Abstract
Currently, atmospheric anthropogenic radionuclides (particulate) are controlled by suspension of the surface dust containing those radionuclides (resuspension). We have found, therefore, that such radionuclides can be used as tracers of the surface dust suspension, transport and its subsequent deposition in distant areas. The 137Cs/90Sr activity ratios in the atmospheric deposition, without the direct influence of nuclear tests and accidents, at the Meteorological Research Institute (MRI, Tsukuba, Japan) during the 1990s were fairly low (average: 2.1). This value is not in agreement with the ratios in Japanese surface soils (range of averages: 4–7), which had been considered as the primary source of the deposited dust. This suggests that the current atmospheric dust deposition in Japan is a mixture of local and remote components. The remote component could be an aeolian dust that has been transported long distances from arid areas. The major component is most likely to be Asian dust. It was further hypothesized that other remote source may exist beyond the Asian domain, based on accumulated observations and model results. To obtain more information about the dust transport, Sahara dust deposited in Monaco in 2002 and a suspended dust collected in the Taklamakan area in 2001 were analyzed for 90Sr and 137Cs. The Taklamakan dust exhibited a 137Cs/90Sr ratio of about 4, which is within the range of atmospheric deposition observed at the MRI, while the Sahara dust exhibited a higher 137Cs/90Sr ratio (about 13). Although the present Sahara datum was negative for our hypothesis of ‘hyper-range transport’, the seasonal change of the 137Cs/90Sr ratio in the atmospheric deposition observed at the MRI requires an aeolian dust source having a low 137Cs/90Sr ratio, other than Asian dust.
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Aoyama, M., Hirose, K., Suzuki, Y., Inoue, H. and Sugimura, Y.: 1986, ‘High level radioactive nuclides in Japan in May’, Nature 321, 819–820.
Aoyama, M., Hirose, K. and Sugimura, Y.: 1991, ‘The temporal variation of stratospheric fallout derived from the Chernobyl accident’, J. Environ. Radioactivity 13, 103–115.
Aoyama, M. and Hirose, K.: 1995, ‘The temporal and spatial variation of 137Cs concentration in the western North Pacific and its marginal seas during the period from 1979 to 1988’, J. Environ. Radioactivity 29, 57–74.
Eisenbud, M. and Gesell, T.: 2000, Environmental Radioactivity (Fourth Edition), Academic Press, New York, USA.
Gao, T., Yu, X., Ma, Q., Li, H., Li, X. and Si, Y.: 2003, ‘Climatology and trends of the temporal and spatial distribution of sandstorms in Inner Mongolia’, Water, Air, and Soil Pollution: Focus 3, 51–66.
Gritchenko, Z. G., Ivanova, L. M., Tishkov, V. P. and Tsvetkov, O. S.: 2001, ‘Radioactive fallout and accumulated level of soil surface contamination with 90Sr and 137Cs around St. Petersburg in 1954–1999’, Radiochemistry 43, 315–319.
Hirose, K. and Sugimura, Y.: 1984, ‘Excess 228Th in the airborne dust: An indicator of continental dust from the East Asian deserts’, Earth Planet. Sci. Lett. 70, 110–114.
Hirose, K., Aoyama, M., Katsuragi, Y. and Sugimura, Y.: 1987, ‘Annual deposition of Sr-90’, J. Meteoro. Soc. Jpn. 65, 259–277.
Hirose, K., Aoyama, M., Miyao, T. and Igarashi, Y.: 2001, ‘Plutonium in seawaters on the western North Pacific’, J. Radioanal. Nucl. Chem. 248, 771–776.
Hirose, K., Igarashi, Y., Aoyama, M., Kim, C. K., Kim, C. S. and Chang, B. W.: 2003, ‘Recent trends of plutonium fallout observed in Japan: Plutonium as a proxy for desertification’, J. Envrion. Monit. 5, 302–307.
Hirose, K., Honda, T., Yanagishita, S., Igarashi, Y. and Aoyama, M.: 2004, ‘Deposition behaviors of 210Pb, 7Be and thorium isotopes observed in Tsukuba and Nagasaki, Japan’, Atmos. Environ. 38, 6601–6608.
