Abstract
The 238U, 226Ra and 232Th contents of six samples from the Mandena black sand placer deposit were determined by gamma-ray spectrometry and varied from 2280 to 4600 Bq/kg, 1530 to 2900 Bq/kg and 11,600 to 25,400 Bq/kg, respectively. The activity concentration of 232Th is significantly higher than 238U and there is no equilibrium between 238U and 226Ra. Due to the gamma interferences at the line 1461 keV and very high 228Ac activity, the 40K was calculated through potassium analyzed using ICP-AES and varied from 1 to 19 Bq/kg. The calculated gamma absorbed dose rate ranged from 7700 to 16,700 nGy/h.
Similar content being viewed by others
References
Alencar AS, Freitas AC (2005) Reference levels of natural radioactivity for the beach sands in a Brazilian southeastern coastal region. J Radiat Meas 40:76–83
Freitas AC, Alencar AS (2004) Gamma dose rates and distribution of natural radionuclides in sand beaches, Ilha Grande Southeastern Brazil. J Environ Radioact 75:211–223
Mohanty AK, Sengupta D, Das SK, Saha SK, Van KV (2004) Natural radioactivity and radiation exposure in the high background area at Chhatrapur beach placer deposit of Orissa, India. J Environ Radioact 75:15–33
Nada A, Abd EM, Abu ZH, El-Asy IE, Mostafa SMI, Abd EA (2012) Correlation between radionuclides associated with zircon and monazite in beach sand of Rosetta, Egypt. J Radioanal Nucl Chem 291:601–610
Papadopoulos A, Christofides G, Koroneos A, Stoulos S (2014) Natural radioactivity distribution and gamma radiation exposure of beach sands from Sithonia Peninsula. Central Eur J Geosci 6:229–242
Papadopoulos A, Koroneos A, Christofides G, Papadopoulou L, Tzifas I, Stoulos S (2016) Assessment of gamma radiation exposure of beach sands in highly touristic areas associated with plutonic rocks of the Atticocycladic zone (Greece). J Environ Radioact 162:235–243
Papadopoulos A, Koroneos A, Christofides G, Stoulos S (2014) Natural radioactivity distribution and gamma radiation exposure of beach sands close the granitoids of NE Chalkidiki, Greece. In: Proceedings of the 10th international congress of the hellenic geographical society, pp 805–814
Papadopoulos A, Koroneos A, Christofides G, Stoulos S (2015) Natural radioactivity distribution and gamma radiation exposure at beach sands close to Kavala pluton, Greece. Open J Geosci 1:407–422
Papadopoulos A, Koroneos A, Christofides G, Stoulos S (2015) Natural radioactivity distribution and gamma radiation exposure of beach sands close to Maronia and Samothraki plutons, NE Greece. Geol Balc 43:99–107
Primal P, Narayana Y (2014) Studies on the seasonal variation and vertical profiles of natural radionuclides in high background radiation areas of Kerala on the south west coast of India. J Radioanal Nucl Chem 302:813–817
Sulekha R, Sengupta D, Guin R, Saha SK (2009) Natural radioactivity measurements in beach sand along southern coast of Orissa, eastern India. Environ Earth Sci 59:593–601
Kumar R, Mahur AK, Rao NS, Sengupta D, Prasad R (2008) Radon exhalation rate from sand samples from the newly discovered high background radiation area at Erasama beach placer deposit of Orissa, India. J Radiat Meas 43:15–33
Abb El Wahab M, El Nahas HA (2013) Radionuclides measurements and mineralogical studies on beach sands, East Rosetta Estuary, Egypt. Chin J Geochem 32:146–156
United Nations Scientific Committee on the Effects of Atomic Radiation (UNSCEAR) (2000) Report to the general assembly, with scientific annexes (UNCEAR 2000), vol 1. Annex B - exposures from natural radiation sources, pp 84–141
A report by Harbinson R, Head of Environment at Panos London (2007). https://friendsoftheearth.uk/sites/default/files/downloads/development_recast.pdf. Accessed 28 June 2018
Kill J, Franchi G (2016) Rio Tinto in Madagascar: a mine destroying the unique biodiversity of the littoral zone of Fort Dauphin. WRM and Re: Common, pp 1–32
Lantoarindriaka A (2016) Master thesis: “Mineral composition of heavy fraction from beach sand and technological sand process, Fort-Dauphin, Madagascar”. In: AGH UST, Krakow, Poland
Gaylord L (2016) Rio Tinto QIT Madagascar minerals report
Jodłowski P, Kalita SJ (2010) Gamma-ray spectrometry laboratory for high-precision measurements of radionuclide concentrations in environmental samples. Nukleonika 55:143–148
Jodłowski P (2006) Self-absorption correction in gamma-ray spectrometry of environmental samples—an overview of methods and correction values obtained for the selected geometries. Nukleonika 51:21–25
Debertin K, Helmer RG (1988) Gamma- and X-ray spectrometry with semiconductor detectors. North-Holland Publications, Amsterdam
DDEP, Decay Data Evaluation Project. http://www.nucleide.org/DDEP_WG/DDEPdata.htm. Accessed 20 Jan 2018
Currie LA (1995) Nomenclatutre in evaluation of analytical methods including detection and quantification capabilities. Pure Appl Chem 67:1699–1723
Drever J (1997) The geochemistry of natural waters. Prentice Hall, New Jersey
Hoatson DM, Jaireth S, Miezitis Y (2011) The major rare earth element deposits of Australia: geological setting, exploration, and resources. Geosc Aust 204:192
Alexandre P, Kyser K, Layton-Matthews D, Yoy B (2015) Chemical composition of natural uraninite. Can Mineral 53:595–622
Wuana RA, Okieimen FE (2011) Heavy metals in contaminated soils: a review of sources, chemistry, risks and best available strategies for remediation. ISRN Ecol. https://doi.org/10.5402/2011/402647
Pehlivanovic B, Avdic S, Gazdic I, Osmanovic A (2016) Measurement of natural environmental radioactivity and estimation of population exposure in Bihac, Bosnia and Herzegovina. J Radioanal Nucl Chem. https://doi.org/10.1007/s10967-016-5155-0
Punniyakotti J, Ponnusamy V (2017) Depth-wise distribution of 238U, 232Th and 40K in sand samples of high background radiation areas (Tamilnadu coast), India. J Radioanal Nucl Chem. https://doi.org/10.1007/s10967-017-5167-4
Wang J, Liu J, Chan Y, Song G, Chaen D, Xiao T, Wu S, Chen F, Yin M (2016) Technologically elevated natural radioactivity and assessment of dose to workers around a granitic uranium deposit area, China. J Radioanal Nucl Chem 1:1. https://doi.org/10.1007/s10967-016-4809-2
Acknowledgements
The work was partly supported by the Ministry of Science and Higher Education (Grant Nos. 11.11.140.645 and 11.11.220.01). The authors would like to express their thankfulness to Drs Beata Ostachowicz and Jakub Nowak for their useful discussions. Many thanks to the colleague from Madagascar, Ms. Lantoarindriaka for providing samples.
Author information
Authors and Affiliations
Corresponding author
Rights and permissions
About this article
Cite this article
Van Hao, D., Nguyen Dinh, C., Jodłowski, P. et al. High-level natural radionuclides from the Mandena deposit, South Madagascar. J Radioanal Nucl Chem 319, 1331–1338 (2019). https://doi.org/10.1007/s10967-018-6378-z
Received:
Published:
Issue Date:
DOI: https://doi.org/10.1007/s10967-018-6378-z