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Study of urban atmospheric pollution in Navarre (Northern Spain)

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Abstract

An ambient air quality study was undertaken in two cities (Pamplona and Alsasua) of the Province of Navarre in northern Spain from July 2001 to June 2004. The data were obtained from two urban monitoring sites. At both monitoring sites, ambient levels of ozone, NOx, and SO2 were measured. Simultaneously with levels of PM10 measured at Alsasua (using a laser particle counter), PM10 levels were also determined at Pamplona (using a beta attenuation monitor). Mean annual PM10 concentrations in Pamplona and Alsasua reached 30 and 28 ¼g m−3, respectively. These concentrations are typical for urban background sites in Northern Spain. By using meteorological information and back trajectories, it was found that the number of exceedances of the daily PM10 limit as well as the PM10 temporal variation was highly influenced by air masses from North Africa. Although North African transport was observed on only 9% of the days, it contributed the highest observed PM10 levels. Transport from the Atlantic Ocean was observed on 68% of the days; transport from Europe on 13%; low transport and local influences on 7%; and transport from the Mediterranean region on 3% of the days. The mean O3 concentrations were 45 and 55 μg m−3 in Pamplona and Alsasua, respectively, which were above the values reported for the main Spanish cities. The mean NO and NO2 levels were very similar in both sites (12 and 26 μg m−3, respectively). Mean SO2 levels were 8 μg m−3 in Pamplona and 5 μg m−3 in Alsasua. Hourly levels of PM10, NO and NO2 showed similar variations with the typically two coincident maximums during traffic rush hours demonstrating a major anthropogenic origin of PM10, in spite of the sporadic dust outbreaks.

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References

  • Aguinaga, I., Guillén, F., Oviedo, P. J., Floristán, M. Y., Laborda, M. S., Martínez, M. T., et al. (1999). Efectos a corto plazo de la contaminación atmosférica sobre la mortalidad: resultados del proyecto EMECAM en la ciudad de Pamplona, 1991’995. Revista Española de Salud Pública, 73, 253’58.

    Google Scholar 

  • Artiñano, B., Querol, X., Salvador, P., Rodríguez, S., Alonso, D., & Alastuey, A. (2001). Assessment of airborne particulate levels in Spain in relation to the new EU-directive. Atmospheric Environment, 35(Suplement no.1), S43–S53.

    Article  Google Scholar 

  • Baldasano, J. M., Jiménez, P., Parra, R., & Gassó, S. (2005). Modelling the ozone weekend effect in very complex terrains: A case study in the Northeastern Iberian Peninsula. Atmospheric Environment, 39, 429’44.

    Article  Google Scholar 

  • Baldasano, J. M., Valera, E., & Jiménez, P. (2003). Air quality data from large cities. Science of the Total Environment, 307, 141’65.

    Article  CAS  Google Scholar 

  • Blum, O., Bytnerowicz, A., Manning, W., & Popovicheva, L. (1997). Ambient tropospheric ozone in the Ukranian Carpathian Mountains and Kiev region: detection with passive samplers and bioindicators plants. Environmental Pollution, 98, 299’04.

    Article  CAS  Google Scholar 

  • Davison, A. W., & Barnes, J. D. (1998). Effects of ozone on wild plants. New Phytologist, 139, 135’51.

    Article  CAS  Google Scholar 

  • Dockery, D. W., Pope, C. A., Xu, X., Spengler, J. D.,Ware, J. H., Fay, M. E., et al. (1993). An association between air pollution and mortality in six US cities. New England Journal of Medicine, 329, 1753’759.

    Article  CAS  Google Scholar 

  • Draxler, R. R., & Rolph, G. D. (2003). HYSPLIT (HYbrid Single-Particle Lagrangian Integrated Trajectory). NOAA Air Resources Laboratory, Silver Spring, MD Web site: http://www.arl.noaa.gov/ready/hysplit4.html.

  • Escudero, M., Castillo, S., Querol, X., Avila, A., Alarcón, M., Viana, M. M., et al. (2005). Wet and dry African dust episodes over Eastern Spain. Journal of Geophysical Research, 110, D18S08. doi:10.1029/2004JD00473.

  • EU (1999). 1999/30/EC Council Directive relating to limit values for sulphur dioxide, nitrogen dioxide and oxide of nitrogen, particulate matter and lead in ambient air. The Council of the European Union.

  • EU (2002). 2002/3/EC Directive of the European Parliament and of the Council relating to ozone in ambient air. The European Parliament and the Council of the European Union.

  • Fenger, J. (1999). Urban air quality. Atmospheric Environment, 33, 4877’900.

    Article  CAS  Google Scholar 

  • Herman, J. R., Bhartia, P. K., Torres, Hsu, O., Seftor, C., & Celarier, E. (1997). Global distribution of UV-absorbing aerosols from Nimbus-7/TOMS data. Journal of Geophysical Research, 102, 16911’6923.