Husar, R. B., Tratt, D. M., Schichtel, B. A., Falke, S. R., Li, F., Jaffe, D., Gassó, S., Gill, T., Laulainen, N. S., Lu, F., Reheis, M.C., Chun, Y., Westphal, D., Holben, B. N., Geymard, C., McKendry, I., Kuring, N., Feldman, G. C., McClain, C., Frouin, R. J., Merrill, J., DuBois, D., Vignola, F., Murayama, T., Nickovic, S., Wilson, W. E., Sassen, K. and Sugimoto, N.: 2001, ‘The Asian dust events of April 1998’, J. Geophys. Res. 106(D16), 18317–18330.
Igarashi, Y., Otsuji-Hatori, M. and Hirose, K.: 1996, ‘Recent deposition of 90Sr and 137Cs observed in Tsukuba’, J. Environ. Radioactivity 31, 157–169.
Igarashi, Y., Aoyama, M., Hirose, K., Miyao, T. and Yabuki, S.: 2001, ‘Is it possible to use 90Sr and 137Cs as tracers for the aeolian transport?’, Water, Air, and Soil Pollution 130, 349–350.
Igarashi, Y.: 2002, ‘Approaches for dust transport by using resuspension of 90Sr and 137Cs’, J. Aerosol Research, Japan 10, 252–258 (in Japanese).
Igarashi, Y., Aoyama, M., Hirose, K., Miyao, T., Kazuhiro Nemoto, K., Tomita, M. and Fujikawa, T.: 2003, ‘Resuspension: Decadal monitoring time series of the anthropogenic radioactivity deposition in Japan’, J. Radiat. Res. 44, 319–328.
Intergovernmental Panel on Climate Change (IPCC): 2001, ‘Climate Chage 2001’, The Scientific Basis, Cambridge University Press, New York, USA.
Kanayama, S., Yabuki, S., Yanagisawa, F. and Motoyama, R.: 2002, ‘The chemical and strontium isotope composition of atmospheric aerosols over Japan: The contribution of long-range-transported Asian dust (Kosa)’, Atmos. Environ. 36, 5159–5175.
Katsuragi, Y.: 1983, ‘A study of 90Sr fallout in Japan’, Pap. Met. Geophys. 33, 277–291.
Kudo, A., Mahara, Y., Santry, D. C., Suzuki, T., Miyahara, S., Sugahara, M., Zheng, J. and Garrec, J.-P.: 1995, ‘Plutonium mass balance released from the Nagasaki A-bomb and the applicability for future environmental research’, Appl. Radiat. Isot. 46, 1089–1098.
Kurosakai, Y. and Mikami, Y.: 2003, ‘Recent frequent dust events and their relation to surface wind in East Asia’, Geophys. Res. Lett. 30, 1736, doi:10.1029/2003GL017261, 2003.
Krey, P. W. and Krajewsky, B.: 1970, ‘Comparison of atmospheric transport model calculations with observations of radioactive debris’, J. Geophys. Res. 75, 2901–2908.
Lee, S.-H., Pham, M. K. and Povinec, P. P.: 2002, ‘Radionuclide variations in the air over Monaco’, J. Radioanal. Nucl. Chem. 254, 445–453.
new Lee, H. N., Igarashi, Y., Chiba, M., Aoyama, M., Hirose, K. and Tanaka, T.: 2005, ‘Global model simulations of the transport of Asian and Sahara dust: Total deposition of dust mass in Japan’, (in press).
Lee, H. N., Tanaka, T., Chiba, M. and Igarashi, Y.: 2003, ‘Global transport of Asian dust from dust storms and its impact on Japan’, Water, Air, and Soil Pollution: Focus 3, 231–243.
Miller, J. R. and Reittemeier R. F.: 1963, ‘The leaching of radiostrontium and radiocesium through soils’, Soil Science Society Proceedings 141–144.
Miyake, Y., Saruhashi, K., Sugimura, Y., Kanazawa, T. and Hirose, K.: 1988, ‘Contents of 137Cs, plutonium and americium isotopes in the southern ocean waters’, Pap. Met. Geophys. 39, 95–113.
Miyao. T, Hirose, K., Aoyama, M. and Igarashi, Y.: 2000, ‘Trace of the resent deep water formation in the Japan Sea deduced from historical 137Cs data’, Geophys. Res. Lett. 27, 22, 3731–3734.
Nouira, A., Sayouty, E. H. and Benmansour, M.: 2003, ‘Use of 137Cs technique for soil erosion study in the agricultural region of Casablanca in Morocco’, J. Envirion. Radioactivity 68, 11–26.
Okada, A., Yabuki, S., Liu, C.-Q. and Huang Z.-W.: 1992, ‘Distribution of salt-constituting chemical species in the desert soils of the Turpan Basin and Junggar Basin, Xingjiang, China’, Journal of Arid Land Studies 2, 29–37.
