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Effects of Substrate Relaxation on Adsorption in Pores

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Abstract

Fluids in porous media are commonly studied with analytical or simulation methods, usually assuming that the host medium is rigid. By evaluating the substrate’s response (relaxation) to the presence of the fluid we assess the error inherent in that assumption. One application is a determination of the ground state of 3He in slit and cylindrical pores. With the relaxation, there results a much stronger cohesion than would be found for a rigid host. Similar increased binding effects of relaxation are found for classical fluids confined within slit pores or nanotube bundles.

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Authors and Affiliations

  1. Department of Chemistry and Physics, Southeastern Louisiana University, Hammond, Louisiana, 70402, USA

    Hye-Young Kim

  2. Department of Physics and Astronomy, Howard University, 2355 Sixth Street NW, Washington, DC, 20059, USA

    Silvina M. Gatica

  3. Department of Chemistry, University of Cincinnati, Cincinnati, OH, 45221-0172, USA

    George Stan

  4. Department of Physics, Penn State University, University Park, PA, 16802, USA

    Milton W. Cole

Authors
  1. Hye-Young Kim
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  2. Silvina M. Gatica
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  3. George Stan
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  4. Milton W. Cole
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Correspondence to Silvina M. Gatica.

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Kim, HY., Gatica, S.M., Stan, G. et al. Effects of Substrate Relaxation on Adsorption in Pores. J Low Temp Phys 156, 1–8 (2009). https://doi.org/10.1007/s10909-009-9884-0

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  • DOI: https://doi.org/10.1007/s10909-009-9884-0

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