Skip to main content
Log in

Influence of Li2O–MgO–ZnO–B2O3–SiO2 glass doping on the microwave dielectric properties and sintering temperature of Li3Mg2NbO6 ceramics

  • Published:
Journal of Materials Science: Materials in Electronics Aims and scope Submit manuscript

Abstract

Li3Mg2NbO6 + x wt% Li2O–MgO–ZnO–B2O3–SiO2 (LMZBS, x = 2, 4, 6, 8, 10) microwave dielectric ceramics with the rock-salt structure were primarily investigated by the traditional solid-state method. The microstructures, microwave dielectric properties, and sintering characteristics were studied systematically according to the doping concentration and sintering temperature. It could be seen that the LMZBS glass effectively lower the sintering temperature of Li3Mg2NbO6 ceramics from 1250 to 925 °C with microwave dielectric properties changing as a function of the amounts of the LMZBS glass. The experimental results showed that 4 wt% LMZBS glass enabled Li3Mg2NbO6 ceramics sintered at 925 °C for 4 h to have excellent microwave dielectric properties: εr = 16.02, Q × f = 56,455 GHz, τf = − 18.81 ppm/°C. Therefore, Li3Mg2NbO6 ceramics doped with LMZBS glass meet the requirements of low-temperature co-fired ceramics.

This is a preview of subscription content, log in via an institution to check access.

Access this article

Price excludes VAT (USA)
Tax calculation will be finalised during checkout.

Instant access to the full article PDF.

Fig. 1
Fig. 2
Fig. 3
Fig. 4
Fig. 5
Fig. 6
Fig. 7
Fig. 8

Similar content being viewed by others

References

  1. I.M. Reaney, D. Iddles, J. Am. Ceram. Soc. 89, 2063–2072 (2006)

    CAS  Google Scholar 

  2. E.T. Thostenson, T.W. Chou, Compos. Pt. A-Appl. Sci. Manuf. 30, 1055–1071 (1999)

    Google Scholar 

  3. M.T. Sebastian, H. Jantunen, Int. Mater. Rev. 53, 57–90 (2008)

    CAS  Google Scholar 

  4. Y.P. Pu, J.W. Li, X.Y. Wang, Y. Shi, R.K. Shi, M.D. Yang, W. Wang, X. Guo, X. Peng, Compos. Sci. Technol. 186, 9 (2020)

    Google Scholar 

  5. L. Zhang, Y.P. Pu, M. Chen, Ceram. Int. 46, 98–105 (2020)

    CAS  Google Scholar 

  6. R.K. Shi, Y.P. Pu, W. Wang, X. Guo, J.W. Li, M.D. Yang, S.Y. Zhou, J. Alloy. Compd. 815, 8 (2020)

    Google Scholar 

  7. H.S. Ren, L. Hao, H.Y. Peng, M.Z. Dang, T.Y. Xie, Y. Zhang, S.H. Jiang, X.G. Yao, H.X. Lin, L. Luo, J. Eur. Ceram. Soc. 38, 3498–3504 (2018)

    CAS  Google Scholar 

  8. H.S. Ren, S.H. Jiang, M.Z. Dang, T.Y. Xie, H. Tang, H.Y. Peng, H.X. Lin, L. Luo, J. Alloy. Compd. 740, 1188–1196 (2018)

    CAS  Google Scholar 

  9. G. Wang, D.N. Zhang, X. Huang, Y.H. Rao, Y. Yang, G.W. Gan, Y.M. Lai, F. Xu, J. Li, Y.L. Liao, C. Liu, L.C. Jin, V.G. Harris, H.W. Zhang, J. Am. Ceram. Soc. 103, 214–223 (2020)

