Skip to main content
Log in

Determination of sorption characteristics for artificial radionuclides in the hydrosphere

  • Published:
Journal of Radioanalytical and Nuclear Chemistry Aims and scope Submit manuscript

Abstract

Adsorption onto solid particles plays an important role in the transport of radioactive contaminants in the hydrosphere. Sorption is usually described with a distribution coefficient: a ratio of radioactivity fixed on solid phase and dissolved in water in equilibrium. In this study, we developed, optimised and verified a method that uses a series of batch experiments for determination of the distribution coefficients of radionuclides in sediment–water and suspended solids–water systems. This can be further used for describing radionuclide behaviour in river courses. This work was funded by the Czech Ministry of Interior, as a part of Safety research project.

This is a preview of subscription content, log in via an institution to check access.

Access this article

Price excludes VAT (USA)
Tax calculation will be finalised during checkout.

Instant access to the full article PDF.

Fig. 1
Fig. 2
Fig. 3

Similar content being viewed by others

References

  1. Violante A (2013) Elucidating mechanisms of competitive sorption at the mineral/water interface. In: Sparks DL (ed) Advances in agronomy, vol 118. Elsevier, Burlington, pp 111–176

  2. Brown GE, Calas G (2012) Mineral-aqueous solution interfaces and their impact on the environment. Geochem Perspect 4–5:483–742

    Article  Google Scholar 

  3. Das DK, Kumar S, Pathak PN, Tomar BS, Manchanda VK (2011) Sorption of Am(III) on natural sediment: experiment and modeling. J Radioanal Nucl Chem 289:137–143

    Article  CAS  Google Scholar 

  4. Garnier J-M, Ciffroy P, Benyahya L (2006) Implications of short and long term (30 days) sorption on the desorption kinetic of trace metals (Cd, Zn Co, Mn, Fe, Ag, Cs) associated with river suspended matter. Sci Total Environ 366:350–360

    Article  CAS  Google Scholar 

  5. Mu D, Du J, Li D, Song H, Yan S, Gu Y (2006) Sorption/desorption of radiozinc on the surface sediments. J Radioanal Nucl Chem 273:585–589

    Article  Google Scholar 

  6. IAEA (2010) Handbook of parameter values for the prediction of radionuclide transfer in terrestrial and freshwater environments. IAEA, Vienna

    Google Scholar 

  7. Pique A, Arcos D, Grandia F, Molinero J, Duro L, Berglund S (2013) conceptual and numerical modeling of radionuclide transport and retention in near-surface systems. Ambio 42:476–487

    Article  CAS  Google Scholar 

  8. Ciffroy P, Durrieu G, Garnier J-M (2009) Probabilistic distribution coefficients (Kds) in freshwater for radioisotopes of Ag, Am, Ba, Be, Ce Co, Cs, I, Mn, Pu, Ra, Ru, Sb, Sr and Th: implications for uncertainty analysis of models simulating the transport of radionuclides in rivers. J Environ Radioact 100:785–794

    Article  CAS  Google Scholar 

  9. Man C, Kwok Y (2001) Assessment of risk to Hong Kong due to accidental releases of radionuclides from a nearby nuclear power plant. J Radioanal Nucl Chem 3:485–490

    Article  Google Scholar 

  10. EPA (2012) Batch-type procedures for estimating soil adsorption for chemicals. BiblioGov, Windsor

    Google Scholar 

  11. ASTM C1733–10 (2002) Standard test method for distribution coefficients of inorganic species by the batch method. ASTM International, West Conshohocken

    Google Scholar 

  12. Duursma EK (1984) Problems of sediment sampling and conservation for radionuclide accumulation studies. IAEA, Vienna

    Google Scholar 

  13. Granados F, Bertin V, Bulbulian S, Solache-Ríos M (2006) 60Co aqueous speciation and pH effect on the adsorption behavior on inorganic materials. Appl Radiat Isot 64:291–297

    Article  CAS  Google Scholar 

  14. Kaplan DI, Serkiz SM, Allison JD (2010) Europium sorption to sediments in the presence of natural organic matter: a laboratory and modeling study. Appl Geochem 25:224–232

    Article  CAS  Google Scholar 

Download references

Acknowledgments

This work was prepared with the support of Project VG20122015088 sponsored by the Czech Ministry of Interior.

Author information

Authors and Affiliations

Authors

Corresponding author

Correspondence to Eva Juranová.

Rights and permissions

Reprints and permissions

About this article

Check for updates. Verify currency and authenticity via CrossMark

Cite this article

Juranová, E., Hanslík, E. Determination of sorption characteristics for artificial radionuclides in the hydrosphere. J Radioanal Nucl Chem 304, 21–26 (2015). https://doi.org/10.1007/s10967-014-3665-1

Download citation

  • Received:

  • Published:

  • Issue Date:

  • DOI: https://doi.org/10.1007/s10967-014-3665-1

Keywords

Navigation