Abstract
A dynamic compartment model was developed to estimate 137Cs concentrations in both seawater and sediment that had been released in the TEPCO’s Fukushima Daiichi Nuclear Power Plant 2011 accident. The model parameters were set from the best fitting of the results observed at the two closest sampling stations to the FDNPP site, then applied these parameters to three other stations located about 15–43 km away from the FDNPP. The 137Cs concentrations in seawater and sediment estimated by the developed model agreed well with observation results for these stations.
Similar content being viewed by others
References
Ministry of Health Labour and Welfare, Japan (2014) Levels of radioactive contaminants in foods tested in respective prefectures. http://www.mhlw.go.jp/english/topics/2011eq/index_food_radioactive.html. Accessed 17 Oct 2014
Iwata K, Tagami K, Uchida S (2013) Ecological half-lives of radiocesium in 16 species in marine biota after the TEPCO Fukushima Daiichi Nuclear Power Plant accident. Environ Sci Technol 47:7696–7703
Tateda Y, Tsumune D, Tsubono T (2013) Simulation of radioactive cesium transfer in the southern Fukushima coastal biota using a dynamic food chain transfer model. J Environ Radioact 124:1–12
Wada T, Nemoto Y, Shimamura S, Fujita T, Mizuno T, Sohtome T, Kamiyama K, Morita T, Igarashi S (2013) Effects of the nuclear disaster on marine products in Fukushima. J Environ Radioact 124:246–254
Garnier-Laplace J, Beaugelin-Seiler K, Hinton TG (2011) Fukushima wildlife dose reconstruction signals ecological consequences. Environ Sci Technol 45:5077–5078
Børretzen P, Salbu B (2002) Fixation of Cs to marine sediments estimated by a stochastic modeling approach. J Environ Radioact 61:1–20
Aldridge JN, Kershaw P, Brown J, McCubbin D, Leonard KS, Young EF (2003) Transfer of plutonium (239/240Pu) and caesium (137Cs) in the Irish Sea: comparison between observations and results from sediment and contaminant transport modelling. Cont Shelf Res 23:869–899
Gao Y, Drange H, Bentsen M, Johannsenn OM (2004) Simulating transport of non-Chernobyl 137Cs and 90Sr in the North Atlantic-Arctic region. J Environ Radioact 71:1–16
Periáñez R (2004) Testing the behaviour of different kinetic models for uptake/release of radionuclides between water and sediments when implemented in a marine dispersion model. J Environ Radioact 71:243–259
Toscano-Jimenez M, García-Tenorio R (2004) Modelling the dispersion of 137Cs in marine ecosystems with Monte Carlo methods. Nucl Instrum Methods B 213:779–783
Nakano M, Povinec P (2003) Oceanic general circulation model for the assessment of the distribution of 137Cs in the world ocean. Deep-sea Res Part II 50:2803–2816
Aoyama M, Tsumune D, Uematsu M, Kondo F, Hamajima Y (2012) Temporal variation of 134Cs and 137Cs activities in surface water at stations along the coastline near the Fukushima Dai-ichi Nuclear Power Plant accident site, Japan. Geochem J 46:321–325
Masumoto Y, Miyazawa Y, Tsumune D, Tsubono T, Kobayashi T, Kawamura H, Estournel C, Marsaleix P, Lanerolle L, Mehra A, Garraffo ZD (2012) Oceanic dispersion simulations of 137Cs released from the Fukushima Daiichi nuclear power plant. Elements 8:201–206
Nakano M, Povinec PP (2012) Long-term simulations of the 137Cs dispersion from the Fukushima accident in the world ocean. J Environ Radioact 111:109–115
Tsumune D, Tsubono T, Aoyama M, Hirose K (2012) Distribution of oceanic 137Cs from the Fukushima Dai-ichi Nuclear Power Plant simulated numerically by a regional ocean model. J Environ Radioact 111:100–108
Tumune D, Tsubono T, Aoyama M, Uematsu M, Misumi K, Maeda Y, Yoshida Y, Hayami H (2013) One-year, regional-scale simulation of 137Cs radioactivity in the ocean following the Fukushima Daiichi Nuclear Power Plant accident. Biogeosci Discuss 10:6259–6314
Oikawa S, Takata H, Watabe T, Misonoo J, Kusakabe M (2013) Distribution of the Fukushima-derived radionuclides in seawater in the Pacific off the coast of Miyagi, Fukushima, and Ibaraki Prefectures, Japan. Biogeosciences 10:5031–5047
