Skip to main content
Log in

Spectrum of prompt fission neutrons from 235U(n, F)

  • Published:
Atomic Energy Aims and scope

A new matrix of the spectra of prompt fission neutrons for the reaction 235U(n, F) has been obtained. The evaluated spectrum of prompt fission neutrons reproduces the measured data for incident neutrons with energy from thermal to 14.7 MeV. A solution is proposed for the problem of inconsistency of the integral testing of the systems with a thermal spectrum and differential measurements of the spectra of prompt fission neutrons. The matrix obtained for the spectra of prompt neutrons for 235U(n, F) eliminates the considerable discrepancy between the differential and integral experiments. The description of the integral experiments for compositions with a fast neutron spectrum revealed the compensation effect in the multiplication factor Keff, due to the difference in the shapes of the spectra of prompt fission neutrons, the present work and known libraries. The description of systems with a thermal neutron spectrum shows that the positive shift of the computed Keff is explained by the influence of the low-energy neutrons.

This is a preview of subscription content, log in via an institution to check access.

Access this article

Price excludes VAT (USA)
Tax calculation will be finalised during checkout.

Instant access to the full article PDF.

Similar content being viewed by others

References

  1. G. Aliberti, I. Kodeli, G. Palmiotti, and M. Salvatores, “Fission spectrum related uncertainties,” in: Proc. NEMEA-4 Neutron Measurements, Evaluations and Applications, Prague, Czech Republic, October 16–18, 2007, JRC-EU-IRMM (2008), pp. 135–138.

  2. R. Roussin, P. Young, and R. McKnight, “Current status of ENDF/BVI,” in: Proc. Int. Conf. Nucl. Data for Sci. and Technol, Gatlinburg, USA, May 9–13, 1994, ANS (1994), pp. 692–694.

  3. M. Chadwick, P. Oblozinsky, M. Herman, et al., “ENDF/BVH.O: next generation evaluated data library for nuclear science and technology,” Nucl. Data Sheets, 107, 2931–3060 (2006).

    Article  ADS  Google Scholar 

  4. K. Shibata, T. Kawano, T. Nakagawa, et al., “Japanese evaluated nuclear data library, version 3, revision-3: JENDL-3.3,” Nucl. Sci. Technol., 39, 1125–1200 (2002).

    Article  Google Scholar 

  5. B. I. Starostov, V. N. Nefedov, and A. A. Boitsov, “Spectra of prompt neutrons from fission of U-233, U-235, Pu-239 by thermal neutrons and spontaneous fission of Cf-252 in the energy interval 0.01–12 MeV,” Vopr. At. Nauk. Tekn., Ser. Yad. Konst., No. 3, 16–26 (1985).

  6. Wang Yufeng, Bai Xixiang, Li Anli, et al, “An experimental study of the prompt neutron spectrum of the 235U fission induced by thermal neutrons,” Chin. Nucl. Phys., 11, 47–54 (1989).

    ADS  Google Scholar 

  7. Fission Neutron Spectra of Uranium-235, NEA/WPEC-9, OECD (2003).

  8. International Reactor Dosimetry File 2002 (IRDF-2002), Technical Reports Ser. No. 452, IAEA, Vienna (2006).

  9. D. Madland and J. Nix, New calculation of prompt fission neutron spectra and average prompt neutron multiplicities,” Nucl. Sci. Eng., 81, 213–221 (1982).

    Google Scholar 

  10. P. Johansson, B. Holmquist, and T. Wiedling, “An experimental study of the prompt fission neutron spectrum induced by 0.5 MeV incident neutrons on U-235,” ibid., 62, 695–708 (1977).

    Google Scholar 

  11. D. Madland, “Total prompt energy release in the neutron-induced fission of 235U, 238U and 239Pu neutron spectra and average prompt neutron multiplicities,” Nucl. Phys., A 772, 131–151 (2006).

    Google Scholar 

  12. I. Kodeli, A. Trkov, R. Capote, et al., “Evaluation and use of the prompt fission neutron spectrum and spectra covariance matrices in criticality and shielding,” Nucl. Instrum. Meth. in Phys. Res A, 610, 540–552 (2009).