    CAS  Google Scholar 

  10. P. Zhang, K.X. Sun, M. Xiao, Z.T. Zheng, J. Am. Ceram. Soc. 102, 4127–4135 (2019)

    CAS  Google Scholar 

  11. L.L. Yuan, J.J. Bian, Ferroelectrics 387, 123–129 (2009)

    CAS  Google Scholar 

  12. H.L. Pan, Y.X. Mao, L. Cheng, H.T. Wu, J. Alloy. Compd. 723, 667–674 (2017)

    CAS  Google Scholar 

  13. P. Zhang, H. Xie, Y.G. Zhao, X.Y. Zhao, M. Xiao, J. Alloy. Compd. 690, 688–691 (2017)

    CAS  Google Scholar 

  14. G. Wang, H.W. Zhang, C. Liu, H. Su, L.J. Jia, J. Li, X. Huang, G.W. Gan, J. Electron. Mater. 47, 4672–4677 (2018)

    CAS  Google Scholar 

  15. G. Wang, H.W. Zhang, C. Liu, H. Su, J. Li, X. Huang, G.W. Gan, F. Xu, Mater. Lett. 217, 48–51 (2018)

    CAS  Google Scholar 

  16. T.Y. Qin, C.W. Zhong, H.C. Yang, Y. Qin, S.R. Zhang, Ceram. Int. 45, 10899–10906 (2019)

    CAS  Google Scholar 

  17. M.X. Wang, C.W. Zhong, T.Y. Qin, Q. Yang, B. Tang, S.R. Zhang, Ceram. Int. 46, 12088–12095 (2020)

    CAS  Google Scholar 

  18. P.L. Wang, M. Zhu, Y. Chen, F. Xie, N. Xiao, B. Hou, W. Lu, F.W. Jiang, W.Z. Zheng, Mater. Res. Express 6, 8 (2019)

    Google Scholar 

  19. Y.V. Bykov, K.I. Rybakov, V.E. Semenov, J. Phys. D-Appl. Phys. 34, R55–R75 (2001)

    CAS  Google Scholar 

  20. S. George, M.T. Sebastian, J. Alloy. Compd. 473, 336–340 (2009)

    CAS  Google Scholar 

  21. Y.C. Liou, Y.C. Wu, J. Electron. Mater. 46, 2387–2392 (2017)

    CAS  Google Scholar 

  22. X.H. Zhou, L.X. Xue, H.B. Sun, H.Y. Yang, S.R. Zhang, J. Mater. Sci.-Mater. Electron. 29, 643–649 (2018)

    CAS  Google Scholar 

  23. H.B. Bafrooei, M. Feizpour, A. Sayyadi-Shahraki, K.X. Song, J. Alloy. Compd. 834, 9 (2020)

    Google Scholar 

  24. L.X. Li, Z.D. Gao, Y.R. Liu, H.C. Cai, S. Li, Mater. Lett. 140, 5–8 (2015)

    CAS  Google Scholar 

  25. L.S. Xie, C.W. Zhong, Z.X. Fang, Y. Zhao, B. Tang, S.R. Zhang, J. Ceram. Soc. Jpn. 126, 163–169 (2018)

    CAS  Google Scholar 

  26. P. Zhang, J.W. Liao, Y.G. Zhao, X.Y. Zhao, M. Xiao, J. Mater. Sci.-Mater. Electron. 28, 686–690 (2017)

    CAS  Google Scholar 

  27. P. Zhang, L. Liu, Y.G. Zhao, M. Xiao, J. Mater. Sci.-Mater. Electron. 28, 5802–5806 (2017)

    CAS  Google Scholar 

  28. C. Luo, Y.D. Hu, S.X. Bao, T. Hong, L.B. Ai, J. Chen, Z.Z. Duan, J. Mater. Sci.-Mater. Electron. 29, 15523–15528 (2018)

    CAS  Google Scholar 

  29. T.W. Zhang, R.Z. Zuo, C. Zhang, Mater. Res. Bull. 68, 109–114 (2015)

    CAS  Google Scholar 

  30. L.P. Zhao, P. Liu, G.Q. Sun, Z.F. Fu, J. Mater. Sci.-Mater. Electron. 29, 5873–5877 (2018)

    CAS  Google Scholar 

Download references

Author information

Authors and Affiliations

Authors

Corresponding author

Correspondence to Xiaohua Zhou.

Additional information

Publisher's Note

Springer Nature remains neutral with regard to jurisdictional claims in published maps and institutional affiliations.

Rights and permissions

Reprints and permissions

About this article

Check for updates. Verify currency and authenticity via CrossMark

Cite this article

Zhou, X., Ning, X., Zhang, X. et al. Influence of Li2O–MgO–ZnO–B2O3–SiO2 glass doping on the microwave dielectric properties and sintering temperature of Li3Mg2NbO6 ceramics. J Mater Sci: Mater Electron 31, 17029–17035 (2020). https://doi.org/10.1007/s10854-020-04260-3

Download citation

  • Received:

  • Accepted:

  • Published:

  • Issue Date:

  • DOI: https://doi.org/10.1007/s10854-020-04260-3

Navigation