Abstract
The nature of the pseudogap in the quasiparticle spectral density in high-T c cuprates is a matter of intense debate. In this study we have investigated the effects of Zn substitution on the uniform (\(\boldsymbol{q}=0\), where \(\boldsymbol{q}\) is the wave vector) magnetic susceptibility, χ(T), of La2−x Sr x Cu1−y Zn y O4 sintered samples with different hole concentrations, p(≡x), over a wide range of Zn contents (y). Non-magnetic Zn suppressed T c most effectively and enhanced χ(T) systematically at low temperatures. We have extracted the characteristic pseudogap energy scale, ε g, from the analysis of χ(T) data. Unlike T c,ε g was found to be fairly insensitive to the level of Zn substitution, even when T c was completely suppressed by Zn. The Zn-induced Curie-like enhancement of the χ(T) was also found to be closely related to the PG energy scale. We discuss the possible implications of these findings in this paper.
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Hussey, N.E.: Advances in Physics 51, 1685 (2002)
Lee, P.A.: Rep. Prog. Phys. 71, 012501 (2008)
Tarascon, J.M., Greene, L.H., Barboux, P., Mckinnon, W.R., Hull, G.W., Orlando, T.P., Delin, K.A., Foner, S., NcNiff Jr. E.J.: Phys. Rev. B 36, 8393 (1987)
Alloul, H., Mendels, P., Casalta, H., Marucco, J.F., Arabski, J.: Phys. Rev. Lett. 67, 3140 (1991)
Zagoulaev, S., Monod, P., Jegoudez, J.: Phys. Rev. B 52, 10474 (1995)
Islam, R.S., Cooper, J.R., Loram, J.W., Naqib, S.H.: Physica C 460–462, 753 (2007)
Alloul, H., Bobroff, J., Gabay, M., Hirschfeld, P.J.: Rev. Mod. Phys. 81, 45 (2009)
Islam, R.S., Cooper, J.R., Loram, J.W., Naqib, S.H.: Phys. Rev. B 81, 054511 (2010)
Naqib, S.H., Cooper, J.R., Tallon, J.L., Panagopoulos, C.: Physica C 387, 365 (2003)
Walker, D.J.C., Mackenzie, A.P., Cooper, J.R.: Phys. Rev. B 51, 15653 (1995)
Naqib, S.H., Cooper, J.R., Tallon, J.L., Islam, R.S., Chakalov, R.A.: Phys. Rev. B 71, 054502 (2005)
Naqib, S.H., Cooper, J.R., Islam, R.S., Tallon, J.L.: Phys. Rev. B 71, 184510 (2005)
Loram, J.W., Mirza, K.A., Wade, J.M., Cooper, J.R., Liang, W.Y.: Physica C 235–240, 134 (1994)
Nakano, T., Oda, M., Manabe, C., Momono, N., Miura, Y., Ido, M.: Phys. Rev. B 49, 1600 (1994)
Mendels, P., Bobroff, J., Collin, G., Alloul, H., Gabay, M., Marucco, J.F., Blanchard, N., Grenier, B.: Europhys. Lett. 46, 678 (1999)
Obertelli, S.D., Cooper, J.R., Tallon, J.L.: Phys. Rev. B 46, 14928 (1992)
Tallon, J.L., Cooper, J.R., De Silva, P.S.I.P.N., Williams, G.V.M., Loram, J.L.: Phys. Rev. Lett. 75, 4114 (1995)
Islam, R.S.: Ph.D. thesis. University of Cambridge, UK (2005)
Cooper, J.R., Loram, J.W.: J. Phys. I (France) 6, 2237 (1996)
Batlogg, B., Hwang, H.Y., Takagi, H., Cava, R.J., Kao, H.L., Kwo, J.: Physica C 235–240, 130 (1994)
Walstedt, R.E., Bell, R.F., Schneemeyer, L.F., Waszczak, J.V., Espinosa, G.P.: Phys. Rev. B 45, 8074 (1992)
Allgeier, C., Schilling, J.S.: Phys. Rev. B 48, 9747 (1993)
Blundell, S.: Magnetism in Condensed Matter. Oxford University Press, London (2001)
Loram, J.W., Luo, J., Cooper, J.R., Liang, W.Y., Tallon, J.L.: J. Phys. Chem. Solids 62, 59 (2001)
Naqib, S.H., Islam, R.S.: Supercond. Sci. Tech. 21, 105017 (2008)
Islam, R.S., Naqib, S.H.: Physica C 470, 79 (2010)
Hüfner, S., Hossain, M.A., Damascelli, A., Sawatzky, G.A.: Rep. Prog. Phys. 71, 062501 (2008)
Liang, W.Y., Loram, J.W., Mirza, K.A., Athanassopoulou, N., Cooper, J.R.: Physica C 263, 277 (1996)
Doiron-Leyraud, N., Proust, C., LeBoeuf, D., Levallois, J., Bonnemaison, J.-B., Liang, R., Bonn, D.A., Hardy, W.N., Taileffer, L.: Nature 447, 565 (2007)
Yelland, E.A., Singleton, J., Meilke, C.H., Harrison, N., Balakirev, F.F., Dabrowski, B., Cooper, J.R.: Phys. Rev. Lett. 100, 047003 (2008)
Sebastian, S.E., Harrison, N., Palm, E., Murphy, T.P., Meilke, C.H., Liang, R., Bonn, D.A., Hardy, W.N., Lonzarich, G.G.: Nature 454, 200 (2008)
Tallon, J.L., Loram, J.W.: Physica C 349, 53 (2001) and references therein
Kao, Y.J., Iyenger, A.P., Stajic, J., Levin, K.: Phys. Rev. B 66, 214519 (2002)
Sonier, J.E., Ilton, M., Pacradouni, V., Kaiser, C.V., Sabok-Sayr, S.A., Ando, Y., Komiya, S., Hardy, W.N., Bonn, D.A., Liang, R., Atkinson, W.A.: Phys. Rev. Lett. 101, 117001 (2008)
Yuli, O., Asulin, I., Kalcheim, Y., Koren, G., Millo, O.: Phys. Rev. Lett. 103, 197003 (2009)
Parker, C.V., Pushp, A., Pasupathy, A.N., Gomes, K.K., Wen, J., Xu, Z., Ono, S., Gu, G., Yazdani, A.: Phys. Rev. Lett. 104, 117001 (2010)
Rullier-Albenque, F., Alloul, H., Tourbot, R.: Phys. Rev. Lett. 87, 157001 (2001)
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Islam, R.S., Hasan, M.M. & Naqib, S.H. Nature of the Pseudogap in High-T c Cuprates: Analysis of the Bulk Magnetic Susceptibility of La2−x Sr x Cu1−y Zn y O4 . J Supercond Nov Magn 23, 1569–1574 (2010). https://doi.org/10.1007/s10948-010-0814-9
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DOI: https://doi.org/10.1007/s10948-010-0814-9