizing radiation. United Nations, New York

    Google Scholar 

  • UNSCEAR (United Nation Scientific Committee on the Effects of Atomic Radiation) (2000) Sources, effects and risks of ionizing radiation. Report to the general assembly. United Nations, New York

    Google Scholar 

  • UNSCEAR (United Nations Scientific Committee on the Effects of Atomic Radiation) (2008) Sources and biological effects of ionizing radiation. United Nations, New York

    Google Scholar 

Download references

Acknowledgements

We gratefully acknowledge the support of Dr. B. R. Ambedkar National Institute of Technology, Jalandhar, and D.A.V. College, Amritsar, for providing the necessary facilities for this work. We are also thankful to the residents of the study area for their cooperation during fieldwork.

Funding

The authors express their gratitude to the Board of Research in Nuclear Sciences (BRNS), Department of Atomic Energy (DAE), Government of India, for providing the financial support for this work (Ref. No. 2013/36/60 BRNS).

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Correspondence to Ajay Kumar.

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Responsible editor: Claudio Bini

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Sharma, S., Kumar, A., Mehra, R. et al. Radiation hazards associated with radionuclides and theoretical evaluation of indoor radon concentration from soil exhalation of Udhampur District, Jammu and Kashmir State, India. J Soils Sediments 19, 1441–1455 (2019). https://doi.org/10.1007/s11368-018-2125-x

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