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Effect of different microwave power applied during microwave assisted radiant heating on the structure, dielectric and electrical properties of Ba0.8 Ca0.2 TiO3 ceramics

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Abstract

Microwave assisted radiant heating (MARH) is hybrid sintering technique, where conventional radiant heating is accompanied by precisely controlled different microwave power (Mw) percentages. Lead-free polycrystalline samples of (Ba, Ca) TiO3 BCT ceramics derived from hydrothermal process were synthesized by MARH technique. A systematic study has been carried out to examine the effect of different microwave power (Mw) percentages applied during MARH on the structure, dielectric and electrical properties of BCT samples. Room temperature X-ray diffraction pattern and Raman Scattering spectra revealed formation of single phase tetragonal structure for all the samples and tetragonality increases with increasing Mw power percentages. However, the dielectric permittivity shows maximum increment (ε′ ~ 16,000) for the samples sintered with 30 Mw power percentage. Impedance spectroscopic analysis suggested negative temperature coefficient of resistance (NTCR) behavior with non-Debye type dielectric relaxation. Electrical resistivity also increases with increasing Mw power percentages for all the samples. Samples sintered with 30 Mw power percentage exhibited enhanced dielectric and electrical properties.

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Acknowledgements

Authors wish to thank Dr V R Reddy, Dr V Sathe and Dr Mukul Gupta for MARH sintering, ferroelectric, X-ray Diffraction and RAMAN spectroscopic measurements of UGC-DAE Consortium for Scientific Research Indore Centre, Indore, India.

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Authors and Affiliations

  1. Materials Research Laboratory, Department of Physics, Anugrah Narayan College, Patna, 800013, India

    Arpana Singh, Md. Kashif Shamim & Seema Sharma

  2. School of Physics, Eternal University, Sirmour, Himachal Pradesh, 173101, India

    R. Rai

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  1. Arpana Singh
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  2. Md. Kashif Shamim
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  3. Seema Sharma
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  4. R. Rai
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Correspondence to Md. Kashif Shamim.

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Singh, A., Shamim, M.K., Sharma, S. et al. Effect of different microwave power applied during microwave assisted radiant heating on the structure, dielectric and electrical properties of Ba0.8 Ca0.2 TiO3 ceramics. J Mater Sci: Mater Electron 29, 8158–8166 (2018). https://doi.org/10.1007/s10854-018-8821-x

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  • DOI: https://doi.org/10.1007/s10854-018-8821-x

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