    Article  ADS  Google Scholar 

  13. N. V. Kornilov, A. B. Kagalenko, and F.-J. Hambsch, “Calculation of the spectra of fission neutrons on the basis of a new systematics of the experimental data,” Yad. Fiz., 62, 209–220 (1999).

    Google Scholar 

  14. J.-C Sublet, “JEFF-3.1, ENDF/BVII and JENDL-3.3 critical assemblies benchmarking with the Monte-Carlo code TRIPOLI,” IEEE Trans. Nucl. Sci., 55, 604–613 (2008).

    Article  ADS  Google Scholar 

  15. M. Jimenez Lopez, B. Morillon, and P. Romain, “Triple humped fission barrier model for a new 238U neutron cross section evaluation and first validation,” An. Nucl. Energy, 32, 195–213 (2005).

    Article  Google Scholar 

  16. I. Fabry, F.-J. Hambsch, N. V. Kornilov, et al., “New experimental 235U(n, f) prompt fission neutron spectrum and old disagreement between microscopic and microscopic data,” in: IV Int. Workshop on Nuclear Fission and Fiss. Product Spectr., Cadarache, France, May 13–16, 2009, ANS, NY (2009), pp. 249–256.

  17. N. V. Kornilov, F.-J. Hambsch, I. Fabry, et al., “235U prompt fission neutron spectrum at 100 K input neutron energy,” Nucl. Sci. Eng., 165, 117–127 (2010).

    Google Scholar 

  18. A. Lajtai, J. Kecskemeti, J. Safar, et al., “Prompt neutron spectra for energy range 30 keV–4 MeV from fission of U-233, U-235 and Pu-239 induced by thermal neutrons,” in: Proc. Int. Conf. on Nuclear Data for Science and Technology, Santa Fe, USA, 1986, Vol. 1, pp. 613–615.

  19. “Properties of neutron sources,” in: IAEA Advisory Group Meeting, Leningrad (USSR), June 9 –13, 1986, IAEATECDOC-410 (1987), pp. 158–168.

  20. International Evaluation of Neutron Cross-Section Standards. IAEA Special Technical Report, STI/PUB/1291, IAEA, Vienna (2007), pp. 99–109.

  21. B. Watt, “Energy spectrum of neutrons from thermal fission of 235U,” Phys. Rev., 87, 1037–1042 (1952).

    Article  ADS  Google Scholar 

  22. P. Staples, J. Egan, G. Kegel, et al., “Prompt fission neutron energy spectra induced by fast neutrons,” Nucl. Phys. A, 591, 41–51 (1995).

    Article  ADS  Google Scholar 

  23. A. M. Strufanov, G. N. Lovchikova, G. N. Smirenko, et al., “Measurement and evaluation of the average energy of neutrons from the reaction 235U(n, f),” Yad. Fiz., 53, 606–616 (1991).

    Google Scholar 

  24. JEFF 3.1.1. Nuclear Data Library Report 21, NEA No. 6190, OECD (2006).

  25. G. S. Boikov,V. D. Dmitriev, G. A. Kudyaev, et al., “Spectrum of neutrons with fission of Th-332, U-235, and U-338 by 2.9 and 14.7 MeV neutrons,” Yad. Fiz., 53, 628–648 (1991).

    Google Scholar 

  26. G. N. Lovchikova, G. N. Smirenkin, A. M. Trufanov, et al., “Ebergy distributions of secondary neutrons from (n, f) reactions for Th–Pu nuclei,” ibid., 62, 1551–1561 (1999).

  27. T. Ethvignot, M. Devlin, H. Duarte, et al., “Neutron multiplicity in the fission of 238U and 235U with neutrons up to 200 MeV,” Phys. Rev. Lett., 94, 052701–052707 (2005).

    Article  ADS  Google Scholar 

  28. V. M. Maslov, N. V. Kornilov, A. B. Kagalenko, et al., “Prompt fission neutron spectra of 233U above emissive fission threshold,” Nucl. Phys., A760, 274– 302 (2005).