Okada, K., Ikegami, M., Uchino, O., Nikaidou, Y., Zaizen, Y., Tsutsumi, Y. and Makino, Y.: 1992a, ‘Kuwaiti soot over Japan’, Nature 355, 120.
Okada, K., Ikegami, M., Uchino, O., Nikaidou, Y., Zaizen, Y., Tsutsumi, Y. and Makino, Y.: 1992b, ‘Extremely high proportions of soot particles in the upper troposphere over Japan’, Geophys. Res. Lett. 19, 921–924.
Ostuji-Hatori, M., Igarashi, Y. and Hirose, K.: 1994, ‘Preparation of a reference fallout material for the radioactivity measurement’, J. Environ. Radioactivity 31, 143–155.
Papastefanou, C. and Manolopoulou, M.: 1989, ‘The radioactivity of coloured rain in Thessaloniki, Greece’, The Science of the Total Environment 80, 225–227.
Papastefanou, C., Manolopoulou, M., Stoulos, S., Ioannidou, A. and Geraspoulos, E.: 2001, ‘Coloured rain dust from Sahara Desert is still radioactive’, J. Environ. Radioactivity 55, 109–112.
Prospero, J. M., Ginoux, P., Torres, O., Nicholson, S. E. and Gill, E.: 2002, ‘Environmental charcterization of global sources of atmospheric soil dust identified with the Nimbus 7 total ozone mapping spectrometer (TOMS) absorbing aerosol product’, Rev. Geophys. 40, 1002, doi: 10.1029/2000RG000095.
Rosner, G. and Winkler, R.: 2001, ‘Long-term variation (1986–1998) of post-Chernobyl 90Sr, 137Cs, 238Pu and 239,240Pu concentrations in air, depositions to ground, resuspension factors and resuspension rates in south Germany’, Sci. Total Environ. 273, 11–25.
Ritchie, J. C. and McHenry J. R.: 1990, ‘Application of radioactive fallout cesium-137 for measuring soil erosion and sediment accumulation rates and patterns: A review’, J. Environ. Qual. 19, 215–233.
Shao, Y.: 2000, Physics and Modeling of Wind Erosion, Kluwer Academic Publishers, Dordrecht/ Boston/ London pp. 118–119.
Shenber, M. A.: 2001, ‘Fallout 137Cs in soils from north western Libya’, J. Radioanal. Nucl. Chem. 250, 193–194.
Tazaki, K., Wakimoto, R., Minami, Y., Yamamoto, M., Miyata, K., Sato, K., Saji, I., Chaerun, S. K., Zou, G., Morishita, T., Asada, R., Segawa, H., Imanishi, H., Kato, R., Otani, Y. and Watanabe, T.: 2004, ‘Transport of carbon-bearing dusts from Iraq to Japan during Iraq's war’, Atmos. Environ. 38, 2091–2109.
United Nations Scientific Committee on the Effects of Atomic Radiation (UNSCEAR): 2000, Sources and effects of ionizing radiation. United Nations Scientific Committee on the Effects of Atomic Radiation 2000 report to the general assembly with scientific annexes. New York, United Nations.
World Meteorological Organization (WMO): 1993, GAW report No. 86, The Global Atmosphere Watch Guide, (WMO TD No. 553).
Yabuki, S., Okada, A., Takahashi, K., Liu, C.-Q., Zhang, J., Fan, Z.-L., Tian, C.-Y. and Chang, Q.: 1993, ‘The compositions of strontium isotopes in water, soil and salt samples from the desert area of Xingjiang, China’, Proceedings of the Japan-China International Symposium on the Study of the Mechanism of Desertification, March 2–4, 1993, Tsukuba.
Yamamoto, M., Tsumura, A. and Tsukatani, T.: 1998, ‘Current levels of Pu isotopes and 137Cs at the former Soviet Union's Semipalatinsk Nuclear Test Site’, Radiochim. Acta 81, 21–28.
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Igarashi, Y., Aoyama, M., Hirose, K. et al. What Anthropogenic Radionuclides (90Sr and 137Cs in Atmospheric Deposition, Surface Soils and Aeolian Dusts Suggest for Dust Transport over Japan. Water Air Soil Pollut: Focus 5, 51–69 (2005). https://doi.org/10.1007/s11267-005-0726-z
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DOI: https://doi.org/10.1007/s11267-005-0726-z