    Article  CAS  Google Scholar 

  • Kallos, G., Kotroni, V., & Lagouvardos. K. (1997). The regional weather forecasting system SKIRON: An overview. In Proceedings of the symposium on regional weather prediction on parallel computer environments (pp. 109’22), University of Athens, Greece.

  • Mayer, H. (1999). Air pollution in cities. Atmospheric Environment, 33, 4029’037.

    Article  CAS  Google Scholar 

  • McClain, C. R., Cleave, M. L., Feldman, G. C., Gregg, W. W., Hooker, S. B., & Kuring, N. (1998). Science quality SeaWiFS data for global biosphere research. Sea Technology, 39(9), 10’6.

    Google Scholar 

  • Monks, P. S. (2000). A review of the observations and origins of the spring ozone maximum. Atmospheric Environment, 34, 3545’561.

    Article  CAS  Google Scholar 

  • Population Reference Bureau (1998). World population data sheet. Demographic data and estimates for the countries and regions of the World. Washington D.C.: Population Reference Bureau.

    Google Scholar 

  • Pun, B. K., Seigneur, Ch., & White, W. (2003). Day-of-week behavior of atmospheric Ozono in three US cities. Air & Waste Management Association, 53, 789’01.

    CAS  Google Scholar 

  • Querol, X., Alastuey, A., Puicercus, J. A., Mantilla, E., Miró, J.V., Lopez-Soler, A., et al. (1998). Seasonal evolution of suspended particles around a large coal-fired power station: Particle levels and sources. Atmospheric Environment, 32, 1963’978.

    Article  CAS  Google Scholar 

  • Querol, X., Alsatuey, A., Rodríguez, S., Plana, F., Ruiz, CR., Cots, N., et al. (2001). PM10 and PM2.5 souerce apportionment in the Barcelona Metropolitan Area, Catalonia, Spain. Atmospheric Environment, 35, 6407’419.

    Article  CAS  Google Scholar 

  • Querol, X., Alsatuey, A., Rodríguez, S., Viana, M. M., Artíñano, B., Salvador, P., et al. (2004). Levels of particulate patter in rural, urban and industrial sites in Spain. Science of the Total Environment, 334’35, 359’76.

    Google Scholar 

  • Ribas, A., & Penuelas, J. (2004). Temporal patterns of surface ozone levels in different habitats of the North Western Mediterranean Basin. Atmospheric Environment, 38, 985’92.

    Google Scholar 

  • Riga-Karandinos, A. N., & Saitanis, C. (2005). Comparative assessment of ambient air quality in two tipical Mediterranean coastal cities in Greece. Chemosphere, 59, 1125’136.

    Article  CAS  Google Scholar 

  • Riga-Karandinos, A. N., Saitanis, C. J., & Arapis, G. (2006). Study of the weekday–weekend variation of air pollutants in a typical Mediterranean coastal town. International Journal of Environment and Pollution, 27(4), 300’12.

    CAS  Google Scholar 

  • Rodríguez, S., Querol, X., Alastuey, A., Kallos, G., & Kakaliagou, O. (2001). Saharan dust contributions to PM10 and TSP levels in Southern and Eastern Spain. Atmospheric Environment, 35/14, 2433’447.

    Article  Google Scholar 

  • Simpson, D. (1995). Biogenic emissions in Europe, 2, implications for ozone control strategies. Journal of Geophysical Research, 100, 891’06.

    Google Scholar 

  • US EPA (1997). National ambiennt air quality standars for particulate matter: Final rule. 40 CFR Part 50.

  • Viana, M., Querol, X., Alastuey, A., Gangoiti, G., & Menéndez, M. (2003). PM levels in the Basque country (Northern Spain): Analysis of a 5-year data record and interpretation of seasonal variations. Atmospheric Environment, 37, 2879’891.

    Article  CAS  Google Scholar 

  • Vignati, E., Berkowicz, R., & Hertel, O. (1996). Coparison of air quality in streets of Copenhagen and Milan, in view of the climatological conditons. Science of the Total Environment, 189’90, 467’73.

    Google Scholar 

  • Wiederkehr, P., & Yoon, S. J. (1998). Air quality indicators. In J. Fenger, O. Hertel, & F. Palmgren (Eds.), Urban Air Pollution, European Aspects (pp. 403’18). Dordrecht: Kluwer.

    Google Scholar 

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Correspondence to P. K. Hopke.

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Zabalza, J., Ogulei, D., Elustondo, D. et al. Study of urban atmospheric pollution in Navarre (Northern Spain). Environ Monit Assess 134, 137–151 (2007). https://doi.org/10.1007/s10661-007-9605-6

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  • DOI: https://doi.org/10.1007/s10661-007-9605-6

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