    ADS  Google Scholar 

  29. V. M. Maslov, Yu. V. Porodzinskij, M. Baba, et al., “Prompt fission neutron spectra of 238U and 2j2Th above emissive fission threshold,” Phys. Rev., C69, 034607–034618 (2004).

    ADS  Google Scholar 

  30. J. Frehaut, A. Berlin, and R. Bois, Measurement of the fission neutron energy spectra for the fast neutron induced fission of U-235 and U-238,” in: Neutron Physics. Proc. 3rd All-Union Conf. on Neutron Physics, June 9–13, 1975, Kiev, Vol. 5, TsNIIatominform (1976), pp. 349–355.

  31. International Handbook of Evaluated Criticality Safety Benchmark Experiments, NEA/NSC/DOC(95)03/IV, OECD-NEA (2001).

  32. J. Both, A. Mazzolo, O. Petit, et al., TRIPOLI-4.3 User Manual for Version of 4.3 of the TRIPOLI-4 Monte Carlo Particle Transport Computer Code, CEA/Saclay, France, Nov. 2003.

  33. Zolotarev K. I., Re-Evaluation of Integral and Microscopic Cross Section Data for Important Dosimetry Reactions, IAEA, Vienna, INDC(NDS)-0526 (2008).

  34. W. Mannhart, “Status of the evaluation of the neutron spectrum of 235U + n lh ,” in: Int. Neutron Cross Section Standards: Measurements and Evaluation Techniques. IAEA Consultants’ Meeting, Vienna, October 13–15, 2008, IAEA, Vienna (2008), p. 27.

  35. O. Horibe, Y. Mizumoto, T. Kusakabe, and H. Chatani, “U-235 fission neutron spectrum averaged cross sections measured for some threshold reactions on Mg, Al, Ca, Sc, Ti, Fe, Co, Ni, Zn, Sr, Mo, Rh, In and Ce,” in: Prop. Conf. 50 Years with Nuclear Fission, Gaithersburg, USA, American Nuclear Society, Inc., April 25–28, 1989, Vol. 2, pp. 923–930.

  36. I. Kimura and K. Kobayashi, “Calibrated fission and fusion fields at the Kyoto university reactor,” Nucl. Sci. Eng., 106, 332–344 (1990).

    Google Scholar 

  37. J. Boldeman, “Fission spectrum averaged cross sections of threshold reactions,” Nucl. Energy, A/B 18, 417−424 (1964).

    Google Scholar 

  38. T. Sekine and H. Baba, “Cross sections of the (n, 2n) reaction of Co-59, Ni-58, Ge-70, Zr-90 and Tl-203 with fission neutrons,” Inorg. Nucl. Chem., 43, 1427–1437 (1981).

    Article  Google Scholar 

  39. K. Kobayashi and I. Kimura, “Fission averaged cross sections for the 93Nb(n, n′)93mNb and 199Hg(n, n′)l99mHg reactions,” in: Progress Report NEANDC(J)-61U, Japan Atomic Energy Research Institute, Tokai-Mura, Ibarakiken, Japan, September 1979, p. 78–80.

  40. K. Kobayashi, S. Yamamoto, and I. Kimura, “The U-235 fission spectrum averaged cross section for the 199Hg(n, n′)199mHg reaction processed with covariances between the data uncertainties,” in: Ann. Rep. of the Research Reactor Institute, Kyoto University, Japan, KURRI-AR-14 (1981), pp. 1–9.

Download references

Author information

Authors and Affiliations

Authors

Additional information

Translated from Atomnaya Énergiya, Vol. 108, No. 6, pp. 352–362, June, 2010.

Rights and permissions

Reprints and permissions

About this article

Cite this article

Maslov, V.M., Tetereva, N.A., Pronyaev, V.G. et al. Spectrum of prompt fission neutrons from 235U(n, F). At Energy 108, 432–443 (2010). https://doi.org/10.1007/s10512-010-9313-0

Download citation

  • Received:

  • Published:

  • Issue Date:

  • DOI: https://doi.org/10.1007/s10512-010-9313-0

Keywords

Navigation