Kusakabe M, Oikawa S, Takata H, Misonoo J (2013) Spatiotemporal distribution of Fukushima-derived radionuclides in nearby marine surface sediments. Biogeosciences 10:5019–5030
Otosaka S, Kobayashi T (2013) Sedimentation and remobilization of radiocesium in the coastal area of Ibaraki, 70 km south of the Fukushima Dai-ichi Nuclear Power Plant. Environ Monit Assess 185:5419–5433
Otosaka S, Kato Y (2014) Radiocesium derived from the Fukushima Daiichi Nuclear Power Plant accident in seabed sediments: initial deposition and inventories. Environ Sci Process Impacts 16:978–990
Misumi K, Tsumune D, Tsubono T, Tateda Y, Aoyama M, Kobayashi T, Hirose K (2014) Factors controlling the spatiotemporal variations of 137Cs in seabed sediment off the Fukushima coast: implications from the numerical simulations. J Environ Radioact 136:218–228
Desai DVM, Kumar SS, Pillai KC (1994) Influence of major cations of sea water on the desorption of 137Cs from marine sediments. J Radioanal Nucl Chem Lett 187:197–205
Sugai SF, Alperin MJ, Reeburgh WS (1994) Episodic deposition and 137Cs immobility in Skan Bay sediments: a ten-year 210Pb and 137Cs time series. Mar Geol 116:351–372
McKay WA, Baxter MS (1985) The partitioning of sellafield-derived radiocaesium in Scottish coastal sediment. J Environ Radioact 2:93–114
Nuclear Regulation Authority (2014) Monitoring plan of marine enviroment. http://radioactivity.nsr.go.jp/ja/contents/10000/9073/24/204_3_20140401.pdf (in Japanese). Accessed 17 Oct 2014
TEPCO (2014) Readings of radioactivity monitoring results in seawater near the Fukushima Daiichi NPP site. www.tepco.co.jp/nu/fukushima-np/f1/smp/2014/images/seawater-newest01-j.csv (in Japanese). Accessed 17 Oct 2014
TEPCO (2014) Readings of radioactivity monitoring results near the Fukushima Daiichi Nuclear Power Plant site, From Dec 2011 to Sep 2014. http://www.tepco.co.jp/nu/fukushima-np/f1/smp/indexold-j.html (in Japanese). Accessed 17 Oct 2014
TEPCO (2014) Readings of radioactivity monitoring results near the Fukushima Daiichi Nuclear Power Plant site, From Mar 2011 to Nov 2011. http://www.tepco.co.jp/nu/fukushima-np/f1/index2-j.html (in Japanese). Accessed 17 Oct 2014
Nuclear Regulation Authority (2014) Readings of sea area monitoring, http://radioactivity.nsr.go.jp/en/list/205/list-1.html. Accessed 17 Oct 2014
Kamei-Ishikawa N, Uchida S, Tagami K (2008) Distribution coefficients for 85Sr and 137Cs in Japanese agricultural soils and their correlations with soil properties. J Radioanal Nucl Chem 277:433–439
Fuhrmann M, Zhou H, Neiheisel J, Schoonen MAA, Dyer R (1997) Sorption/desorption of radioactive contaminants by sediment from the Kara Sea. Sci Total Environ 202:5–24
Amano H, Takahashi T, Uchida S, Matsuoka S, Ikeda H, Hayashi H, Kurosawa N (2003) Development of a code MOGRA for predicting the migration of ground additions and its application to various land utilization areas. J Nucl Sci Technol 40:975–979
Oughton DH, Børretzen P, Salbu B, Tronstad E (1997) Mobilisation of 137Cs and 90Sr from sediments: potential sources to arctic waters. Sci Total Environ 202:155–165
Carroll J, Boisson F, Teyssie JL, King SE, Krosshavn M, Carroll ML, Fowler SW, Povinec PP, Baxter MS (1999) Distribution coefficients (K d’s) for use in risk assessment models of the Kara Sea. Appl Radiat Isot 51:12–129
Tagami K, Uchida S (2013) Sediment-seawater distribution coefficient for radionuclides and estimation of radionuclide desorption ratio from soil in seawater. Bunseki Kagaku 62:527–533
Acknowledgments
This work was partially supported by the Agency for Natural Resources and Energy, the Ministry of Economy, Trade and Industry (METI), Japan.
Author information
Authors and Affiliations
Corresponding author
Rights and permissions
About this article
Cite this article
Yamamoto, K., Tagami, K., Uchida, S. et al. Model estimation of 137Cs concentration change with time in seawater and sediment around the Fukushima Daiichi Nuclear Power Plant site considering fast and slow reactions in the seawater-sediment systems. J Radioanal Nucl Chem 304, 867–881 (2015). https://doi.org/10.1007/s10967-014-3897-0
Received:
Published:
Issue Date:
DOI: https://doi.org/10.1007/s10967-014-3897-0